Field-induced spin polarization in the lightly Cr-substituted layered antiferromagnet NiP S3

Basnet, Rabindra; Upreti, Dinesh; Patel, Taksh; Karki Chhetri, Santosh; Acharya, Gokul; Nabi, Md Rafique Un; Sharma, M. M.; Sakon, Josh; Mortazavi, Mansour; Hu, Jin

doi:10.1103/physrevb.109.184405

Field-induced spin polarization in the lightly Cr-substituted layered antiferromagnet NiP S₃

Journal Article · Fri May 03 00:00:00 EDT 2024 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.109.184405· OSTI ID:2350579

^[1]; Upreti, Dinesh ^[2]; ^[3]; Karki Chhetri, Santosh ^[2]; Acharya, Gokul ^[2]; ^[2]; Sharma, M. M. ^[2]; Sakon, Josh ^[2]; Mortazavi, Mansour ^[4]; ^[2]

Univ. of Arkansas, Pine Bluff, AR (United States); Univ. of Arkansas, Fayetteville, AR (United States); University of Arkansas
Univ. of Arkansas, Fayetteville, AR (United States)
Fayetteville High School, Fayetteville, AR (United States)
Univ. of Arkansas, Pine Bluff, AR (United States)

Tuning magnetic properties in layered magnets is an important route to realize novel phenomenon related to two-dimensional (2D) magnetism. Recently, tuning antiferromagnetic (AFM) properties through substitution and intercalation techniques has been widely studied in MPX₃ compounds. Interesting phenomena, such as diverse AFM structures and even the signatures of ferrimagnetism, have been reported. However, long-range ferromagnetic (FM) ordering has remained elusive. Here, in this work, we explored the magnetic properties of the Cr-substituted NiP S₃. We found that Cr substitution is extremely efficient in controlling spin orientation in NiP S₃. Our study reveals a field-induced spin polarization in lightly (9%) Cr-substituted NiP S₃, which is likely attributed to the attenuation of AFM interactions and magnetic anisotropy due to Cr doping. Our work provides a possible strategy to achieve FM phase in AFM MPX₃, which could be useful for investigating 2D magnetism as well as potential device applications.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Arkansas, Fayetteville, AR (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0022006; SC0023412

OSTI ID:: 2350579

Alternate ID(s):: OSTI ID: 2356878
OSTI ID: 2368530

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 18 Vol. 109; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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magnetic order
magnetic phase transitions
magnetization measurements