Engineering Crystal Modifiers: Bridging Classical and Nonclassical Crystallization

Olafson, Katy N.; Li, Rui; Alamani, Bryan G.; Rimer, Jeffrey D.

doi:10.1021/acs.chemmater.6b03550

Title: Engineering Crystal Modifiers: Bridging Classical and Nonclassical Crystallization

Journal Article · Wed Sep 28 00:00:00 EDT 2016 · Chemistry of Materials

DOI:https://doi.org/10.1021/acs.chemmater.6b03550· OSTI ID:1534443

Olafson, Katy N. ^[1]; Li, Rui ^[1]; Alamani, Bryan G. ^[2]; Rimer, Jeffrey D. ^[1]

Univ. of Houston, TX (United States)
Univ. of Houston, TX (United States); Univ. of the Philippines, Diliman, Quezon City (Philippines)

The use of growth modifiers in natural, biological, and synthetic crystallization is a ubiquitous strategy for controlling growth and achieving desired physicochemical properties. For crystals that grow classically (i.e., monomer-by-monomer addition), theories of crystallization are well established and the field of growth modification is rather mature, although many questions remain regarding the molecular driving forces of modifier–crystal interactions. A new frontier in crystallization is the application of classical methods to tailor materials that grow nonclassically (i.e., growth by the addition of species more complex than monomers). A recent surge of interest and activity in this field has been driven by mounting evidence of both inorganic and organic materials that grow via nonclassical pathways. In these systems, the challenge of elucidating the mechanism(s) of crystallization is underscored by a diversity of growth units that far outnumber those available for classical routes. In this Perspective, we consider growth modification in nonclassical crystallization, including examples in the literature, the challenges associated with elucidating the modes of modifier action, and to what degree classical theories can be applied to these complex problems as a means of establishing versatile blueprints for crystal engineering.

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Research Organization:: Univ. of Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); The Welch Foundation

Grant/Contract Number:: SC0014468; E-1794

OSTI ID:: 1534443

Journal Information:: Chemistry of Materials, Vol. 28, Issue 23; ISSN 0897-4756

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 93 works

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Nanosized MCM-22 zeolite using simple non-surfactant organic growth modifiers: synthesis and catalytic applications Gallego, Eva M.; Paris, Cecilia; Martínez, Cristina Chemical Communications, Vol. 54, Issue 71 https://doi.org/10.1039/c8cc05356a	journal	January 2018
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Assembly of Sub-Crystals on the Macroscale and Construction of Composite Building Units on the Microscale for SAPO-34 Yuan, Delin; Xing, Aihua; Miao, Ping Chemistry - An Asian Journal, Vol. 13, Issue 20 https://doi.org/10.1002/asia.201801069	journal	September 2018
Preparation of ZnO Nanoparticles with High Dispersibility Based on Oriented Attachment (OA) Process Cao, Dingding; Gong, Sheng; Shu, Xugang Nanoscale Research Letters, Vol. 14, Issue 1 https://doi.org/10.1186/s11671-019-3038-3	journal	June 2019
Hydroxycitrate: a potential new therapy for calcium urolithiasis Kim, Doyoung; Rimer, Jeffrey D.; Asplin, John R. Urolithiasis, Vol. 47, Issue 4 https://doi.org/10.1007/s00240-019-01125-1	journal	March 2019
Crystallization of Small Organic Molecules in a Polymer Matrix: Multistep Mechanism Enables Structural Control Bronshtein, Ilya; Weissman, Haim; Kaplan‐Ashiri, Ifat Small, Vol. 15, Issue 38 https://doi.org/10.1002/smll.201902936	journal	August 2019
Zeolite Y microspheres with perpendicular mesochannels and metal@Y heterostructures for catalytic and SERS applications Chen, Zhuwen; Chen, Chao; Zhang, Jian Journal of Materials Chemistry A, Vol. 6, Issue 15 https://doi.org/10.1039/c7ta10444h	journal	January 2018
Organic Mesopore Generating Agents (OMeGAs) for Hierarchical Zeolites: Combining Functions on Multiple Scales Hong, Mei; Dong, Lei; Yang, Shihe ChemNanoMat, Vol. 5, Issue 7 https://doi.org/10.1002/cnma.201900186	journal	May 2019
Cover Feature: Time‐Resolved Dynamics of Struvite Crystallization: Insights from the Macroscopic to Molecular Scale (Chem. Eur. J. 16/2020) Kim, Doyoung; Olympiou, Chara; McCoy, Colin P. Chemistry – A European Journal, Vol. 26, Issue 16 https://doi.org/10.1002/chem.201905476	journal	March 2020

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Related Subjects

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
36 MATERIALS SCIENCE
Chemistry
Materials science
Crystals
Crystallization
Precursors
Monomers
Zeolites