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Characterization of the hyperline of D{sub 1}/D{sub 0} conical intersections between the maleic acid and fumaric acid anion radicals

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.1785144· OSTI ID:20658010
;  [1]
  1. Department of Chemistry, University of Tsukuba, Tsukuba 305-8571 (Japan)
The cation and anion radicals of symmetrical 1,2-disubstituted ethylenes are expected to have a symmetry-allowed conical intersection (CI) between the ground doublet state (D{sub 0}) and the lowest excited doublet state (D{sub 1}) near a 90 deg.-twisted geometry. By the complete active space self-consistent field method, we characterized the hyperline formed by D{sub 1}/D{sub 0} CIs between the anion radicals of maleic acid (cis) and fumaric acid (trans). An implication of the results for the known one-way cis{yields}trans photoisomerization of the maleic acid anion radical and other related ion radicals is presented.
OSTI ID:
20658010
Journal Information:
Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 14 Vol. 121; ISSN JCPSA6; ISSN 0021-9606
Country of Publication:
United States
Language:
English

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