Strongly-overdoped $\mathrm{La}$2-$_{x}$$\mathrm{Sr}$$_{x}$$\mathrm{CuO}$4: Evidence for Josephson-coupled grains of strongly-correlated superconductor

Li, Yangmu; Sapkota, A.; Lozano, P. M.; Du, Zengyi; Li, Hui; Wu, Zebin; Kundu, Asish K.; Koch, R. J.; Wu, Lijun; Winn, B. L.; Chi, Songxue; Matsuda, M.; Frontzek, M.; Božin, E. S.; Zhu, Yimei; Božović, I.; Pasupathy, Abhay N.; Drozdov, Ilya K.; Fujita, Kazuhiro; Gu, G. D.; Zaliznyak, I. A.; Li, Qiang; Tranquada, J. M.

doi:10.1103/physrevb.106.224515

Title: Strongly-overdoped $$\mathrm{La}$$_2-$$_{x}$$$$\mathrm{Sr}$$$$_{x}$$$$\mathrm{CuO}$$₄: Evidence for Josephson-coupled grains of strongly-correlated superconductor

Journal Article · Wed Dec 21 00:00:00 EST 2022 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.106.224515· OSTI ID:1907224

Li, Yangmu ^[1]; Sapkota, A. ^[1];

^[2];

^[1];

^[2]; Wu, Zebin ^[1];

^[1]; Koch, R. J. ^[1]; Wu, Lijun ^[1];

^[3]; Chi, Songxue ^[3];

^[3]; Frontzek, M. ^[3]; Božin, E. S. ^[1]; Zhu, Yimei ^[1]; Božović, I. ^[1]; Pasupathy, Abhay N. ^[4]; Drozdov, Ilya K. ^[1]; Fujita, Kazuhiro ^[1]; Gu, G. D. ^[1] more »

Brookhaven National Laboratory (BNL), Upton, NY (United States)
Brookhaven National Laboratory (BNL), Upton, NY (United States); Stony Brook University, NY (United States)
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Brookhaven National Laboratory (BNL), Upton, NY (United States); Columbia University, New York, NY (United States)

The interpretation of how superconductivity disappears in cuprates at large hole doping has been controversial. To address this issue, here we present an experimental study of single-crystal and thin film samples of La_2-xSr_xCuO₄ (LSCO) with x ≥0.25. In particular, measurements of bulk susceptibility on LSCO crystals with x = 0.25 indicate an onset of diamagnetism at T_c1=38.5 K, with a sharp transition to a phase with full bulk shielding at T_c2=18 K, independent of field direction. Strikingly, the in-plane resistivity only goes to zero at T_c2. Inelastic neutron scattering on 0.25 crystals confirms the presence of low-energy incommensurate magnetic excitations with reduced strength compared to lower doping levels. The ratio of the spin gap to T_c2 is anomalously large. Our results are consistent with a theoretical prediction for strongly overdoped cuprates by Spivak, Oreto, and Kivelson, in which superconductivity initially develops within disconnected self-organized grains characterized by a reduced hole concentration, with bulk superconductivity occurring only after superconductivity is induced by proximity effect in the surrounding medium of higher hole concentration. Beyond the superconducting-to-metal transition, local differential conductance measurements on an LSCO thin film suggest that regions with pairing correlations survive, but are too dilute to support superconducting order. Future experiments will be needed to test the degree to which these results apply to overdoped cuprates in general.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC05-00OR22725; SC0012704; AC02-06CH11357

OSTI ID:: 1907224

Alternate ID(s):: OSTI ID: 1906164

Report Number(s):: BNL-223811-2022-JAAM; TRN: US2311800

Journal Information:: Physical Review. B, Vol. 106, Issue 22; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
percolation
superconductivity
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angle-resolved photoemission spectroscopy
inelastic neutron scattering
magnetization measurements
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Title: Strongly-overdoped $$\mathrm{La}$$2-$$_{x}$$$$\mathrm{Sr}$$$$_{x}$$$$\mathrm{CuO}$$4: Evidence for Josephson-coupled grains of strongly-correlated superconductor

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Title: Strongly-overdoped $$\mathrm{La}$$_2-$$_{x}$$$$\mathrm{Sr}$$$$_{x}$$$$\mathrm{CuO}$$₄: Evidence for Josephson-coupled grains of strongly-correlated superconductor