Magnetic properties of the Shastry-Sutherland lattice material BaNd2ZnO5

Ishii, Yuto; Sala, Gabriele; Stone, Matthew B.; Garlea, Vasile O.; Calder, Stuart; Chen, Jie; Yoshida, Hiroyuki; Fukuoka, Shuhei; Yan, Jiaqiang; Dela Cruz, Clarina R.; Du, Mao-Hua; Parker, David S.; Zhang, Hao; Batista, Cristian D.; Yamaura, Kazunari; Christianson, Andrew

doi:10.1103/PhysRevMaterials.5.064418

Magnetic properties of the Shastry-Sutherland lattice material BaNd₂ZnO₅

Journal Article · Mon Jun 28 00:00:00 EDT 2021 · Physical Review Materials

DOI:https://doi.org/10.1103/PhysRevMaterials.5.064418· OSTI ID:1807237

Ishii, Yuto ^[1]; ^[2]; ^[3]; ^[3]; ^[3]; Chen, Jie ^[4]; Yoshida, Hiroyuki ^[5]; Fukuoka, Shuhei ^[6]; ^[7]; ^[3]; ^[7]; ^[7]; Zhang, Hao ^[8]; Batista, Cristian D. ^[9]; Yamaura, Kazunari ^[4]; ^[7]

Hokkaido Univ., Sapporo (Japan). Dept. of Physics; National Institute for Materials Science (NIMS), Tsukuba (Japan). International Center for Materials Nanoarchitectonics
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
National Institute for Materials Science (NIMS), Tsukuba (Japan). International Center for Materials Nanoarchitectonics; Hokkaido Univ., Sapporo (Japan). Graduate School of Chemical Sciences and Engineering
National Institute for Materials Science (NIMS), Tsukuba (Japan). International Center for Materials Nanoarchitectonics; Hokkaido Univ., Sapporo (Japan). Dept. of Physics
Hokkaido Univ., Sapporo (Japan). Dept. of Physics
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division; Univ. of Tennessee, Knoxville, TN (United States). Dept. of Physics and Astronomy
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division; Univ. of Tennessee, Knoxville, TN (United States). Dept. of Physics and Astronomy

We investigate the physical properties of the Shastry-Sutherland lattice material BaNd₂ZnO₅. Neutron diffraction, magnetic susceptibility, and specific heat measurements reveal antiferromagnetic order below 1.65 K. The magnetic order is found to be a 2–Q magnetic structure with the magnetic moments lying in the Shastry-Sutherland lattice planes comprising the tetragonal crystal structure of BaNd₂ZnO₅. The ordered moment for this structure is 1.9(1) μB per Nd ion. Inelastic neutron scattering measurements reveal that the crystal field ground state doublet is well separated from the first excited state at 8 meV. The crystal field Hamiltonian is determined through simultaneous refinement of models with both the LS coupling and intermediate coupling approximations to the inelastic neutron scattering and magnetic susceptibility data. The ground state doublet indicates that the magnetic moments lie primarily in the basal plane with magnitude consistent with the size of the determined ordered moment.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1807237

Alternate ID(s):: OSTI ID: 1863649

Journal Information:: Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 6 Vol. 5; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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