Recent Advances in Nonclassical Crystallization: Fundamentals, Applications, and Challenges

Fu, Haoyang; Gao, Xing; Zhang, Xin; Ling, Lan

doi:10.1021/acs.cgd.1c01084

Recent Advances in Nonclassical Crystallization: Fundamentals, Applications, and Challenges

Journal Article · Thu Nov 25 23:00:00 EST 2021 · Crystal Growth and Design

DOI:https://doi.org/10.1021/acs.cgd.1c01084· OSTI ID:1888007

Fu, Haoyang ^[1]; Gao, Xing ^[1]; ^[2]; ^[1]

Tongji University, Shanghai (China)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

We report crystals are ubiquitous and play an important role in our daily life. Recent studies on properties and formation of crystals have proven the attachment of particle ranging from ion pairs to well-crystallized nanocrystal is one of the most important ways for crystallization. Compared with the monomer-by-monomer (i.e., atoms, ions, or molecules) addition described in longstanding classical theories, so-called nonclassical crystallization pathways are more complex as the non-specific interaction of variation in system free energy and reaction kinetics. In view of the detailed insights into nonclassical crystallization pathways has broadened the scope of research across various disciplines such as geological events, biomineralization mechanisms, environmental remediation, and the development of functional materials, this paper reviews the current state of the art in nonclassical nucleation (the prenucleation clusters pathway, aggregation pathway, etc.) and growth pathways (oriented attachment and random attachment) based on several spotlights. In addition, the observed specific phenomena on crystallization in the last 10 years as well as recent advancements and achievements made on the synthesis of mesocrystals are also elucidated. With implications and perspectives of nonclassical crystallization researches proposed in this paper, this review aims to summarize research advancement regarding crystallizing systems. Emphasis will be placed on novel insights into nonclassical crystallization of materials, which are expected to provide completely new perspectives on the underlying crystallization mechanisms.

View Accepted Manuscript (DOE)

Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; National Science Fund for Excellent Young Scholars; National Natural Science Foundation of China; Fundamental Research Funds for Central Universities

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1888007

Report Number(s):: PNNL-SA-165993

Journal Information:: Crystal Growth and Design, Journal Name: Crystal Growth and Design Journal Issue: 2 Vol. 22; ISSN 1528-7483

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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