Hydronium Ions on the Surface of a Partially Hydrolyzed α-Zirconium Phosphate: Solid-State 2 H and 31 P MAS NMR Evidence

Bakhmutov, Vladimir I.; Drake, Hannah F.; Zhou, Hong-Cai

doi:10.1021/acs.inorgchem.2c00838

Hydronium Ions on the Surface of a Partially Hydrolyzed α-Zirconium Phosphate: Solid-State ² H and ³¹ P MAS NMR Evidence

Journal Article · 29 April 2022 · Inorganic Chemistry

DOI:https://doi.org/10.1021/acs.inorgchem.2c00838· OSTI ID:1977887

^[1]; Drake, Hannah F. ^[2]; ^[3]

NMR Laboratory, Department of Chemistry, Texas A&M University, College Station, Texas 77843, United States
Department of Chemistry, Texas A&M University, College Station, Texas 77843, United States
Department of Materials Science and Engineering, Texas A&M University, College Station, Texas 77843-3003, United States

Not provided.

Research Organization:: Texas A & M Univ., College Station, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: SC0017864

OSTI ID:: 1977887

Journal Information:: Inorganic Chemistry, Vol. 61, Issue 18; ISSN 0020-1669

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (35)

Preparation of Layered α-Zirconium Phosphate with a Controlled Degree of Hydrolysis via Delamination Procedure Alberti, G.; Marmottini, F. Journal of Colloid and Interface Science, Vol. 157, Issue 2 https://doi.org/10.1006/jcis.1993.1217	journal	May 1993
Zirconium Phosphate: The Pathway from Turbostratic Disorder to Crystallinity Contreras-Ramirez, Aida; Tao, Songsheng; Day, Gregory S. Inorganic Chemistry, Vol. 58, Issue 20 https://doi.org/10.1021/acs.inorgchem.9b02442	journal	October 2019
Elucidating structure and dynamics of crystalline α‐zirconium phosphates intercalated with water and methanol by multinuclear solid‐state MAS NMR: A comprehensive NMR approach Bakhmutov, Vladimir I.; Contreras‐Ramirez, Aida; Drake, Hannah Magnetic Resonance in Chemistry, Vol. 60, Issue 6 https://doi.org/10.1002/mrc.5262	journal	March 2022
Structure and surface chemistry of crystalline zirconium phosphate catalysts Segawa, K.; Nakata, S.; Asaoka, S. Materials Chemistry and Physics, Vol. 17, Issue 1-2 https://doi.org/10.1016/0254-0584(87)90055-1	journal	April 1987
Characterization of crystalline zirconium phosphates and their isomerization activities Segawa, K. Journal of Catalysis, Vol. 94, Issue 2 https://doi.org/10.1016/0021-9517(85)90213-1	journal	August 1985
Zirconium and titanium phosphates as catalysts: a review Clearfield, Abraham; Thakur, Deepak S. Applied Catalysis, Vol. 26 https://doi.org/10.1016/S0166-9834(00)82538-5	journal	January 1986
Recent advances in solid-state NMR spectroscopy of quadrupolar nuclei Ashbrook, Sharon E. Physical Chemistry Chemical Physics, Vol. 11, Issue 32 https://doi.org/10.1039/b907183k	journal	January 2009
Modification and intercalation of layered zirconium phosphates: a solid-state NMR monitoring: Solid-state NMR Bakhmutov, Vladimir I.; Kan, Yuwei; Sheikh, Javeed Ahmad Magnetic Resonance in Chemistry, Vol. 55, Issue 7 https://doi.org/10.1002/mrc.4568	journal	January 2017
High-resolution 2H solid-state NMR of 2H2O adsorbed onto activated carbon Harris, Robin K.; Thompson, Timothy V.; Norman, Paul R. Journal of the Chemical Society, Faraday Transactions, Vol. 91, Issue 12 https://doi.org/10.1039/ft9959101795	journal	January 1995
Deuteron magnetic resonance studies of water associated with phospholipids Salsbury, N. J.; Darke, A.; Chapman, D. Chemistry and Physics of Lipids, Vol. 8, Issue 2 https://doi.org/10.1016/0009-3084(72)90026-6	journal	March 1972
Deuteron Magnetic Resonance Study of Barium Chlorate Monohydrate Chiba, Takehiko The Journal of Chemical Physics, Vol. 39, Issue 4 https://doi.org/10.1063/1.1734396	journal	August 1963
Nuclear Magnetic Resonance of Single Crystals of D ₂ O Ice Waldstein, Peter; Rabideau, Sherman W.; Jackson, Jasper A. The Journal of Chemical Physics, Vol. 41, Issue 11 https://doi.org/10.1063/1.1725740	journal	December 1964
Unexpected structural/motional mode of water intercalated into an α‐crystalline zirconium phosphate deduced by ³¹ P and ² H solid‐state MAS NMR spectra Bakhmutov, Vladimir I.; Contreras‐Ramirez, Aida; Banerjee, Sayan Magnetic Resonance in Chemistry, Vol. 60, Issue 2 https://doi.org/10.1002/mrc.5225	journal	October 2021
Surface hydroxyl concentration on Zr(OH)4 quantified by 1H MAS NMR Mogilevsky, Gregory; Karwacki, Christopher J.; Peterson, Gregory W. Chemical Physics Letters, Vol. 511, Issue 4-6 https://doi.org/10.1016/j.cplett.2011.06.072	journal	August 2011
2H chemical shift anisotropies from high-field 2H MAS NMR spectroscopy Hauch, Anne; Bildsøe, Henrik; Jakobsen, Hans J. Journal of Magnetic Resonance, Vol. 165, Issue 2 https://doi.org/10.1016/j.jmr.2003.09.007	journal	December 2003
Nuclear quadrupole coupling constants and hydrogen bonding. Molecular orbital study of oxygen-17 and deuterium field gradients in formaldehyde-water hydrogen bonding Butler, Leslie G.; Brown, Theodore L. Journal of the American Chemical Society, Vol. 103, Issue 22 https://doi.org/10.1021/ja00412a001	journal	November 1981
Characterization of defects and the local structure in natural and synthetic alunite (K, Na, H3O)Al3(SO4)2(OH)6 by multi-nuclear solid-state NMR spectroscopy Nielsen, U. G.; Majzlan, J.; Phillips, B. American Mineralogist, Vol. 92, Issue 4 https://doi.org/10.2138/am.2007.2414	journal	April 2007
Organically Modified Zirconium Phosphate by Reaction with 1,2-Epoxydodecane as Host Material for Polymer Intercalation: Synthesis and Physicochemical Characterization Casciola, Mario; Capitani, Donatella; Donnadio, Anna Inorganic Chemistry, Vol. 49, Issue 7 https://doi.org/10.1021/ic902330n	journal	April 2010
Proton NMR Chemical Shifts of Hydronium and Hydroxyl Ions Kresge, A. J. The Journal of Chemical Physics, Vol. 39, Issue 5 https://doi.org/10.1063/1.1734449	journal	September 1963
A 2H NMR Study of the Phases and Motions in Solid Oxonium Perchlorate, D3O+ClO4- Ratcliffe, C. I. The Journal of Physical Chemistry, Vol. 98, Issue 42 https://doi.org/10.1021/j100093a041	journal	October 1994
Structure of the Active Sites on H₃PO₄/ZrO₂ Catalysts for Dimethyl Carbonate Synthesis from Methanol and Carbon Dioxide Ikeda, Yoshiki; Asadullah, Mohammad; Fujimoto, Kaoru The Journal of Physical Chemistry B, Vol. 105, Issue 43 https://doi.org/10.1021/jp0121522	journal	October 2001
Intercalation of Organic Molelecules into Layered Phosphates Nakayama, Hirokazu Phosphorus Research Bulletin, Vol. 23 https://doi.org/10.3363/prb.23.1	journal	January 2009
Kinetics of Cross-Polarization in Solid-State NMR: A Guide for Chemists Kolodziejski, Waclaw; Klinowski, Jacek Chemical Reviews, Vol. 102, Issue 3 https://doi.org/10.1021/cr000060n	journal	March 2002
A fourier-transform infrared and catalytic study of the evolution of the surface acidity of zirconium phosphate following heat treatment Busca, Guido; Lorenzelli, Vincenzo; Galli, Paola Journal of the Chemical Society, Faraday Transactions 1: Physical Chemistry in Condensed Phases, Vol. 83, Issue 3 https://doi.org/10.1039/f19878300853	journal	January 1987
Marvelous self-assembly of hierarchically nanostructured porous zirconium phosphate solid acids with high thermal stability Yuan, Zhong-Yong; Ren, Tie-Zhen; Azioune, Ammar Catalysis Today, Vol. 105, Issue 3-4 https://doi.org/10.1016/j.cattod.2005.06.038	journal	August 2005
Zirconium Phosphate with a High Surface Area as a Water-Tolerant Solid Acid Kamiya, Yuichi; Sakata, Shoko; Yoshinaga, Yusuke Catalysis Letters, Vol. 94, Issue 1/2 https://doi.org/10.1023/B:CATL.0000019329.82828.e4	journal	April 2004
Theoretical Studies on Proton Transfer among a High Density of Acid Groups: Surface of Zirconium Phosphate with Adsorbed Water Molecules Ogawa, Takaya; Ushiyama, Hiroshi; Lee, Ju-Myeung The Journal of Physical Chemistry C, Vol. 115, Issue 13 https://doi.org/10.1021/jp107767d	journal	March 2011
Proton Migration on Hydrated Surface of Cubic ZrO ₂ : Ab initio Molecular Dynamics Simulation Sato, Ryuhei; Ohkuma, Shohei; Shibuta, Yasushi The Journal of Physical Chemistry C, Vol. 119, Issue 52 https://doi.org/10.1021/acs.jpcc.5b09026	journal	December 2015
Neutron Scattering Study of the Dynamics of Hydronium Ion in (H₃O)Zr₂(PO₄)₃ Nasicon Across the Order−Disorder Transition Bove, L. E.; Catti, M.; Paciaroni, A. The Journal of Physical Chemistry B, Vol. 108, Issue 26 https://doi.org/10.1021/jp037463m	journal	May 2004
A Solid-State NMR and Theoretical Study of the ¹⁷O Electric Field Gradient and Chemical Shielding Tensors of the Oxonium Ion in p-Toluenesulfonic Acid Monohydrate Wu, Gang; Hook, Andrea; Dong, Shuan The Journal of Physical Chemistry A, Vol. 104, Issue 17 https://doi.org/10.1021/jp994422a	journal	April 2000
Genesis and Stability of Hydronium Ions in Zeolite Channels Wang, Meng; Jaegers, Nicholas R.; Lee, Mal-Soon Journal of the American Chemical Society, Vol. 141, Issue 8 https://doi.org/10.1021/jacs.8b07969	journal	January 2019
Peculiarities of Quadrupolar Relaxation in Electrolyte Solutions Pavlova, Maria; Chizhik, Vladimir Hyperfine Interactions, Vol. 158, Issue 1-4 https://doi.org/10.1007/s10751-005-9016-4	journal	November 2004
A first-principles determination of the orientation of H3O+ in hydronium alunite Gale, J. D.; Wright, K.; Hudson-Edwards, K. A. American Mineralogist, Vol. 95, Issue 7 https://doi.org/10.2138/am.2010.3537	journal	June 2010
Unexpected IR Characteristics of Hydrogen Bonds in the 18-Crown-6-Ether Complex of the H₃O⁺ Hydronium Ion. Can the Location of the Protons Be Specified? Stoyanov, Evgenii S.; Reed, Christopher A. The Journal of Physical Chemistry A, Vol. 108, Issue 5 https://doi.org/10.1021/jp0368177	journal	January 2004
Synthesis and Characterization of a H+ Exchanged Zirconate Orera, A.; Kuhn, A.; Alvarado, F. García Zeitschrift für anorganische und allgemeine Chemie, Vol. 631, Issue 11 https://doi.org/10.1002/zaac.200570041	journal	August 2005

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