Magnetic properties of the quasi-XY Shastry-Sutherland magnet ER2 Be2 SiO7

Brassington, A.; Ma, Q.; Sala, G.; Kolesnikov, A. I.; Taddei, K. M.; Wu, Y.; Choi, E. S.; Wang, H.; Xie, W.; Ma, J.; Zhou, H. D.; Aczel, A. A.

doi:10.1103/physrevmaterials.8.094001

Magnetic properties of the quasi-XY Shastry-Sutherland magnet ER₂ Be₂ SiO₇

Journal Article · Tue Sep 10 00:00:00 EDT 2024 · Physical Review Materials

DOI:https://doi.org/10.1103/physrevmaterials.8.094001· OSTI ID:2483425

^[1]; ^[2]; Sala, G. ^[2]; ^[2]; Taddei, K. M. ^[2]; ^[2]; ^[3]; Wang, H. ^[4]; Xie, W. ^[4]; ^[5]; ^[1]; ^[2]

Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Laboratory (MagLab)
Michigan State Univ., East Lansing, MI (United States)
Shanghai Jiao Tong Univ. (China)

Polycrystalline and single-crystal samples of the insulating Shastry-Sutherland compound Er₂⁢Be₂⁢SiO₇ were synthesized via a solid-state reaction and the floating zone method, respectively. The crystal structure, Er single-ion anisotropy, zero-field magnetic ground state, and magnetic phase diagrams along high-symmetry crystallographic directions were investigated with bulk measurement techniques, x-ray and neutron diffraction, and neutron spectroscopy. Here, we establish that Er₂⁢Be₂⁢SiO₇ crystallizes in a tetragonal space group with planes of orthogonal Er dimers and a strong preference for the Er moments to lie in the local plane perpendicular to each dimer bond. We also find that this system has a noncollinear ordered ground state in zero field with a transition temperature of 0.841 K consisting of antiferromagnetic dimers and in-plane moments. Finally, we mapped out the H-T phase diagrams for Er₂⁢Be₂⁢SiO₇ along the directions H ∥ [001], [100], and [110]. While an increasing in-plane field simply induces a phase transition to a field-polarized phase, we identify three metamagnetic transitions in the H ∥ [001] case. Single-crystal neutron diffraction results reveal that the H ∥ [001] phase diagram can be explained predominantly by the expected field-induced behavior of classical, anisotropic moments, although the microscopic origin of one phase requires further investigation.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE; USDOE Office of Science (SC), Advanced Scientific Computing Research (ASCR); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725; SC0023648

OSTI ID:: 2483425

Alternate ID(s):: OSTI ID: 2473362

Journal Information:: Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 9 Vol. 8; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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