Evaluated 238U(n,f) Average Prompt Fission Neutron Multiplicities Including the CGMF Model
This report documents an evaluation of the average prompt fission neutron multiplicity, $$\overline{v}_p$$, of 238U from 800 keV to MeV. This evaluation had to be re-done from “scratch” as the input to previous $$\overline{v}_p$$ evaluations, specifically ENDF/B-VIII.0, was not found. That means that all available experimental data were re-analyzed and uncertainties were re-estimated. The new evaluated 238U $$\overline{v}_p$$ based on only experimental data differs distinctly from ENDF/B-VIII.0 $$\overline{v}_p$$ from 2 to 4.5 MeV, and from 6 to 7 MeV, and is otherwise similar. The difference from 2 to 4.5 MeV stems from the fact that ENDF/B-VIII.0 was tweaked in this energy range to data of Frehaut, while two other, equally trustworthy, data sets would indicate an evaluated 238U $$\overline{v}_p$$ that is up to 2% higher. Also, second chance fission in ENDF/B-VIII.0 was smoothed over from 6–7 MeV. Another major difference to ENDF/B-VIII.0 is that one of the evaluations presented here includes model information from the Hauser-Feshbach fission fragment decay code CGMF, while ENDF/B-VIII.0 is based purely on experimental data. CGMF links several fission quantities with each other; $$\overline{v}_p$$ is predicted by assumptions made on, e.g., pre-neutron emission yields as a function of mass, the total kinetic energy, or spin and parity of fission fragments. This allows to validate the new 238U $$\overline{v}_p$$ by using CGMF parameters obtained from fitting to experimental 238U $$\overline{v}_p$$ to predict yields as a function of mass, the average total kinetic energy, or the mean energy of the prompt fission neutron spectrum. These model-predicted values can then be compared to experimental and evaluated data. The model-predicted fission-observable values using evaluated parameters obtained here are reasonably close to experimental data for some observables, but are farther away from experimental data related to TKE observables. In addition to that, the evaluated 238U(n,f) $$\overline{v}_p$$ shows similar deviations from ENDF/B-VIII.0 as for the evaluation with only experimental data. This difference is expected to lead to changes in simulated effective neutron multiplication factor, $$k_{eff}$$ of ICSBEP critical assemblies that are sensitive to 238U in the fast range (BigTen, Flattop, Flattop-Pu). These changes in $$k_{eff}$$ need to be counter-balanced. Chi-Nu PFNS experimental data are expected to be released in the next few months that might lead to the needed changes in the PFNS. Until then, we hold off in benchmarking the new 238U(n,f) $$\overline{v}_p$$ as well as submitting it to ENDF/B-VIII.1. Also, new high-precision 238U $$\overline{v}_p$$ are expected to be measured by the CEA in the next two years that will shed further light on question on 238U $$\overline{v}_p$$ from 2–4.5 and 6–7 MeV.
- Research Organization:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Organization:
- USDOE National Nuclear Security Administration (NNSA), Nuclear Criticality Safety Program (NCSP)
- DOE Contract Number:
- 89233218CNA000001
- OSTI ID:
- 1889944
- Report Number(s):
- LA-UR-22-29906; TRN: US2309013
- Country of Publication:
- United States
- Language:
- English
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