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Exchange Bias Between van der Waals Materials: Tilted Magnetic States and Field-Free Spin–Orbit-Torque Switching

Journal Article · · Advanced Materials
 [1];  [1];  [1];  [2];  [2];  [3];  [2];  [4];  [4];  [5]
  1. Cornell Univ., Ithaca, NY (United States)
  2. Columbia Univ., New York, NY (United States)
  3. Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
  4. Cornell Univ., Ithaca, NY (United States); Kavli Institute at Cornell, Ithaca, NY (United States)
  5. Cornell Univ., Ithaca, NY (United States); Kavli Institute at Cornell, Ithaca, NY (United States); Univ. of Southern California, Los Angeles, CA (United States)
Magnetic van der Waals heterostructures provide a unique platform to study magnetism and spintronics device concepts in the 2D limit. Here, studies of exchange bias from the van der Waals antiferromagnet CrSBr acting on the van der Waals ferromagnet Fe3GeTe2 (FGT) are reported. Additionally, the orientation of the exchange bias is along the in-plane easy axis of CrSBr, perpendicular to the out-of-plane anisotropy of the FGT, inducing a strongly tilted magnetic configuration in the FGT. Furthermore, the in-plane exchange bias provides sufficient symmetry breaking to allow deterministic spin–orbit torque switching of the FGT in CrSBr/FGT/Pt samples at zero applied magnetic field. A minimum thickness of the CrSBr of >10 nm is needed to provide a non-zero exchange bias at 30 K.
Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Programmable Quantum Materials (Pro-QM); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
National Science Foundation (NSF); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)
Grant/Contract Number:
AC05-00OR22725; SC0019443
OSTI ID:
2434347
Alternate ID(s):
OSTI ID: 2280703
Journal Information:
Advanced Materials, Journal Name: Advanced Materials Journal Issue: 13 Vol. 36; ISSN 0935-9648
Publisher:
WileyCopyright Statement
Country of Publication:
United States
Language:
English

References (56)

Proximity‐Coupling‐Induced Significant Enhancement of Coercive Field and Curie Temperature in 2D van der Waals Heterostructures journal August 2020
Layered Antiferromagnetism Induces Large Negative Magnetoresistance in the van der Waals Semiconductor CrSBr journal August 2020
Strain‐Sensitive Magnetization Reversal of a van der Waals Magnet journal September 2020
Manipulating Exchange Bias in a Van der Waals Ferromagnet journal February 2022
A Van der Waals Interface Hosting Two Groups of Magnetic Skyrmions journal March 2022
Exchange Bias in Molecule/Fe 3 GeTe 2 van der Waals Heterostructures via Spinterface Effects journal April 2022
Coexistence of Merons with Skyrmions in the Centrosymmetric Van Der Waals Ferromagnet Fe5–xGeTe2 journal March 2023
Tuning the Exchange Bias Effect in 2D van der Waals Ferro‐/Antiferromagnetic Fe 3 GeTe 2 /CrOCl Heterostructures journal March 2022
Spin Waves and Magnetic Exchange Hamiltonian in CrSBr journal July 2022
�ber Chalkogenidhalogenide des Chroms Synthese, Kristallstruktur und Magnetismus von Chromsulfidbromid, CrSBr journal June 1990
Exchange Bias in van der Waals CrCl 3 /Fe 3 GeTe 2 Heterostructures journal May 2020
Magnetic Order and Symmetry in the 2D Semiconductor CrSBr journal April 2021
Gate-Controlled Magnetic Phase Transition in a van der Waals Magnet Fe 5 GeTe 2 journal June 2021
Anisotropic Gigahertz Antiferromagnetic Resonances of the Easy-Axis van der Waals Antiferromagnet CrSBr journal August 2022
Valley Manipulation by Optically Tuning the Magnetic Proximity Effect in WSe 2 /CrI 3 Heterostructures journal May 2018
Stacking-Dependent Magnetism in Bilayer CrI 3 journal November 2018
Highly Efficient Spin–Orbit Torque and Switching of Layered Ferromagnet Fe 3 GeTe 2 journal June 2019
Observation of Magnetic Skyrmion Bubbles in a van der Waals Ferromagnet Fe 3 GeTe 2 journal December 2019
Enhancement of the Coercive Field and Exchange Bias Effect in Fe3GeTe2/MnPX3 (X = S and Se) van der Waals Heterostructures journal May 2021
Role of Oxygen in Ionic Liquid Gating on Two-Dimensional Cr 2 Ge 2 Te 6 : A Non-oxide Material journal December 2017
Layer-Dependent Interlayer Antiferromagnetic Spin Reorientation in Air-Stable Semiconductor CrSBr journal May 2022
Perpendicular switching of a single ferromagnetic layer induced by in-plane current injection journal August 2011
Van der Waals heterostructures journal July 2013
Field-free magnetization reversal by spin-Hall effect and exchange bias journal March 2016
Magnetization switching by spin–orbit torque in an antiferromagnet–ferromagnet bilayer system journal February 2016
Field-free switching of perpendicular magnetization through spin–orbit torque in antiferromagnet/ferromagnet/oxide structures journal July 2016
Spin–orbit torque switching without an external field using interlayer exchange coupling journal May 2016
Tunable metal–insulator transition in double-layer graphene heterostructures journal October 2011
Hard magnetic properties in nanoflake van der Waals Fe3GeTe2 journal April 2018
Switching 2D magnetic states via pressure tuning of layer stacking journal October 2019
Pressure-controlled interlayer magnetism in atomically thin CrI3 journal October 2019
Emergent phenomena and proximity effects in two-dimensional magnets and heterostructures journal September 2020
Coupling between magnetic order and charge transport in a two-dimensional magnetic semiconductor journal May 2022
Asymmetric magnetic proximity interactions in MoSe2/CrBr3 van der Waals heterostructures journal December 2022
Controlling magnetism in 2D CrI3 by electrostatic doping journal May 2018
Layer-resolved magnetic proximity effect in van der Waals heterostructures journal January 2020
Coexisting ferromagnetic–antiferromagnetic state in twisted bilayer CrI3 journal November 2021
Reversible strain-induced magnetic phase transition in a van der Waals magnet journal January 2022
Tunable interaction between excitons and hybridized magnons in a layered semiconductor journal December 2022
Light-induced ferromagnetism in moiré superlattices journal April 2022
Exciton-coupled coherent magnons in a 2D semiconductor journal September 2022
A practical guide for crystal growth of van der Waals layered materials journal August 2020
Exchange bias and spin–orbit torque in the Fe3GeTe2-based heterostructures prepared by vacuum exfoliation approach journal June 2021
Electric field effect in multilayer Cr 2 Ge 2 Te 6 : a ferromagnetic 2D material journal May 2017
Field-free approaches for deterministic spin–orbit torque switching of the perpendicular magnet journal April 2022
New Magnetic Anisotropy journal June 1956
Magnetic Proximity Effect in a van der Waals Moiré Superlattice journal August 2019
Triaxial magnetic anisotropy in the two-dimensional ferromagnetic semiconductor CrSBr journal October 2021
Large magneto-optical effects and magnetic anisotropy energy in two-dimensional Cr 2 Ge 2 Te 6 journal September 2018
Strain-tunable magnetic anisotropy in monolayer CrCl 3 , CrBr 3 , and CrI 3 journal October 2018
Effect of nickel substitution on magnetism in the layered van der Waals ferromagnet Fe 3 GeTe 2 journal October 2018
Current-Induced Switching of Perpendicularly Magnetized Magnetic Layers Using Spin Torque from the Spin Hall Effect journal August 2012
Gate-Tuned Interlayer Coupling in van der Waals Ferromagnet Fe 3 GeTe 2 Nanoflakes journal July 2020
Current-driven magnetization switching in a van der Waals ferromagnet Fe 3 GeTe 2 journal August 2019
Spin-Torque Switching with the Giant Spin Hall Effect of Tantalum journal May 2012
Direct visualization of magnetic domains and moiré magnetism in twisted 2D magnets journal November 2021