Cross sections and calculated yields of some radionuclides of yttrium, strontium and rubidium formed in proton-induced reactions on enriched strontium-86: possibility of production of 85gSr, 83Rb and 82mRb in no-carrier-added form

Uddin, M. Shuza; Basunia, M. Shamsuzzoha; Spahn, Ingo; Spellerberg, Stefan; Khan, Rahat; Uddin, M. Mezbah; Bernstein, Lee A.; Neumaier, Bernd; Qaim, Syed M.

doi:10.1515/ract-2022-0086

Cross sections and calculated yields of some radionuclides of yttrium, strontium and rubidium formed in proton-induced reactions on enriched strontium-86: possibility of production of ^85gSr, ⁸³Rb and ^82mRb in no-carrier-added form

Journal Article · Tue Nov 29 00:00:00 EST 2022 · Radiochimica Acta

DOI:https://doi.org/10.1515/ract-2022-0086· OSTI ID:2248022

Uddin, M. Shuza ^[1]; Basunia, M. Shamsuzzoha ^[2]; Spahn, Ingo ^[3]; Spellerberg, Stefan ^[3]; Khan, Rahat ^[4]; Uddin, M. Mezbah ^[4]; Bernstein, Lee A. ^[5]; Neumaier, Bernd ^[3]; Qaim, Syed M. ^[3]

Forschungszentrum Juelich (Germany); Atomic Energy Research Establishment (AERE), Savar (Bangladesh)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Forschungszentrum Juelich (Germany)
Atomic Energy Research Establishment (AERE), Savar (Bangladesh)
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)

Here, cross sections of the ⁸⁶Sr(p,3n)^84mY, ⁸⁶Sr(p,αn)^82mRb, and ⁸⁶Sr(p,x)^85gSr reactions were measured from their respective thresholds up to 16.2 MeV and from 23.0 to 44.1 MeV at FZJ, and from 14.3 to 24.5 MeV at LBNL, using 96.4% enriched ⁸⁶SrCO₃ as target material. Thin targets prepared by sedimentation were irradiated with protons in a stacked-form, and the induced radioactivity was measured by high-resolution γ-ray spectrometry. Nuclear model calculations based on the code TALYS reproduced our experimental cross section data well. From the excitation functions, the integral yields of the above three radionuclides were calculated. The yield of ^85gSr via the natSr(n,γ) process was also measured using the TRIGA Mark-II reactor at AERE, Savar. A comparison of the reactor and cyclotron production of carrier-added ^85gSr is given. The production possibilities of the three investigated radionuclides in no-carrier-added forms at a 30 MeV cyclotron via new routes are discussed.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Nuclear Physics (NP); USDOE Office of Science (SC), Office of Isotope R&D and Production (IRP)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 2248022

Journal Information:: Radiochimica Acta, Journal Name: Radiochimica Acta Journal Issue: 2 Vol. 111; ISSN 0033-8230

Publisher:: de GruyterCopyright Statement

Country of Publication:: United States

Language:: English

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Cross sections and calculated yields of some radionuclides of yttrium, strontium and rubidium formed in proton-induced reactions on enriched strontium-86: possibility of production of 85gSr, 83Rb and 82mRb in no-carrier-added form

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Cross sections and calculated yields of some radionuclides of yttrium, strontium and rubidium formed in proton-induced reactions on enriched strontium-86: possibility of production of ^85gSr, ⁸³Rb and ^82mRb in no-carrier-added form