Charge-Density-Wave Thin-Film Devices Printed with Chemically Exfoliated 1T-TaS2 Ink

Baraghani, Saba; Barani, Zahra; Ghafouri, Yassamin; Mohammadzadeh, Amirmahdi; Salguero, Tina T.; Kargar, Fariborz; Balandin, Alexander A.

doi:10.1021/acsnano.2c00378

Charge-Density-Wave Thin-Film Devices Printed with Chemically Exfoliated 1T-TaS₂ Ink

Journal Article · Thu Mar 24 00:00:00 EDT 2022 · ACS Nano

DOI:https://doi.org/10.1021/acsnano.2c00378· OSTI ID:1903735

^[1]; Barani, Zahra ^[2]; Ghafouri, Yassamin ^[3]; Mohammadzadeh, Amirmahdi ^[2]; ^[3]; ^[2]; ^[2]

Univ. of California, Riverside, CA (United States); University of California Riverside
Univ. of California, Riverside, CA (United States)
Univ. of Georgia, Athens, GA (United States)

In this work, we report on the preparation of inks containing fillers derived from quasi-two-dimensional charge-density-wave materials, their application for inkjet printing, and the evaluation of their electronic properties in printed thin-film form. The inks were prepared by liquid-phase exfoliation of CVT-grown 1T-TaS₂ crystals to produce fillers with nm-scale thickness and μm-scale lateral dimensions. Exfoliated 1T-TaS₂ was dispersed in a mixture of isopropyl alcohol and ethylene glycol to allow fine-tuning of filler particles thermophysical properties for inkjet printing. The temperature-dependent electrical and current fluctuation measurements of printed thin films demonstrated that the charge-density-wave properties of 1T-TaS₂ are preserved after processing. The functionality of the printed thin-film devices can be defined by the nearly commensurate to the commensurate charge-density-wave phase transition of individual exfoliated 1T-TaS₂ filler particles rather than by electron-hopping transport between them. The obtained results are important for the development of printed electronics with diverse functionality achieved by the incorporation of quasi-two-dimensional van der Waals quantum materials.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of California, Riverside, CA (United States)

Sponsoring Organization:: US Department of the Navy, Office of Naval Research (ONR); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0021020

OSTI ID:: 1903735

Journal Information:: ACS Nano, Journal Name: ACS Nano Journal Issue: 4 Vol. 16; ISSN 1936-0851

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Room temperature depinning of the charge-density waves in quasi-two-dimensional 1T-TaS₂ devices

Journal Article · Mon May 31 20:00:00 EDT 2021 · Applied Physics Letters · OSTI ID:1853705

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1T-TaS2
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
charge density waves
low-frequency noise
printed electronics
quantum materials
resistive switching
van der Waals materials

Charge-Density-Wave Thin-Film Devices Printed with Chemically Exfoliated 1T-TaS2 Ink

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Charge-Density-Wave Thin-Film Devices Printed with Chemically Exfoliated 1T-TaS₂ Ink