Interrelationships between nematicity, antiferromagnetic spin fluctuations, and superconductivity: Role of hotspots in FeSe1-xSx revealed by high pressure Se77 NMR study

Rana, K.; Ambika, D. V.; Bud'ko, S. L.; Böhmer, A. E.; Canfield, P. C.; Furukawa, Y.

doi:10.1103/physrevb.107.134507

Interrelationships between nematicity, antiferromagnetic spin fluctuations, and superconductivity: Role of hotspots in FeSe 1-x Sx revealed by high pressure Se 77 NMR study

Journal Article · Mon Apr 10 00:00:00 EDT 2023 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.107.134507· OSTI ID:1969555

^[1]; Ambika, D. V. ^[1]; ^[1]; Böhmer, A. E. ^[2]; Canfield, P. C. ^[1]; ^[1]

Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)
Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States); Ruhr Univ., Bochum (Germany)

The sulfur-substituted FeSe, FeSe_1-xS_x, is one of the unique systems that provides an independent tunability of nematicity, antiferromagnetism, and superconductivity under pressure (p). Recently, Rana et al. [K. Rana et al., Phys. Rev. B 101, 180503(R) (2020)] reported, from ⁷⁷Se nuclear magnetic resonance (NMR) measurements on FeSe_0.91S_0.09 under pressure, that there exists a clear role of nematicity in the relationship between antiferromagnetic (AFM) spin fluctuations and the superconducting transition temperature (T_c), where the AFM spin fluctuations are more effective in enhancing T_c in the absence of nematicity than with nematicity. Here, motivated by the work, we carried out ⁷⁷Se NMR measurements on FeSe_1-xS_x with x=0.15 and 0.29 under pressure up to 2.10 GPa to investigate the relationship in a wide range of x in the FeSe_1-xS_x system. Based on the new results together with the previously reported data for x=0 [P. Wiecki et al., Phys. Rev. B 96, 180502(R) (2017)] and 0.09 [K. Rana et al. Phys. Rev. B 101, 180503(R) (2020)], we established a p–x–temperature (T) phase diagram exhibiting the evolution of AFM spin fluctuations. From the systematic analysis of the NMR data, we found that the superconducting (SC) state in a nematic state arises from a non-Fermi-liquid state with strong stripe-type AFM spin fluctuations, while the SC state without nematicity comes from a Fermi-liquid state with mild stripe-type AFM spin fluctuations. Furthermore, we show that the previously reported impact of nematicity on the relationship between AFM fluctuations and superconductivity holds throughout the wide range of x from x=0 to 0.29 in FeSe_1-xS_x under pressure. We discuss the origin of the role of nematicity in terms of the different numbers of hotspots on Fermi surfaces with and without nematicity.

View Accepted Manuscript (DOE)

Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1969555

Report Number(s):: IS-J-11,043

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 13 Vol. 107; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Interrelationships between nematicity, antiferromagnetic spin fluctuations, and superconductivity: Role of hotspots in FeSe 1-x Sx revealed by high pressure Se 77 NMR study

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