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Tunneling magnetoresistance in Co-ZrO{sub 2} granular thin films

Journal Article · · Physical Review. B, Condensed Matter and Materials Physics
DOI:https://doi.org/10.1103/PHYSREVB.73.0· OSTI ID:20787856
; ; ; ; ;  [1]
  1. Departament de Fisica Fonamental, Universitat de Barcelona, Avinguda Diagonal 647, 08028 Barcelona (Spain)
Granular films composed of well defined nanometric Co particles embedded in an insulating ZrO{sub 2} matrix were prepared by pulsed laser deposition in a wide range of Co volume concentrations (0.15<x<0.43). High-resolution transmission electron microscopy (TEM) showed very sharp interfaces between the crystalline particles and the amorphous matrix. Narrow particle size distributions were determined from TEM and by fitting the low-field magnetic susceptibility and isothermal magnetization in the paramagnetic regime to a distribution of Langevin functions. The magnetic particle size varies little for Co volume concentrations x<0.32 and increases as the percolation limit is approached. The tunneling magnetoresistance (TMR) was successfully reproduced using the Inoue-Maekawa model. The maximum value of TMR was temperature-independent within 50-300 K, and largely increased at low T, suggesting the occurrence of higher-order tunneling processes. Consequently, the tunneling conductance and TMR in clean granular metals are dominated by the Coulomb gap and the inherent particle size distribution.
OSTI ID:
20787856
Journal Information:
Physical Review. B, Condensed Matter and Materials Physics, Journal Name: Physical Review. B, Condensed Matter and Materials Physics Journal Issue: 4 Vol. 73; ISSN 1098-0121
Country of Publication:
United States
Language:
English