Production of neutron-rich isotopes for 𝑍 ≥ 98 in the 238U + 248Cm reaction

Ocal, S. E.; Yilmaz, O.; Arik, M.; Ayik, S.; Umar, A. S.

doi:10.1103/PhysRevC.111.054613

Production of neutron-rich isotopes for 𝑍 ≥ 98 in the ²³⁸U + ²⁴⁸Cm reaction

Journal Article · Mon May 12 00:00:00 EDT 2025 · Physical Review. C

DOI:https://doi.org/10.1103/PhysRevC.111.054613· OSTI ID:2568299

^[1]; Yilmaz, O. ^[1]; Arik, M. ^[2]; ^[3]; ^[2]

Middle East Technical University, Ankara (Turkey)
Vanderbilt University, Nashville, TN (United States)
Tennessee Technological University, Cookeville, TN (United States)

Multinucleon transfer (MNT) reactions in actinide systems are a promising method to synthesize transuranium neutron-rich elements. Appropriate theoretical approaches are needed to understand the mechanisms behind MNT. We employ a microscopic approach to calculate neutron-rich isotope production in the reaction ²³⁸U + ²⁴⁸Cm system. Here, the stochastic mean-field (SMF) approach is used to calculate the primary cross sections in MNT reactions based on the quasifission and inverse quasifission processes, and a statistical de-excitation model with GEMINI₊₊ code to calculate the secondary fragment cross sections. The calculated cross sections using SMF and GEMINI₊₊ explain available experimental results for the ²³⁸U + ²⁴⁸Cm system at 𝐸_c.m. = 898.7 MeV energy. This shows the effectiveness and applicability of the quantal diffusion approach, based on the SMF theory, in heavy-ion collisions. Production of transuranium neutron-rich elements with a proton number up to 𝑍=101 is obtained with sizable cross sections. Theoretical results calculated for the 𝑍=102–105 region, for which there are no experimental data, show that the cross-section values would be lower than the microbarn level. SMF theory does not contain any adjustable parameters other than the standard parameters of the energy density functional used in the TDHF theory and is an important approach for the microscopic understanding of reaction mechanisms.

View Accepted Manuscript (DOE)

Research Organization:: Vanderbilt University, Nashville, TN (United States)

Sponsoring Organization:: TUBITAK; USDOE

Grant/Contract Number:: SC0013847

OSTI ID:: 2568299

Alternate ID(s):: OSTI ID: 2565770

Journal Information:: Physical Review. C, Journal Name: Physical Review. C Journal Issue: 5 Vol. 111; ISSN 2469-9985; ISSN 2469-9993

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (67)

Nuclear Ground-State Masses and Deformations Moller, P.; Nix, J. R.; Myers, W. D. Atomic Data and Nuclear Data Tables, Vol. 59, Issue 2, p. 185-381 https://doi.org/10.1006/adnd.1995.1002	journal	March 1995
Theoretical Nuclear Physics Blatt, John M.; Weisskopf, Victor F. https://doi.org/10.1007/978-1-4612-9959-2	book	January 1979
The Fokker-Planck Equation Risken, Hannes Springer Series in Synergetics https://doi.org/10.1007/978-3-642-61544-3	book	January 1996
Microscopic transport theory of heavy-ion collisions: V. transfer of neutrons and protons Merchant, A. C.; N�renberg, W. Zeitschrift f�r Physik A Atoms and Nuclei, Vol. 308, Issue 4 https://doi.org/10.1007/BF01415880	journal	December 1982
Time-dependent variational principle for the expectation value of an observable: Mean-field applications Balian, Roger; Vénéroni, Marcel Annals of Physics, Vol. 164, Issue 2 https://doi.org/10.1016/0003-4916(85)90020-X	journal	October 1985
Correlations and fluctuations in static and dynamic mean-field approaches Balian, Roger; Vénéroni, Marcel Annals of Physics, Vol. 216, Issue 2 https://doi.org/10.1016/0003-4916(92)90181-K	journal	June 1992
The role of the compound nucleus in complex fragment emission at low and intermediate energies Moretto, Luciano G.; Wozniak, Gordon J. Progress in Particle and Nuclear Physics, Vol. 21 https://doi.org/10.1016/0146-6410(88)90036-1	journal	January 1988
Memory effects in the energy dissipation for slow collective nuclear motion Nörenberg, W. Physics Letters B, Vol. 104, Issue 2 https://doi.org/10.1016/0370-2693(81)90570-0	journal	August 1981
Neutron and proton diffusion in heavy-ion collisions Merchant, A. C.; Nörenberg, W. Physics Letters B, Vol. 104, Issue 1 https://doi.org/10.1016/0370-2693(81)90844-3	journal	August 1981
Correlated mass and charge transport induced by statistical nucleon exchange in damped nuclear reactions Schröder, W. U.; Huizenga, J. R.; Randrup, J. Physics Letters B, Vol. 98, Issue 5 https://doi.org/10.1016/0370-2693(81)90924-2	journal	January 1981
Statistical emission of large fragments: A general theoretical approach Moretto, Luciano G. Nuclear Physics A, Vol. 247, Issue 2 https://doi.org/10.1016/0375-9474(75)90632-6	journal	August 1975
Theory of transfer-induced transport in nuclear collisions Randrup, J. Nuclear Physics A, Vol. 327, Issue 2 https://doi.org/10.1016/0375-9474(79)90271-9	journal	September 1979
Time-dependent HF approach to SHE dynamics Umar, A. S.; Oberacker, V. E. Nuclear Physics A, Vol. 944 https://doi.org/10.1016/j.nuclphysa.2015.02.011	journal	December 2015
Syntheses of transuranium isotopes with atomic numbers Z≤ 103 in multi-nucleon transfer reactions Kratz, J. V.; Loveland, W.; Moody, K. J. Nuclear Physics A, Vol. 944 https://doi.org/10.1016/j.nuclphysa.2015.06.004	journal	December 2015
A stochastic mean-field approach for nuclear dynamics Ayik, Sakir Physics Letters B, Vol. 658, Issue 4 https://doi.org/10.1016/j.physletb.2007.09.072	journal	January 2008
New neutron-rich isotope production in 154 Sm+ 160 Gd Wang, Ning; Guo, Lu Physics Letters B, Vol. 760 https://doi.org/10.1016/j.physletb.2016.06.073	journal	September 2016
Optimal condition for the production of heavy and superheavy neutron-rich isotopes with multinucleon transfer reaction Bao, Xiao Jun Physics Letters B, Vol. 833 https://doi.org/10.1016/j.physletb.2022.137307	journal	October 2022
Heavy-ion collisions and fission dynamics with the time-dependent Hartree–Fock theory and its extensions Simenel, C.; Umar, A. S. Progress in Particle and Nuclear Physics, Vol. 103 https://doi.org/10.1016/j.ppnp.2018.07.002	journal	November 2018
Three-dimensional TDHF calculations for reactions of unstable nuclei Kim, Ka-Hae; Otsuka, Takaharu; Bonche, Paul Journal of Physics G: Nuclear and Particle Physics, Vol. 23, Issue 10 https://doi.org/10.1088/0954-3899/23/10/014	journal	October 1997
New way for the production of heavy neutron-rich nuclei Zagrebaev, Valery; Greiner, Walter Journal of Physics G: Nuclear and Particle Physics, Vol. 35, Issue 12 https://doi.org/10.1088/0954-3899/35/12/125103	journal	September 2008
The Inelastic Scattering of Neutrons Hauser, Walter; Feshbach, Herman Physical Review, Vol. 87, Issue 2 https://doi.org/10.1103/PhysRev.87.366	journal	July 1952
Quantal diffusion approach for multinucleon transfers in Xe + Pb collisions Ayik, S.; Yilmaz, B.; Yilmaz, O. Physical Review C, Vol. 100, Issue 1 https://doi.org/10.1103/PhysRevC.100.014609	journal	July 2019
Deformed shell effects in Ca 48 + Bk 249 quasifission fragments Godbey, K.; Umar, A. S.; Simenel, C. Physical Review C, Vol. 100, Issue 2 https://doi.org/10.1103/PhysRevC.100.024610	journal	August 2019
Microscopic predictions for the production of neutron-rich nuclei in the reaction Yb 176 + Yb 176 Godbey, K.; Simenel, C.; Umar, A. S. Physical Review C, Vol. 101, Issue 3 https://doi.org/10.1103/PhysRevC.101.034602	journal	March 2020
Quantal diffusion approach for multinucleon transfer processes in the Ni 58 , 64 + Pb 208 reactions: Toward the production of unknown neutron-rich nuclei Sekizawa, Kazuyuki; Ayik, Sakir Physical Review C, Vol. 102, Issue 1 https://doi.org/10.1103/PhysRevC.102.014620	journal	July 2020
Merging of transport theory with the time-dependent Hartree-Fock approach: Multinucleon transfer in U + U collisions Ayik, S.; Yilmaz, B.; Yilmaz, O. Physical Review C, Vol. 102, Issue 2 https://doi.org/10.1103/PhysRevC.102.024619	journal	August 2020
Quantal diffusion description of isotope production via the multinucleon transfer mechanism in Ca48+U238 collisions Ayik, S.; Arik, M.; Karanfil, E. C. Physical Review C, Vol. 104, Issue 5 https://doi.org/10.1103/PhysRevC.104.054614	journal	November 2021
Multinucleon transfer mechanism inCf250+Th232collisions using the quantal transport description based on the stochastic mean-field approach Ayik, S.; Arik, M.; Yilmaz, O. Physical Review C, Vol. 107, Issue 1 https://doi.org/10.1103/PhysRevC.107.014609	journal	January 2023
Exploring the optimal way to produce Z=100–106 neutron-rich nuclei Zhao, Tian Liang; Bao, Xiao Jun; Zhang, Hong Fei Physical Review C, Vol. 108, Issue 2 https://doi.org/10.1103/PhysRevC.108.024602	journal	August 2023
Multinucleon transfer mechanism in Gd160+W186 collisions in stochastic mean-field theory Ayik, S.; Arik, M.; Erbayri, E. Physical Review C, Vol. 108, Issue 5 https://doi.org/10.1103/PhysRevC.108.054605	journal	November 2023
Exploring the optimal way to produce new nuclides in the region of heavy and superheavy nuclei Zhao, Tian Liang; Zhu, Shi Hao; Zhang, Hong Fei Physical Review C, Vol. 110, Issue 6 https://doi.org/10.1103/PhysRevC.110.064609	journal	December 2024
Nuclear Hartree-Fock calculations with splines Umar, A. S.; Strayer, M. R.; Wu, J. -S. Physical Review C, Vol. 44, Issue 6 https://doi.org/10.1103/PhysRevC.44.2512	journal	December 1991
Conclusive evidence for the influence of nuclear orientation on quasifission Hinde, D. J.; Dasgupta, M.; Leigh, J. R. Physical Review C, Vol. 53, Issue 3 https://doi.org/10.1103/PhysRevC.53.1290	journal	March 1996
Three-dimensional unrestricted time-dependent Hartree-Fock fusion calculations using the full Skyrme interaction Umar, A. S.; Oberacker, V. E. Physical Review C, Vol. 73, Issue 5 https://doi.org/10.1103/PhysRevC.73.054607	journal	May 2006
Quantum molecular dynamics study of the mass distribution of products in 7.0 A MeV U 238 + U 238 collisions Zhao, Kai; Wu, Xizhen; Li, Zhuxia Physical Review C, Vol. 80, Issue 5 https://doi.org/10.1103/PhysRevC.80.054607	journal	November 2009
Production of heavy isotopes in transfer reactions by collisions of U 238 + U 238 Feng, Zhao-Qing; Jin, Gen-Ming; Li, Jun-Qing Physical Review C, Vol. 80, Issue 6 https://doi.org/10.1103/PhysRevC.80.067601	journal	December 2009
New inverse quasifission mechanism to produce neutron-rich transfermium nuclei Kedziora, David J.; Simenel, Cédric Physical Review C, Vol. 81, Issue 4 https://doi.org/10.1103/PhysRevC.81.044613	journal	April 2010
Systematic description of evaporation spectra for light and heavy compound nuclei Charity, R. J. Physical Review C, Vol. 82, Issue 1 https://doi.org/10.1103/PhysRevC.82.014610	journal	July 2010
Production of heavy and superheavy neutron-rich nuclei in transfer reactions Zagrebaev, V. I.; Greiner, Walter Physical Review C, Vol. 83, Issue 4 https://doi.org/10.1103/PhysRevC.83.044618	journal	April 2011
Reexamining the heavy-ion reactions 238 U+ 238 U and 238 U+ 248 Cm and actinide production close to the barrier Kratz, J. V.; Schädel, M.; Gäggeler, H. W. Physical Review C, Vol. 88, Issue 5 https://doi.org/10.1103/PhysRevC.88.054615	journal	November 2013
Dissipative dynamics in quasifission Oberacker, V. E.; Umar, A. S.; Simenel, C. Physical Review C, Vol. 90, Issue 5 https://doi.org/10.1103/PhysRevC.90.054605	journal	November 2014
Shape evolution and collective dynamics of quasifission in the time-dependent Hartree-Fock approach Umar, A. S.; Oberacker, V. E.; Simenel, C. Physical Review C, Vol. 92, Issue 2 https://doi.org/10.1103/PhysRevC.92.024621	journal	August 2015
Time-dependent Hartree-Fock calculations for multinucleon transfer and quasifission processes in the Ni 64 + U 238 reaction Sekizawa, Kazuyuki; Yabana, Kazuhiro Physical Review C, Vol. 93, Issue 5 https://doi.org/10.1103/PhysRevC.93.054616	journal	May 2016
Production of unknown neutron-rich isotopes in U 238 + U 238 collisions at near-barrier energy Zhao, Kai; Li, Zhuxia; Zhang, Yingxun Physical Review C, Vol. 94, Issue 2 https://doi.org/10.1103/PhysRevC.94.024601	journal	August 2016
Production of neutron-rich isotopes around N = 126 in multinucleon transfer reactions Feng, Zhao-Qing Physical Review C, Vol. 95, Issue 2 https://doi.org/10.1103/PhysRevC.95.024615	journal	February 2017
Modeling near-barrier collisions of heavy ions based on a Langevin-type approach Karpov, A. V.; Saiko, V. V. Physical Review C, Vol. 96, Issue 2 https://doi.org/10.1103/PhysRevC.96.024618	journal	August 2017
Transport properties of isospin asymmetric nuclear matter using the time-dependent Hartree-Fock method Umar, A. S.; Simenel, C.; Ye, W. Physical Review C, Vol. 96, Issue 2 https://doi.org/10.1103/PhysRevC.96.024625	journal	August 2017
Quantal diffusion description of multinucleon transfers in heavy-ion collisions Ayik, S.; Yilmaz, B.; Yilmaz, O. Physical Review C, Vol. 97, Issue 5 https://doi.org/10.1103/PhysRevC.97.054618	journal	May 2018
Analysis of multinucleon transfer reactions with spherical and statically deformed nuclei using a Langevin-type approach Saiko, V. V.; Karpov, A. V. Physical Review C, Vol. 99, Issue 1 https://doi.org/10.1103/PhysRevC.99.014613	journal	January 2019
Production of New Heavy Isotopes in Low-Energy Multinucleon Transfer Reactions Zagrebaev, Valery; Greiner, Walter Physical Review Letters, Vol. 101, Issue 12 https://doi.org/10.1103/PhysRevLett.101.122701	journal	September 2008
Particle Transfer Reactions with the Time-Dependent Hartree-Fock Theory Using a Particle Number Projection Technique Simenel, Cédric Physical Review Letters, Vol. 105, Issue 19 https://doi.org/10.1103/PhysRevLett.105.192701	journal	November 2010
Particle-Number Fluctuations and Correlations in Transfer Reactions Obtained Using the Balian-Vénéroni Variational Principle Simenel, Cédric Physical Review Letters, Vol. 106, Issue 11 https://doi.org/10.1103/PhysRevLett.106.112502	journal	March 2011
Exploring Zeptosecond Quantum Equilibration Dynamics: From Deep-Inelastic to Fusion-Fission Outcomes in Ni 58 + Ni 60 Reactions Williams, E.; Sekizawa, K.; Hinde, D. J. Physical Review Letters, Vol. 120, Issue 2 https://doi.org/10.1103/PhysRevLett.120.022501	journal	January 2018
Timescales of Quantum Equilibration, Dissipation and Fluctuation in Nuclear Collisions Simenel, C.; Godbey, K.; Umar, A. S. Physical Review Letters, Vol. 124, Issue 21 https://doi.org/10.1103/PhysRevLett.124.212504	journal	May 2020
Discovery of New Isotope U241 and Systematic High-Precision Atomic Mass Measurements of Neutron-Rich Pa-Pu Nuclei Produced via Multinucleon Transfer Reactions Niwase, T.; Watanabe, Y. X.; Hirayama, Y. Physical Review Letters, Vol. 130, Issue 13 https://doi.org/10.1103/PhysRevLett.130.132502	journal	March 2023
Actinide Production in Collisions of U 238 with Cm 248 Schädel, M.; Brüchle, W.; Gäggeler, H. Physical Review Letters, Vol. 48, Issue 13 https://doi.org/10.1103/PhysRevLett.48.852	journal	March 1982
Time-dependent density-functional description of nuclear dynamics Nakatsukasa, Takashi; Matsuyanagi, Kenichi; Matsuo, Masayuki Reviews of Modern Physics, Vol. 88, Issue 4 https://doi.org/10.1103/RevModPhys.88.045004	journal	November 2016
Nuclear quantum many-body dynamics: From collective vibrations to heavy-ion collisions Simenel, Cédric The European Physical Journal A, Vol. 48, Issue 11 https://doi.org/10.1140/epja/i2012-12152-0	journal	November 2012
Stochastic quantum dynamics beyond mean field Lacroix, Denis; Ayik, Sakir The European Physical Journal A, Vol. 50, Issue 6 https://doi.org/10.1140/epja/i2014-14095-8	journal	June 2014
How to extend the chart of nuclides? Adamian, G. G.; Antonenko, N. V.; Diaz-Torres, A. The European Physical Journal A, Vol. 56, Issue 2 https://doi.org/10.1140/epja/s10050-020-00046-7	journal	February 2020
Quasi-fission and fusion-fission reactions in $$^{48}\hbox {Ca}+^{208}\hbox {Pb}$$48Ca+208Pb collisions at $$\hbox {E}_{\mathrm{c.m.}}=190\ \hbox {MeV}$$Ec.m.=190MeV Yilmaz, O.; Turan, G.; Yilmaz, B. The European Physical Journal A, Vol. 56, Issue 2 https://doi.org/10.1140/epja/s10050-020-00053-8	journal	February 2020
Multinucleon transfer as a method for production of new heavy neutron-enriched isotopes of transuranium elements Saiko, Vyacheslav; Karpov, Alexander The European Physical Journal A, Vol. 58, Issue 3 https://doi.org/10.1140/epja/s10050-022-00688-9	journal	March 2022
Production of neutron-rich heavy nuclei around $$N = 162$$ in multinucleon transfer reactions Peng, Cheng; Feng, Zhao-Qing The European Physical Journal A, Vol. 58, Issue 9 https://doi.org/10.1140/epja/s10050-022-00819-2	journal	September 2022
Heavy and superheavy elements: next generation experiments, ideas and considerations Münzenberg, G.; Gupta, M.; Devaraja, H. M. The European Physical Journal A, Vol. 59, Issue 2 https://doi.org/10.1140/epja/s10050-023-00939-3	journal	February 2023
A theoretical study on quasifission and fusion–fission processes in heavy-ion collisions Kayaalp, A.; Ocal, S. E.; Yaprakli, B. The European Physical Journal A, Vol. 60, Issue 4 https://doi.org/10.1140/epja/s10050-024-01303-9	journal	April 2024
Quantum Dissipative Systems Weiss, Ulrich https://doi.org/10.1142/4239	book	October 1999
Quasifission Dynamics in Microscopic Theories Godbey, Kyle; Umar, A. S. Frontiers in Physics, Vol. 8 https://doi.org/10.3389/fphy.2020.00040	journal	February 2020

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Production of neutron-rich isotopes for 𝑍 ≥ 98 in the 238U + 248Cm reaction

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Production of neutron-rich isotopes for 𝑍 ≥ 98 in the ²³⁸U + ²⁴⁸Cm reaction