Extended Kohler's rule of magnetoresistance in TaCo2 Te2

Pate, Samuel; Chen, Bowen; Shen, Bing; Li, Kezhen; Zhou, Xiuquan; Chung, Duck Young; Divan, Ralu; Kanatzidis, Mercouri G.; Welp, Ulrich; Kwok, Wai-Kwong; Xiao, Zhi-Li

doi:10.1103/physrevb.109.035129

Extended Kohler's rule of magnetoresistance in TaCo2 Te2

Journal Article · Tue Jan 16 00:00:00 EST 2024 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.109.035129· OSTI ID:2563557

Pate, Samuel ^[1]; ^[2]; Shen, Bing ^[2]; ^[1]; Zhou, Xiuquan ^[3]; ^[3]; Divan, Ralu ^[4]; Kanatzidis, Mercouri G. ^[5]; Welp, Ulrich ^[3]; Kwok, Wai-Kwong ^[3]; ^[1]

Argonne National Laboratory (ANL), Argonne, IL (United States); Northern Illinois Univ., DeKalb, IL (United States)
Sun Yat-Sen Univ., Guangzhou (China)
Argonne National Laboratory (ANL), Argonne, IL (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM)
Argonne National Laboratory (ANL), Argonne, IL (United States); Northwestern Univ., Evanston, IL (United States)

TaCo₂Te₂ is recently reported to be an air-stable, high mobility van der Waals material with probable magnetic order. Here we investigate the scaling behavior of its magnetoresistance. Here we measured both the longitudinal (p_xx) and Hall (p_xy) magnetoresistivities of TaCo₂Te₂ crystals in magnetic fields parallel to the c axis and found that the magnetoresistance violates the Kohler's rule MR similar to f [H/p₀] while obeying the extended Kohler's rule MR ~ f [H/(n_T p₀)], where MR ~ [p_xx(H) - p₀]/p₀, H is the magnetic field, n_T is a thermal factor, and p_xx(H) and p₀ are the resistivities at H and zero field, respectively. Further, while deviating from those of the densities of electrons (n_e) and holes (n_h) obtained from the two-band model analysis of the magnetoconductivities, the temperature dependence of n_T is close to that of the Hall carrier densities n_H calculated from the slopes of p_xy(H) curves at low magnetic fields, providing a different way to obtain the thermal factor in the extended Kohler's rule.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM)

Sponsoring Organization:: National Natural Science Foundation of China (NSFC); National Science Foundation (NSF); Natural Science Foundation of Guangdong Province; USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 2563557

Alternate ID(s):: OSTI ID: 2474188

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 3 Vol. 109; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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