Quantifying silicon anode restructuring during calendar aging of lithium-ion batteries by plasma focused ion beam tomography and chemical mapping

Quinn, Joseph; Badami, Pavan; Huang, Qian; Wang, Chongmin; Abraham, Daniel P.

doi:10.1039/D5EB00036J

Quantifying silicon anode restructuring during calendar aging of lithium-ion batteries by plasma focused ion beam tomography and chemical mapping

Journal Article · Wed Jan 01 00:00:00 EST 2025 · EES Batteries

DOI:https://doi.org/10.1039/D5EB00036J· OSTI ID:2562964

^[1]; Badami, Pavan ^[2]; ^[1]; ^[3]; ^[2]

Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, WA 99354, USA
Chemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, Illinois, 60439, USA
Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington 99354, USA

A characterization technique was developed to generate 3D chemo-mechanical reconstructions of battery microstructures. The technique was used to observe degradation mechanisms caused by aging over time in Si anode-based lithium-ion batteries.

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Sponsoring Organization:: USDOE

OSTI ID:: 2562964

Journal Information:: EES Batteries, Journal Name: EES Batteries; ISSN EBEAA5; ISSN 3033-4071

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

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Quantifying silicon anode restructuring during calendar aging of lithium-ion batteries by plasma focused ion beam tomography and chemical mapping

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