Orientation Sensitive SEIRA Sensors Based on Single-Walled Carbon Nanotube Near Fields

Georgiou, Kyriacos; Wang, Yulei; Ma, Xuedan

doi:10.1021/acs.nanolett.4c02618

Orientation Sensitive SEIRA Sensors Based on Single-Walled Carbon Nanotube Near Fields

Journal Article · Wed Aug 14 00:00:00 EDT 2024 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.4c02618· OSTI ID:2523626

^[1]; Wang, Yulei ^[1]; ^[2]

Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM); University of Chicago, IL (United States)
Argonne National Laboratory (ANL), Argonne, IL (United States). Center for Nanoscale Materials (CNM); University of Chicago, IL (United States); Rice University, Houston, TX (United States)

Molecular vibrations that bear information about intrinsic properties of chemical compounds are challenging to detect at submonolayer densities. Surface-enhanced infrared absorption (SEIRA) spectroscopy has been proven to be a viable approach to enhance and detect weak vibration signals. Here, in this study, we report a SEIRA sensor based on mid-infrared surface plasmon resonances supported by single-walled carbon nanotubes (SWCNTs). Due to the 1D nature of SWCNTs, their plasmon modes are highly polarized with the electromagnetic fields spatially confined to nanometer scales. Leveraging these characteristics of SWCNTs, we observe a polarization selective coupling between their surface plasmons and vibrational modes of chemical bonds introduced onto their surfaces. A maximum modulation of similar to 15% to the plasmon resonance peak is obtained for a submonolayer chemical group coverage. These findings suggest that SWCNTs may potentially serve as a highly sensitive SEIRA platform for revealing intricate information about molecular compositions and bond orientations.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 2523626

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 34 Vol. 24; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
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infrared absorption
molecular vibration
surface plasmon

Orientation Sensitive SEIRA Sensors Based on Single-Walled Carbon Nanotube Near Fields

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