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Title: A comparative study of LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} based gamma-ray spectrometers for planetary remote sensing applications

Abstract

The recent availability of large volume cerium bromide crystals raises the possibility of substantially improving gamma-ray spectrometer limiting flux sensitivities over current systems based on the lanthanum tri-halides, e.g., lanthanum bromide and lanthanum chloride, especially for remote sensing, low-level counting applications or any type of measurement characterized by poor signal to noise ratios. The Russian Space Research Institute has developed and manufactured a highly sensitive gamma-ray spectrometer for remote sensing observations of the planet Mercury from the Mercury Polar Orbiter (MPO), which forms part of ESA’s BepiColombo mission. The Flight Model (FM) gamma-ray spectrometer is based on a 3-in. single crystal of LaBr{sub 3}(Ce{sup 3+}) produced in a separate crystal development programme specifically for this mission. During the spectrometers development, manufacturing, and qualification phases, large crystals of CeBr{sub 3} became available in a subsequent phase of the same crystal development programme. Consequently, the Flight Spare Model (FSM) gamma-ray spectrometer was retrofitted with a 3-in. CeBr{sub 3} crystal and qualified for space. Except for the crystals, the two systems are essentially identical. In this paper, we report on a comparative assessment of the two systems, in terms of their respective spectral properties, as well as their suitability for use in planetarymore » mission with respect to radiation tolerance and their propensity for activation. We also contrast their performance with a Ge detector representative of that flown on MESSENGER and show that: (a) both LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} provide superior detection systems over HPGe in the context of minimally resourced spacecraft and (b) CeBr{sub 3} is a more attractive system than LaBr{sub 3}(Ce{sup 3+}) in terms of sensitivities at lower gamma fluxes. Based on the tests, the FM has now been replaced by the FSM on the BepiColombo spacecraft. Thus, CeBr{sub 3} now forms the central gamma-ray detection element on the MPO spacecraft.« less

Authors:
; ; ; ; ; ; ; ; ; ; ;  [1]; ;  [2];  [3];  [4]; ;  [5]; ; more »;  [6] « less
  1. Space Research Institute of the Russian Academy of Sciences (IKI), 84/32 Profsoyuznaya St., Moscow 117997 (Russian Federation)
  2. European Space Agency, ESTEC, Keplerlaan, 2200 AG Noordwijk (Netherlands)
  3. AP, RST, FAME, Delft University of Technology, Mekelweg 15, 2629 JB Delft (Netherlands)
  4. (Netherlands)
  5. Joint Institute for Nuclear Research, Joliot-Curie 6, Dubna, Moscow Region 141980 (Russian Federation)
  6. Institute of Experimental and Applied Physics, Czech Technical University in Prague, Horska 3a/22, 12800 Prague 2 (Czech Republic)
Publication Date:
OSTI Identifier:
22597684
Resource Type:
Journal Article
Resource Relation:
Journal Name: Review of Scientific Instruments; Journal Volume: 87; Journal Issue: 8; Other Information: (c) 2016 Author(s); Country of input: International Atomic Energy Agency (IAEA)
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; CERIUM BROMIDES; CERIUM IONS; GAMMA DETECTION; GAMMA RADIATION; GAMMA SPECTROMETERS; GE SEMICONDUCTOR DETECTORS; LANTHANUM; LANTHANUM BROMIDES; LANTHANUM CHLORIDES; LOW LEVEL COUNTING; MERCURY; MONOCRYSTALS; REMOTE SENSING; SENSITIVITY; SIGNAL-TO-NOISE RATIO

Citation Formats

Kozyrev, A., E-mail: kozyrev@mx.iki.rssi.ru, Mitrofanov, I., Bakhtin, B., Fedosov, F., Golovin, D., Litvak, M., Malakhov, A., Mokrousov, M., Nuzhdin, I., Sanin, A., Tretyakov, V., Vostrukhin, A., Owens, A., Benkhoff, J., Quarati, F., Gonitec BV, J. Bildersstraat 60, 2596 EJ Den Haag, Timoshenko, G., Shvetsov, V., Granja, C., Slavicek, T., and Pospisil, S.. A comparative study of LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} based gamma-ray spectrometers for planetary remote sensing applications. United States: N. p., 2016. Web. doi:10.1063/1.4958897.
Kozyrev, A., E-mail: kozyrev@mx.iki.rssi.ru, Mitrofanov, I., Bakhtin, B., Fedosov, F., Golovin, D., Litvak, M., Malakhov, A., Mokrousov, M., Nuzhdin, I., Sanin, A., Tretyakov, V., Vostrukhin, A., Owens, A., Benkhoff, J., Quarati, F., Gonitec BV, J. Bildersstraat 60, 2596 EJ Den Haag, Timoshenko, G., Shvetsov, V., Granja, C., Slavicek, T., & Pospisil, S.. A comparative study of LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} based gamma-ray spectrometers for planetary remote sensing applications. United States. doi:10.1063/1.4958897.
Kozyrev, A., E-mail: kozyrev@mx.iki.rssi.ru, Mitrofanov, I., Bakhtin, B., Fedosov, F., Golovin, D., Litvak, M., Malakhov, A., Mokrousov, M., Nuzhdin, I., Sanin, A., Tretyakov, V., Vostrukhin, A., Owens, A., Benkhoff, J., Quarati, F., Gonitec BV, J. Bildersstraat 60, 2596 EJ Den Haag, Timoshenko, G., Shvetsov, V., Granja, C., Slavicek, T., and Pospisil, S.. Mon . "A comparative study of LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} based gamma-ray spectrometers for planetary remote sensing applications". United States. doi:10.1063/1.4958897.
@article{osti_22597684,
title = {A comparative study of LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} based gamma-ray spectrometers for planetary remote sensing applications},
author = {Kozyrev, A., E-mail: kozyrev@mx.iki.rssi.ru and Mitrofanov, I. and Bakhtin, B. and Fedosov, F. and Golovin, D. and Litvak, M. and Malakhov, A. and Mokrousov, M. and Nuzhdin, I. and Sanin, A. and Tretyakov, V. and Vostrukhin, A. and Owens, A. and Benkhoff, J. and Quarati, F. and Gonitec BV, J. Bildersstraat 60, 2596 EJ Den Haag and Timoshenko, G. and Shvetsov, V. and Granja, C. and Slavicek, T. and Pospisil, S.},
abstractNote = {The recent availability of large volume cerium bromide crystals raises the possibility of substantially improving gamma-ray spectrometer limiting flux sensitivities over current systems based on the lanthanum tri-halides, e.g., lanthanum bromide and lanthanum chloride, especially for remote sensing, low-level counting applications or any type of measurement characterized by poor signal to noise ratios. The Russian Space Research Institute has developed and manufactured a highly sensitive gamma-ray spectrometer for remote sensing observations of the planet Mercury from the Mercury Polar Orbiter (MPO), which forms part of ESA’s BepiColombo mission. The Flight Model (FM) gamma-ray spectrometer is based on a 3-in. single crystal of LaBr{sub 3}(Ce{sup 3+}) produced in a separate crystal development programme specifically for this mission. During the spectrometers development, manufacturing, and qualification phases, large crystals of CeBr{sub 3} became available in a subsequent phase of the same crystal development programme. Consequently, the Flight Spare Model (FSM) gamma-ray spectrometer was retrofitted with a 3-in. CeBr{sub 3} crystal and qualified for space. Except for the crystals, the two systems are essentially identical. In this paper, we report on a comparative assessment of the two systems, in terms of their respective spectral properties, as well as their suitability for use in planetary mission with respect to radiation tolerance and their propensity for activation. We also contrast their performance with a Ge detector representative of that flown on MESSENGER and show that: (a) both LaBr{sub 3}(Ce{sup 3+}) and CeBr{sub 3} provide superior detection systems over HPGe in the context of minimally resourced spacecraft and (b) CeBr{sub 3} is a more attractive system than LaBr{sub 3}(Ce{sup 3+}) in terms of sensitivities at lower gamma fluxes. Based on the tests, the FM has now been replaced by the FSM on the BepiColombo spacecraft. Thus, CeBr{sub 3} now forms the central gamma-ray detection element on the MPO spacecraft.},
doi = {10.1063/1.4958897},
journal = {Review of Scientific Instruments},
number = 8,
volume = 87,
place = {United States},
year = {Mon Aug 15 00:00:00 EDT 2016},
month = {Mon Aug 15 00:00:00 EDT 2016}
}