Measurement of {sup 235}U content and flow of UF{sub 6} using delayed neutrons or gamma rays following induced fission
Feasibility experiments conducted at Pacific Northwest National Laboratory demonstrate that either delayed neutrons or energetic gamma rays from short-lived fission products can be used to monitor the blending of UF{sub 6} gas streams. A {sup 252}Cf neutron source was used to induce {sup 235}U fission in a sample, and delayed neutrons and gamma rays were measured after the sample moved {open_quotes}down-stream.{close_quotes} The experiments used a UO{sub 2} powder that was transported down the pipe to simulate the flowing UF{sub 6} gas. Computer modeling and analytic calculation extended the test results to a flowing UF{sub 6} gas system. Neutron or gamma-ray measurements made at two downstream positions can be used to indicate both the {sup 235}U content and UF{sub 6} flow rate. Both the neutron and gamma-ray techniques have the benefits of simplicity and long-term reliability, combined with adequate sensitivity for low-intrusion monitoring of the blending process. Alternatively, measuring the neutron emission rate from (a, n) reactions in the UF{sub 6} provides an approximate measure of the {sup 235}U content without using a neutron source to induce fission.
- Research Organization:
- Pacific Northwest Lab., Richland, WA (United States)
- Sponsoring Organization:
- USDOE, Washington, DC (United States)
- DOE Contract Number:
- AC06-76RL01830
- OSTI ID:
- 253194
- Report Number(s):
- PNNL--11210; ON: DE96012326
- Country of Publication:
- United States
- Language:
- English
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