Role of CeNiSi2 and BaNiSn3 Structure Types in the Emergent Magnetism of the Homologous Series Lnn+1MnX3n+1:Ce4Fe3Ge10

Montero, Alexis Dominguez; Stoian, Sebastian A.; McCandless, Gregory T.; Baumbach, Ryan E.; Chan, Julia Y.

doi:10.1021/acs.chemmater.4c01938

Role of CeNiSi₂ and BaNiSn₃ Structure Types in the Emergent Magnetism of the Homologous Series Ln_n+1M_nX_3n+1:Ce₄Fe₃Ge₁₀

Journal Article · Tue Aug 27 00:00:00 EDT 2024 · Chemistry of Materials

DOI:https://doi.org/10.1021/acs.chemmater.4c01938· OSTI ID:2503905

Montero, Alexis Dominguez ^[1]; ^[2]; McCandless, Gregory T. ^[3]; Baumbach, Ryan E. ^[4]; ^[3]

Baylor University, Waco, TX (United States); Baylor University
University of Idaho, Moscow, ID (United States)
Baylor University, Waco, TX (United States)
University of California, Santa Cruz, CA (United States)

The synthesis and characterization of Ce₄Fe₃Ge₁₀, n =3 member of the homologous series Ln_n+1M_nX_3n+1 (Ln = lanthanides, M = transition metal, X = tetrel), is reported. The structure can be modelled with the Cmcm space group adopting the Eu₂Ni_2-xSn₅ structure type, with lattice parameters of a = 4.3323 (15) Å, b = 35.507 (9) Å, and c = 4.3069 (12) Å. Members of the series for n > 2 consist of stacking of ordered (CeNiSi₂ type) and disordered (BaNiSn₃/ AuCu₃ type) subunits with the acting as a “spacer” between CeNiSi₂ subunits. Although neither CeFeGe₃ nor CeFe_0.63Ge₂ order magnetically down to 2 K, Ce₄Fe₃Ge₁₀ is an antiferromagnet below 3.6 K. To rationalize the emergent magnetism: (i) we established the Kondo and RKKY interaction dominant regions for the Ce analogues adopting the BaNiSn₃ and CeNiSi₂ by creating an electronic landscape for each, (ii) mapped the strained subunits, due to stacking, within the series. Here, we established the CeFeGe₃ subunit within Ce₄Fe₃Ge₁₀ contracts and is located within the Kondo-interaction dominant region, while the CeFe_0.63Ge₂ subunit expands and is in the RKKY-interaction dominant region.

View Accepted Manuscript (DOE)

Research Organization:: Baylor University, Waco, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0022854

OSTI ID:: 2503905

Journal Information:: Chemistry of Materials, Journal Name: Chemistry of Materials Journal Issue: 17 Vol. 36; ISSN 0897-4756

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Complex Magnetic Phase Diagram in the Non-Centrosymmetric Compound CePtSi₃ Ueta, Daichi; Yoshida, Masahiro; Kobuke, Tomohiro Journal of the Physical Society of Japan, Vol. 90, Issue 6 https://doi.org/10.7566/JPSJ.90.064712	journal	June 2021
Oval-cycloidal Magnetic Structure with Phase-shift in the Non-centrosymmetric Tetragonal Compound CePdSi ₃ Ueta, Daichi; Yoshida, Masahiro; Kobuke, Tomohiro Journal of the Physical Society of Japan, Vol. 90, Issue 11 https://doi.org/10.7566/JPSJ.90.114702	journal	November 2021

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