Double-domed temperature-pressure phase diagram of CePd3S4

Huyan, S.; Slade, T. J.; Wang, H.; Flint, R.; Ribeiro, R. A.; Xie, W.; Bud'ko, S. L.; Canfield, P. C.

doi:10.1103/physrevb.109.094406

Double-domed temperature-pressure phase diagram of CePd3 S4

Journal Article · Wed Mar 06 00:00:00 EST 2024 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.109.094406· OSTI ID:2323280

^[1]; Slade, T. J. ^[1]; ^[2]; Flint, R. ^[1]; ^[1]; Xie, W. ^[2]; ^[1]; Canfield, P. C. ^[1]

Ames Laboratory (AMES), Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
Michigan State Univ., East Lansing, MI (United States)

CePd₃S₄ exhibits interplay between ferromagnetism (FM), quadrupolar order, and the Kondo effect at low temperatures with a FM transition temperature that is much higher than the value expected from the de Gennes scaling of the heavier RPd₃S₄ compounds. In this work, we investigated the electrical transport and magnetic properties of CePd₃S₄ under pressure up through 12 GPa so as to better understand the interplay between electronic and magnetic phases in this material. Our findings show that the low pressure FM state is suddenly replaced by a new magnetically ordered phase that is most likely antiferromagnetic that spans from ~ 7 GPa to ~ 11 GPa. Whereas this could be described as an example of avoided quantum criticality, given that clear changes in resistance and Hall data are detected near 6.3 GPa for all temperatures below 300 K, it is also possible that the change in ground state is a response to a pressure induced change in structure. Furthermore, the lack of any discernible change in the pressure dependence of the room temperature unit cell parameter/volume across this whole pressure range suggests that this change in structure is either more subtle than could be detected by our measurements (i.e. development of weak, new wave vector) or the transition is electronic (such as a Lifshitz transition).

View Accepted Manuscript (DOE)

Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: AC02-07CH11358; SC0023648

OSTI ID:: 2323280

Alternate ID(s):: OSTI ID: 2473983

Report Number(s):: IS-J--11,283

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 9 Vol. 109; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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