Progress and Prospects of Inorganic Solid-State Electrolyte-Based All-Solid-State Pouch Cells

Wang, Changhong; Kim, Jung Tae; Wang, Chunsheng; Sun, Xueliang

doi:10.1002/adma.202209074

Progress and Prospects of Inorganic Solid-State Electrolyte-Based All-Solid-State Pouch Cells

Journal Article · Fri Nov 18 00:00:00 EST 2022 · Advanced Materials

DOI:https://doi.org/10.1002/adma.202209074· OSTI ID:2418050

^[1]; Kim, Jung Tae ^[2]; ^[3]; ^[2]

Univ. of Western Ontario, London, ON (Canada); Univ. of Maryland, College Park, MD (United States); OSTI
Univ. of Western Ontario, London, ON (Canada)
Univ. of Maryland, College Park, MD (United States)

Here, all-solid-state batteries have piqued global research interest because of their unprecedented safety and high energy density. Significant advances have been made in achieving high room-temperature ionic conductivity and good air stability of solid-state electrolytes (SSEs), mitigating the challenges at the electrode–electrolyte interface, and developing feasible manufacturing processes. Along with the advances in fundamental study, all-solid-state pouch cells using inorganic SSEs have been widely demonstrated, revealing their immense potential for industrialization. This review provides an overview of inorganic all-solid-state pouch cells, focusing on ultrathin SSE membranes, sheet-type thick solid-state electrodes, and bipolar stacking. Moreover, several critical parameters directly influencing the energy density of all-solid-state Li-ion and lithium–sulfur pouch cells are outlined. Finally, perspectives on all-solid-state pouch cells are provided and specific metrics to meet certain energy density targets are specified. This review looks to facilitate the development of inorganic all-solid-state pouch cells with high energy density and excellent safety.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Maryland, College Park, MD (United States)

Sponsoring Organization:: USDOE; USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: EE0008856

OSTI ID:: 2418050

Alternate ID(s):: OSTI ID: 1963334

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 19 Vol. 35; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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