Quantal diffusion approach for multinucleon transfer processes in the 58,64Ni + 208Pb reactions: Toward the production of unknown neutron-rich nuclei

Sekizawa, Kazuyuki; Ayik, Sakir

doi:10.1103/physrevc.102.014620

Quantal diffusion approach for multinucleon transfer processes in the ^58,64Ni + ²⁰⁸Pb reactions: Toward the production of unknown neutron-rich nuclei

Journal Article · Mon Jul 27 00:00:00 EDT 2020 · Physical Review C

DOI:https://doi.org/10.1103/physrevc.102.014620· OSTI ID:1657081

^[1]; ^[2]

Niigata Univ. (Japan); Univ. of Tsukuba, Ibaraki (Japan); Tennessee Technological University
Tennessee Technological Univ., Cookeville, TN (United States)

In recent years, substantial efforts have been made for the study of multinucleon transfer reactions at energies around the Coulomb barrier both experimentally and theoretically, aiming at the production of unknown neutron-rich heavy nuclei. It is crucial to provide reliable theoretical predictions based on microscopic theories with sufficient predictive power. Purpose: This article aims to clarify the applicability of the quantal diffusion approach based on the stochastic mean-field (SMF) theory for multinucleon transfer processes. Isotope production cross sections are evaluated for the reactions of ⁶⁴Ni + ²⁰⁸Pb at E_c.m. = 268 MeV and ⁵⁸Ni + ²⁰⁸Pb at E_c.m. = 270 MeV and are compared with available experimental data. Methods: Three-dimensional time-dependent Hartree-Fock (TDHF) calculations are carried out for a range of initial orbital angular momenta with Skyrme SLy4d functional. Quantal diffusion equations, derived based on the SMF theory, for variances and covariance of neutron and proton numbers of reaction products are solved, with microscopic drift and diffusion coefficients obtained from time evolution of occupied single-particle orbitals in TDHF. Secondary de-excitation processes, both particle evaporation and fission, are simulated by a statistical compound-nucleus de-excitation model, gemini++. Dynamics of a fast isospin equilibration process followed by a slow drift toward the mass symmetry are commonly observed, as expected. Various reaction outcomes are evaluated, including average mass and charge numbers of reaction products, total kinetic energy loss (TKEL), scattering angle, contact time, and production cross sections for primary and secondary products. By comparing with the experimental data, we find that SMF and TDHF quantitatively reproduce experimental data for few-nucleon-transfer channels around the average values. In contrast, for many-nucleon-transfer channels, we find that the SMF approach provides much better description of the experimentally measured isotopic distributions. The results underline the importance of beyond-mean-field effects, especially one-body (mean-field) fluctuations and correlations, in describing multinucleon transfer processes. Moreover, through a combined analysis of SMF with a statistical model, gemini++, we find a significant contribution of transfer-induced fission, which is consistent with the experimental observation. In some cases, the SMF approach overestimates the isotopic width, requiring further improvements of the theoretical description. Possible ways to improve the description are discussed. The SMF approach is designed to describe the quantum many-body problem according to an ensemble of mean-field trajectories, taking into account part of many-body correlations in the description. As it requires feasible computational costs comparable to the ordinary TDHF approach, together with further model improvements, it will be a promising tool in the search for optimal reaction conditions to produce yet-unknown neutron-rich heavy nuclei through the multinucleon transfer reaction.

View Accepted Manuscript (DOE)

Research Organization:: Tennessee Technological Univ., Cookeville, TN (United States)

Sponsoring Organization:: JSPS; USDOE Office of Science (SC), Nuclear Physics (NP)

Grant/Contract Number:: SC0015513

Other Award/Contract Number:: 19K14704

OSTI ID:: 1657081

Journal Information:: Physical Review C, Journal Name: Physical Review C Journal Issue: 1 Vol. 102; ISSN 2469-9985

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Quantal diffusion approach for multinucleon transfer processes in the 58,64Ni + 208Pb reactions: Toward the production of unknown neutron-rich nuclei

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Quantal diffusion approach for multinucleon transfer processes in the ^58,64Ni + ²⁰⁸Pb reactions: Toward the production of unknown neutron-rich nuclei