skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Influence of strain and dislocations on GaSb/GaAs quantum dots: From nested to staggered band alignment

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/5.0070657· OSTI ID:1978975

We investigate the influence of strain and dislocations on band alignment in GaSb/GaAs quantum dot systems. Composition profiles from cross-sectional scanning tunneling microscopy images are interpolated onto a finite element mesh in order to calculate the distribution of local elastic strain, which is converted to a spatially varying band alignment using deformation potential theory. Our calculations predict that dislocation-induced strain relaxation and charging lead to significant local variations in band alignment. Furthermore, misfit strain induces a transition from a nested (type I) to a staggered (type II) band alignment. Although dislocation-induced strain relaxation prevents the type I to type II transition, electrostatic charging at dislocations induces the staggered band alignment once again.

Research Organization:
Univ. of Michigan, Ann Arbor, MI (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
Grant/Contract Number:
FG02-06ER46339; DGE-1256260; ECCS-1610362; FG02-06EF46339
OSTI ID:
1978975
Alternate ID(s):
OSTI ID: 1846471
Journal Information:
Journal of Applied Physics, Vol. 131, Issue 8; ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (37)

GaSb∕GaAs type II quantum dot solar cells for enhanced infrared spectral response journal April 2007
III/V ratio based selectivity between strained Stranski-Krastanov and strain-free GaSb quantum dots on GaAs journal October 2006
Suppression of dislocations by Sb spray in the vicinity of InAs/GaAs quantum dots journal May 2014
Type II–type I conversion of GaAs/GaAsSb heterostructure energy spectrum under optical pumping journal April 2013
Quantum ring formation and antimony segregation in GaSb∕GaAs nanostructures
  • Timm, R.; Lenz, A.; Eisele, H.
  • Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures, Vol. 26, Issue 4 https://doi.org/10.1116/1.2952451
journal January 2008
Atomic-column scanning transmission electron microscopy analysis of misfit dislocations in GaSb/GaAs quantum dots journal May 2016
Differences between photoluminescence spectra of type-I and type-II quantum dots journal March 2008
GaSb/GaAs quantum dot formation and demolition studied with cross-sectional scanning tunneling microscopy journal April 2012
Mechanics of coherent and dislocated island morphologies in strained epitaxial material systems journal May 1997
Optical studies of type-I GaAs1−xSbx/GaAs multiple quantum well structures journal June 2009
Confined States of Individual Type-II GaSb/GaAs Quantum Rings Studied by Cross-Sectional Scanning Tunneling Spectroscopy journal September 2010
Radiative states in type-II GaSb/GaAs quantum wells journal November 1995
Two-dimensional imaging of III-V quantum dots confinement potential journal December 2009
Contrast mechanisms in cross-sectional scanning tunneling microscopy of GaSb/GaAs type-II nanostructures journal May 2009
Nanometer-scale studies of vertical organization and evolution of stacked self-assembled InAs/GaAs quantum dots journal May 1999
Predicted band-gap pressure coefficients of all diamond and zinc-blende semiconductors: Chemical trends journal August 1999
Origin of the blueshift of photoluminescence in a type-II heterostructure journal November 2012
Tunneling spectroscopy of the (110) surface of direct-gap III-V semiconductors journal August 1994
Optical properties of strained antimonide-based heterostructures journal August 2003
Interfacial misfit array formation for GaSb growth on GaAs journal May 2009
Local conduction band offset of GaSb self-assembled quantum dots on GaAs journal March 1997
Band edge alignment of pseudomorphic GaAs 1 y Sb y on GaAs journal November 2004
Height stabilization of GaSb/GaAs quantum dots by Al-rich capping journal September 2014
Band parameters for III–V compound semiconductors and their alloys journal June 2001
Type II GaSb/GaAs quantum dot/ring stacks with extended photoresponse for efficient solar cells journal May 2012
Stress relaxation scenario for buried quantum dots journal June 2009
Band lineups and deformation potentials in the model-solid theory journal January 1989
Effect of strain on band alignment of GaAsSb/GaAs quantum wells journal July 2017
Influence of quantum dot morphology on the optical properties of GaSb/GaAs multilayers journal June 2020
Multi-stacked GaSb/GaAs type-II quantum nanostructures for application to intermediate band solar cells journal June 2017
Radiative recombination in type‐II GaSb/GaAs quantum dots journal July 1995
Influence of GaAs surface termination on GaSb/GaAs quantum dot structure and band offsets journal August 2013
Influence of as on the Morphologies and Optical Characteristics of GaSb/GaAs Quantum Dots journal March 2011
Finite element analysis of strain effects on electronic and transport properties in quantum dots and wires journal October 1998
450 meV hole localization in GaSb/GaAs quantum dots journal April 2003
Formation and optical characteristics of strain-relieved and densely stacked GaSb∕GaAs quantum dots journal November 2006
The structural, electronic and optical properties of GaSb/GaAs nanostructures for charge-based memory journal June 2013