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Quantum Gate Operations on a Spectrally Addressable Photogenerated Molecular Electron Spin-Qubit Pair

Journal Article · · Journal of the American Chemical Society
DOI:https://doi.org/10.1021/jacs.3c01243· OSTI ID:2421887
 [1];  [2];  [3];  [3];  [3]
  1. Department of Chemistry, Center for Molecular Quantum Transduction, and Institute for Sustainability and Energy at Northwestern, Northwestern University, Evanston, Illinois 60208-3113, United States; OSTI
  2. Department of Chemistry, Center for Molecular Quantum Transduction, and Institute for Sustainability and Energy at Northwestern, Northwestern University, Evanston, Illinois 60208-3113, United States; Physical and Theoretical Chemistry Laboratory, Department of Chemistry, University of Oxford, Oxford OX1 3QZ, U.K.
  3. Department of Chemistry, Center for Molecular Quantum Transduction, and Institute for Sustainability and Energy at Northwestern, Northwestern University, Evanston, Illinois 60208-3113, United States
Not provided.
Research Organization:
Northwestern Univ., Evanston, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
SC0021314
OSTI ID:
2421887
Journal Information:
Journal of the American Chemical Society, Journal Name: Journal of the American Chemical Society Journal Issue: 11 Vol. 145; ISSN 0002-7863
Publisher:
American Chemical Society (ACS)
Country of Publication:
United States
Language:
English

References (59)

The Usefulness of NMR Quantum Computing journal September 1997
Enhancing coherence in molecular spin qubits via atomic clock transitions journal March 2016
g -Engineering in Hybrid Rotaxanes To Create AB and AB 2 Electron Spin Systems: EPR Spectroscopic Studies of Weak Interactions between Dissimilar Electron Spin Qubits journal July 2015
Electronic spectra and transitions of the fullerene C60 journal March 1992
The nuts and bolts of distance determination and zero- and double-quantum coherence in photoinduced radical pairs journal December 1998
Quantum computational supremacy journal September 2017
Excited-State Properties of C 60 Fullerene Derivatives journal October 2000
Pulse Protocols for Quantum Computing with Electron Spins as Qubits journal November 2011
Molecular spins for quantum information technologies journal January 2011
Picosecond Control of Photogenerated Radical Pair Lifetimes Using a Stable Third Radical journal April 2016
Selectively Addressable Photogenerated Spin Qubit Pairs in DNA Hairpins journal February 2020
A two-qubit molecular architecture for electron-mediated nuclear quantum simulation journal January 2018
Photogenerated Spin-Correlated Radical Pairs: From Photosynthetic Energy Transduction to Quantum Information Science journal September 2021
Electron paramagnetic resonance of spin-correlated radical pairs in photosynthetic reactions journal July 1987
EasySpin, a comprehensive software package for spectral simulation and analysis in EPR journal January 2006
CNOT gate operation on a photogenerated molecular electron spin-qubit pair journal January 2020
Heterodimetallic [LnLn′] Lanthanide Complexes: Toward a Chemical Design of Two-Qubit Molecular Spin Quantum Gates journal August 2014
On the Einstein Podolsky Rosen paradox journal November 1964
Theoretical calculations of microwave effects on the triplet yield in photosynthetic reaction centers journal January 1983
An electron spin echo phase shift observed in photosynthetic algae journal December 1980
Spin-polarized electron paramagnetic resonance spectra of radical pairs in micelles: observation of electron spin-spin interactions journal June 1987
The quantum state tomography on an NMR system journal December 2002
Optically addressable molecular spins for quantum information processing journal November 2020
A Porous Array of Clock Qubits journal May 2017
ESEEM study of spin-spin interactions in spin-polarised P+QA− pairs in the photosynthetic purple bacterium Rhodobacter sphaeroides R26 journal April 1995
Ultrafast Conformational Dynamics of Electron Transfer in ExBox 4+ ⊂Perylene journal November 2013
Molecular spins for quantum computation journal March 2019
Electron Spin Polarization Transfer from Photogenerated Spin-Correlated Radical Pairs to a Stable Radical Observer Spin journal June 2013
Using Photoexcited Core/Shell Quantum Dots To Spin Polarize Appended Radical Qubits journal July 2020
Analysis of density matrix reconstruction in NMR quantum computing journal November 2001
Millisecond Coherence Time in a Tunable Molecular Electronic Spin Qubit journal December 2015
Molecular qubits based on photogenerated spin-correlated radical pairs for quantum sensing journal June 2022
Catalyst: Qubits from the Bottom Up journal April 2020
Tunable Cr4+ Molecular Color Centers journal November 2021
Spin Dynamics of Photogenerated Triradicals in Fixed Distance Electron Donor−Chromophore−Acceptor−TEMPO Molecules journal May 2006
Spin Polarization Transfer from a Photogenerated Radical Ion Pair to a Stable Radical Controlled by Charge Recombination journal June 2017
Electron spin echo envelope modulation due to exchange and dipolar interactions in a spin-correlated radical pair journal March 1994
Exploiting chemistry and molecular systems for quantum information science journal July 2020
Making hybrid [n]-rotaxanes as supramolecular arrays of molecular electron spin qubits journal January 2016
Quantum machine learning journal September 2017
Controlling the Dynamics of Three Electron Spin Qubits in a Donor–Acceptor–Radical Molecule Using Dielectric Environment Changes journal February 2021
Molecular magnetism: from chemical design to spin control in molecules, materials and devices journal October 2019
A concentrated array of copper porphyrin candidate qubits journal January 2019
A Synthetic Two-Spin Quantum Bit: g -Engineered Exchange-Coupled Biradical Designed for Controlled-NOT Gate Operations journal August 2012
A Supramolecular Approach for Modulated Photoprotection, Lysosomal Delivery, and Photodynamic Activity of a Photosensitizer journal June 2019
Transient EPR of weakly coupled spin-correlated radical pairs in photosynthetic reaction centres: increase spectral resolution from nutation analysis journal November 1991
Peculiarities of free induction and primary spin echo signals for spin-correlated radical pairs journal January 1992
Photodriven quantum teleportation of an electron spin state in a covalent donor–acceptor–radical system journal September 2019
Fulleropyrrolidines:  A Family of Full-Fledged Fullerene Derivatives journal September 1998
Quantum units from the topological engineering of molecular graphenoids journal November 2019
The Second Quantum Revolution: Role and Challenges of Molecular Chemistry journal June 2019
Near-Infrared Excitation of the peri-Xanthenoxanthene Radical Cation Drives Energy-Demanding Hole Transfer Reactions journal September 2018
The Direct Dimension in Pulse EPR journal June 2021
Molecular electron-spin quantum computers and quantum information processing: pulse-based electron magnetic resonance spin technology applied to matter spin-qubits journal January 2009
Quantum sensing journal July 2017
Electron spin resonance of spin-correlated radical pairs journal April 1987
Multistep Photochemical Charge Separation in Rod-like Molecules Based on Aromatic Imides and Diimides journal January 1996
The Physical Implementation of Quantum Computation journal September 2000
Principles of Pulse Electron Paramagnetic Resonance book May 2001

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