Quantum Enhanced Probes of Magnetic Circular Dichroism

Hua, Chengyun; Marvinney, Claire E.; Hong, Seongjin; Feldman, Matthew; Pai, Yun‐Yi; Chilcote, Michael; Rabinowitz, Joshua; Pooser, Raphael C.; Marino, Alberto M.; Lawrie, Benjamin J.

doi:10.1002/qute.202300126

Quantum Enhanced Probes of Magnetic Circular Dichroism

Journal Article · Tue Sep 19 00:00:00 EDT 2023 · Advanced Quantum Technologies

DOI:https://doi.org/10.1002/qute.202300126· OSTI ID:2006932

^[1]; Marvinney, Claire E. ^[1]; Hong, Seongjin ^[1]; ^[1]; ^[1]; Chilcote, Michael ^[1]; Rabinowitz, Joshua ^[2]; Pooser, Raphael C. ^[1]; Marino, Alberto M. ^[1]; ^[1]

Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Duke University, Durham, NC (United States)

Magneto-optical microscopies, including optical measurements of magnetic circular dichroism, are increasingly ubiquitous tools for probing spin-orbit coupling, charge-carrier g-factors, and chiral excitations in matter, but the minimum detectable signal in classical magnetic circular dichroism measurements is fundamentally limited by the shot-noise limit of the optical readout field. Here, a two-mode squeezed light source is used to improve the minimum detectable signal in magnetic circular dichroism measurements by 3 decibels compared with state-of-the-art classical measurements, even with relatively lossy samples like terbium gallium garnet. Furthermore, these results provide a framework for new quantum-enhanced magneto-optical microscopies that are particularly critical for environmentally sensitive materials and for low temperature measurements where increased optical power can introduce unacceptable thermal perturbations.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2006932

Journal Information:: Advanced Quantum Technologies, Journal Name: Advanced Quantum Technologies Journal Issue: 4 Vol. 8; ISSN 2511-9044

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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