The promise of metal-halide-perovskite solar photovoltaics: A brief review

Padture, Nitin P.

doi:10.1557/s43577-023-00585-6

The promise of metal-halide-perovskite solar photovoltaics: A brief review

Journal Article · Thu Sep 14 00:00:00 EDT 2023 · MRS Bulletin

DOI:https://doi.org/10.1557/s43577-023-00585-6· OSTI ID:2282113

^[1]

Brown University, Providence, RI (United States); Brown University

Solar photovoltaics (PVs) based on metal-halide perovskites (MHPs) have taken the renewable-energy world by storm. The excitement stems from the promise of a high-efficiency, low-cost, and low “carbon-footprint” new PV technology. Here, a brief overview of the important topics pertaining to MHPs, perovskite solar cells (PSCs) and perovskite solar modules (PSMs) is presented. The topics include: (1) PSC architectures, (2) MHPs, (3) synthesis and processing of MHP thin films, (4) MHP thin-film microstructures, (5) PSC functional layers, (6) interfacial engineering in PSCs, (7) PSC performance, (8) PSC stability, (9) PSMs, (10) lead toxicity, and (11) mechanical behavior and reliability. The significant challenges in the path toward commercialization of this burgeoning PV technology are also highlighted. Chief among them are scalability, stability, reliability, and safety, while achieving high efficiency, low cost, and low “carbon-footprint.” Furthermore, the promise of this new PV technology and the fascinating underlying science make it a worthwhile endeavor to address these challenges.

View Accepted Manuscript (DOE)

Research Organization:: Brown University, Providence, RI (United States)

Sponsoring Organization:: National Science Foundation (NSF); Office of Naval Research; USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: EE0009511

OSTI ID:: 2282113

Journal Information:: MRS Bulletin, Journal Name: MRS Bulletin Journal Issue: 10 Vol. 48; ISSN 0883-7694

Publisher:: Materials Research SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites Lee, M. M.; Teuscher, J.; Miyasaka, T. Science, Vol. 338, Issue 6107, p. 643-647 https://doi.org/10.1126/science.1228604	journal	October 2012
Low trap-state density and long carrier diffusion in organolead trihalide perovskite single crystals Shi, D.; Adinolfi, V.; Comin, R. Science, Vol. 347, Issue 6221 https://doi.org/10.1126/science.aaa2725	journal	January 2015
Electron-hole diffusion lengths > 175 μm in solution-grown CH ₃ NH ₃ PbI ₃ single crystals Dong, Qingfeng; Fang, Yanjun; Shao, Yuchuan Science, Vol. 347, Issue 6225 https://doi.org/10.1126/science.aaa5760	journal	January 2015
Photon recycling in lead iodide perovskite solar cells Pazos-Outon, L. M.; Szumilo, M.; Lamboll, R. Science, Vol. 351, Issue 6280 https://doi.org/10.1126/science.aaf1168	journal	March 2016
Quantum dot-induced phase stabilization of -CsPbI3 perovskite for high-efficiency photovoltaics Swarnkar, A.; Marshall, A. R.; Sanehira, E. M. Science, Vol. 354, Issue 6308 https://doi.org/10.1126/science.aag2700	journal	October 2016
Challenges for commercializing perovskite solar cells Rong, Yaoguang; Hu, Yue; Mei, Anyi Science, Vol. 361, Issue 6408 https://doi.org/10.1126/science.aat8235	journal	September 2018
Atomic-scale microstructure of metal halide perovskite Rothmann, Mathias Uller; Kim, Judy S.; Borchert, Juliane Science, Vol. 370, Issue 6516 https://doi.org/10.1126/science.abb5940	journal	October 2020
Interfacial toughening with self-assembled monolayers enhances perovskite solar cell reliability Dai, Zhenghong; Yadavalli, Srinivas K.; Chen, Min Science, Vol. 372, Issue 6542 https://doi.org/10.1126/science.abf5602	journal	May 2021
Conformal quantum dot–SnO ₂ layers as electron transporters for efficient perovskite solar cells Kim, Minjin; Jeong, Jaeki; Lu, Haizhou Science, Vol. 375, Issue 6578 https://doi.org/10.1126/science.abh1885	journal	January 2022
Deterministic fabrication of 3D/2D perovskite bilayer stacks for durable and efficient solar cells Sidhik, Siraj; Wang, Yafei; De Siena, Michael Science, Vol. 377, Issue 6613 https://doi.org/10.1126/science.abq7652	journal	September 2022
Unveiling facet-dependent degradation and facet engineering for stable perovskite solar cells Ma, Chunqing; Eickemeyer, Felix T.; Lee, Sun-Ho Science, Vol. 379, Issue 6628 https://doi.org/10.1126/science.adf3349	journal	January 2023
Photovoltaics at multi-terawatt scale: Waiting is not an option Haegel, Nancy M.; Verlinden, Pierre; Victoria, Marta Science, Vol. 380, Issue 6640 https://doi.org/10.1126/science.adf6957	journal	April 2023
Photon recycling in perovskite solar cells and its impact on device design Raja, Waseem; De Bastiani, Michele; Allen, Thomas G. Nanophotonics, Vol. 10, Issue 8 https://doi.org/10.1515/nanoph-2021-0067	journal	May 2021

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