Emergence of ferrimagnetism in Li-intercalated NiPS 3

Basnet, Rabindra; Ford, Dawn; TenBarge, Kaylee; Lochala, Joshua; Hu, Jin

doi:10.1088/1361-648X/ac8a81

Emergence of ferrimagnetism in Li-intercalated NiPS ₃

Journal Article · Fri Sep 02 00:00:00 EDT 2022 · Journal of Physics. Condensed Matter

DOI:https://doi.org/10.1088/1361-648X/ac8a81· OSTI ID:1885202

; Ford, Dawn; TenBarge, Kaylee; Lochala, Joshua;

Abstract

Intercalation has become a powerful approach to tune the intrinsic properties and introduce novel phenomena in layered materials. Intercalating van der Waals (vdW) magnetic materials is a promising route to engineer the low-dimensional magnetism. Recently, metal thiophosphates, M P X ₃ , has been widely studied because their magnetic orders are highly tunable and persist down to the two-dimensional limit. In this work, we used electrochemical technique to intercalate Li into NiPS ₃ single crystals and found the emergence of ferrimagnetism at low temperature in Li-intercalated NiPS ₃ . Such tuning of magnetic properties highlights the effectiveness of intercalation, providing a novel strategy to manipulate the magnetism in vdW magnets.

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Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0022006

OSTI ID:: 1885202

Alternate ID(s):: OSTI ID: 1882032
OSTI ID: 1901944

Journal Information:: Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 43 Vol. 34; ISSN 0953-8984

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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Emergence of ferrimagnetism in Li-intercalated NiPS ₃

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Emergence of ferrimagnetism in Li-intercalated NiPS ₃