Conductive surface states and Kondo exhaustion in insulating YbIr3Si7
- Rice University, Houston, TX (United States)
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Rice University, Houston, TX (United States); University of British Columbia, Vancouver, BC (Canada); Max Planck Institute for Chemical Physics of Solids, Dresden (Germany)
- University of British Columbia, Vancouver, BC (Canada); Max Planck Institute for Chemical Physics of Solids, Dresden (Germany)
- Max Planck Institute for Chemical Physics of Solids, Dresden (Germany)
- University of British Columbia, Vancouver, BC (Canada)
- National Synchrotron Radiation Research Center (NSRRC), Taiwan (China)
- Johns Hopkins University, Baltimore, MD (United States)
- National Institute of Standards and Technology, Gaithersburg, MD (United States)
- Harvey Mudd College, Claremont, CA (United States)
- Canadian Light Source, Inc., Saskatoon (Canada)
- University of St. Andrews (United Kingdom)
The interplay of Kondo screening and magnetic ordering in strongly correlated materials containing local moments is a subtle problem. Usually the number of conduction electrons per unit cell matches or exceeds the number of moments, and a Kondo-screened heavy Fermi liquid develops at low temperatures. Changing the pressure, magnetic field, or chemical doping can displace this heavy Fermi liquid in favor of a magnetically ordered state. Alternatively, Kondo singlet formation can be suppressed when the number of conduction electrons is small compared to the number of magnetic moments, known as the Kondo exhaustion scenario. Furthermore we report the discovery of such an “exhausted” Kondo lattice material, YbIr3Si7, where the bulk electrical conductivity tends to zero in the antiferromagnetic state below the Néel temperature TN = 4.1 K, as all the free carriers are consumed in the formation of Kondo singlets. By contrast, the surface is conducting, as the Yb3+ ions relax into larger nonmagnetic Yb2+ in the presence of reduced chemical pressure, which shifts the chemical potential.
- Research Organization:
- Rice Univ., Houston, TX (United States)
- Sponsoring Organization:
- USDOE; Robert A. Welch Foundation; National Science Foundation (NSF)
- Grant/Contract Number:
- SC0019503; C-2114; DMR-1644779; DMR-1539918
- OSTI ID:
- 2281382
- Journal Information:
- Physical Review. B, Vol. 109, Issue 3; ISSN 2469-9950
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
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