Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La 1.65 Eu 0.2 Sr 0.15 CuO 4

Bluschke, Martin; Gupta, Naman K.; Jang, Hoyoung; Husain, Ali. A.; Lee, Byungjune; Kim, Minjune; Na, MengXing; Dos Remedios, Brandon; Smit, Steef; Moen, Peter; Park, Sang-Youn; Kim, Minseok; Jang, Dogeun; Choi, Hyeongi; Sutarto, Ronny; Reid, Alexander H.; Dakovski, Georgi L.; Coslovich, Giacomo; Nguyen, Quynh L.; Burdet, Nicolas G.; Lin, Ming-Fu; Revcolevschi, Alexandre; Park, Jae-Hoon; Geck, Jochen; Turner, Joshua J.; Damascelli, Andrea; Hawthorn, David G.

doi:10.1073/pnas.2400727121

Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La _1.65 Eu _0.2 Sr _0.15 CuO ₄

Journal Article · Fri May 31 00:00:00 EDT 2024 · Proceedings of the National Academy of Sciences of the United States of America

DOI:https://doi.org/10.1073/pnas.2400727121· OSTI ID:2369023

^[1]; ^[2]; ^[3]; Husain, Ali. A. ^[1]; ^[4]; ^[1]; Na, MengXing ^[1]; Dos Remedios, Brandon ^[1]; Smit, Steef ^[1]; Moen, Peter ^[1]; ^[5]; Kim, Minseok ^[5]; Jang, Dogeun ^[5]; ^[5]; ^[6]; Reid, Alexander H. ^[7]; Dakovski, Georgi L. ^[7]; Coslovich, Giacomo ^[7]; Nguyen, Quynh L. ^[8]; Burdet, Nicolas G. ^[9] more »

Quantum Matter Institute, University of British Columbia, Vancouver, BC V6T 1Z4, Canada, Department of Physics and Astronomy, University of British Columbia, Vancouver, BC V6T 1Z1, Canada
Department of Physics and Astronomy, University of Waterloo, Waterloo, ON N2L 3G1, Canada
X-ray Free Electron Laser Beamline Division, Pohang Accelerator Laboratory, Pohang University of Science and Technology, Pohang 37673, Gyeongbuk, Republic of Korea, Photon Science Center, Pohang University of Science and Technology, Pohang 37673, Gyeongbuk, Republic of Korea
Max Planck - Pohang University of Science and Technology/Korea Research Initiative, Center for Complex Phase Materials, Pohang 37673, Republic of Korea, Department of Physics, Pohang University of Science and Technology, Pohang 37673, Republic of Korea
X-ray Free Electron Laser Beamline Division, Pohang Accelerator Laboratory, Pohang University of Science and Technology, Pohang 37673, Gyeongbuk, Republic of Korea
Canadian Light Source, Saskatoon, SK S7N 2V3, Canada
Linac Coherent Light Source, Stanford Linear Accelerator Center National Accelerator Laboratory, Menlo Park, CA 94025
Linac Coherent Light Source, Stanford Linear Accelerator Center National Accelerator Laboratory, Menlo Park, CA 94025, Stanford PULSE Institute, Stanford University and Stanford Linear Accelerator Center National Accelerator Laboratory, Menlo Park, CA 94025
Linac Coherent Light Source, Stanford Linear Accelerator Center National Accelerator Laboratory, Menlo Park, CA 94025, Stanford Institute for Materials and Energy Sciences, Stanford Linear Accelerator Center National Accelerator Laboratory and Stanford University, Menlo Park, CA 94025
Institut de Chimie Moléculaire et des Matériaux d’Orsay, Université Paris-Saclay, Centre National de la Recherche Scientifique, UMR 8182, 91405 Orsay, France
Institute of Solid State and Materials Physics, Technische Universität Dresden, 01069 Dresden, Germany, Würzburg-Dresden Cluster of Excellence ct.qmat, Technische Universität Dresden, 01062 Dresden, Germany

Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump–probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu $L_{3}$ and O $K$ resonances, we investigate nonequilibrium dynamics of $Q_{a} = Q_{b} = 0$ nematic order and its association with both charge density wave (CDW) order and lattice dynamics in La $_{1.65}$ Eu $_{0.2}$ Sr $_{0.15}$ CuO $_{4}$ . The orbital selectivity of the resonant X-ray scattering cross-section allows nematicity dynamics associated with the planar O 2 $p$ and Cu 3 $d$ states to be distinguished from the response of anisotropic lattice distortions. A direct time-domain comparison of CDW translational-symmetry breaking and nematic rotational-symmetry breaking reveals that these broken symmetries remain closely linked in the photoexcited state, consistent with the stability of CDW topological defects in the investigated pump fluence regime.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: Gordon and Betty Moore Foundation (GMBF); Ministry of Science and ICT (MSIT); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 2369023

Alternate ID(s):: OSTI ID: 2403412

Journal Information:: Proceedings of the National Academy of Sciences of the United States of America, Journal Name: Proceedings of the National Academy of Sciences of the United States of America Journal Issue: 23 Vol. 121; ISSN 0027-8424

Publisher:: Proceedings of the National Academy of SciencesCopyright Statement

Country of Publication:: United States

Language:: English

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Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La 1.65 Eu 0.2 Sr 0.15 CuO 4

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Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La _1.65 Eu _0.2 Sr _0.15 CuO ₄