Interface‐Induced Stability of Nontrivial Topological Spin Textures: Unveiling Room‐Temperature Hopfions and Skyrmions

Katmis, Ferhat; Lauter, Valeria; Yagan, Rawana; Brandt, Iuri S.; Cheghabouri, Arash M.; Zhou, Hua; Freeland, John W.; de Araujo, Clodoaldo I. L.; Jamer, Michelle E.; Heiman, Don; Onbasli, Mehmet C.; Moodera, Jagadeesh S.

doi:10.1002/adma.202511754

Interface‐Induced Stability of Nontrivial Topological Spin Textures: Unveiling Room‐Temperature Hopfions and Skyrmions

Journal Article · Mon Aug 18 00:00:00 EDT 2025 · Advanced Materials

DOI:https://doi.org/10.1002/adma.202511754· OSTI ID:2584458

^[1]; ^[2]; Yagan, Rawana ^[3]; Brandt, Iuri S. ^[4]; Cheghabouri, Arash M. ^[3]; Zhou, Hua ^[5]; Freeland, John W. ^[5]; de Araujo, Clodoaldo I. L. ^[4]; Jamer, Michelle E. ^[6]; Heiman, Don ^[7]; Onbasli, Mehmet C. ^[3]; Moodera, Jagadeesh S. ^[1]

Massachusetts Institute of Technology, Cambridge, MA (United States)
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Koç University, Istanbul (Türkiye)
Universidade Federal de Viçosa (Brazil)
Argonne National Laboratory (ANL), Argonne, IL (United States)
United States Naval Academy, Annapolis, MD (United States)
Massachusetts Institute of Technology, Cambridge, MA (United States); Northeastern University, Boston, MA (United States)

Topological spin configurations, such as soliton-like spin texture and Dirac electron assemblies, have recently emerged in fundamental science and technology. Achieving stable topological spin textures at room temperature is crucial for their use as long-range information carriers. However, their creation and manipulation are hindered by multi-step field training and competing interactions. Thus, a spontaneous ground state for multidimensional topological spin textures is desirable, with skyrmions forming swirling, hedgehog-like spin structures in two dimensions and hopfions as their twisted 3D counterparts. Here, the first observation of robust and reproducible topological spin textures of hopfions and skyrmions observed at room temperature and in zero magnetic field is reported, which are stabilized by geometric confinement and protected by interfacial magnetism in a ferromagnet/topological insulator/ferromagnet trilayer heterostructure. These skyrmion-hopfion configurations are directly observed at room temperature with Lorenz transmission electron microscopy. Using micromagnetic modeling, the experimental observations of hopfion-skyrmion assemblies are reproduced. This model reveals a complete picture of how spontaneously organized skyrmion lattices encircled by hopfion rings are controlled by surface electrons, uniaxial anisotropy, and Dzyaloshinskii-Moriya interaction. This study provides evidence that topological chiral spin textures can facilitate the development of magnetic topological carriers, paving the way for ultralow-power and high-density information processing.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: Army Research Office; European Research Council; National Science Foundation; Office of Naval Research; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357; AC05-00OR22725

Other Award/Contract Number:: ARO W911NF‐20‐2‐0061
DMR‐1905662
1207469
N00014‐20‐1‐2306
N00014‐13‐1‐0301
948063

OSTI ID:: 2584458

Journal Information:: Advanced Materials, Journal Name: Advanced Materials; ISSN 1521-4095; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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