Long-term interactive corrosion between International Simple Glass and stainless steel

Mohanty, Chandi; Guo, Xiaolei; Kaya, Huseyin; Gin, Stephane; Yang, Kun; Zhang, Zelong; Kim, Seong H.; Lian, Jie; Wang, Jianwei; Frankel, Gerald S.

doi:10.1038/s41529-022-00262-0

Long-term interactive corrosion between International Simple Glass and stainless steel

Journal Article · Wed Jun 29 00:00:00 EDT 2022 · npj Materials Degradation

DOI:https://doi.org/10.1038/s41529-022-00262-0· OSTI ID:1881006

^[1]; Guo, Xiaolei ^[2]; Kaya, Huseyin ^[3]; ^[4]; Yang, Kun ^[5]; ^[6]; ^[3]; ^[5]; Wang, Jianwei ^[6]; ^[2]

The Ohio State Univ., Columbus, OH (United States); The Ohio State University
The Ohio State Univ., Columbus, OH (United States)
Pennsylvania State Univ., University Park, PA (United States)
Univ. of Montpellier (France)
Rensselaer Polytechnic Inst., Troy, NY (United States)
Louisiana State Univ., Baton Rouge, LA (United States)

The interactive corrosion between stainless steel 316 (SS) and International Simple Glass (ISG) has been studied for 12 months. The samples were placed in intimate contact to create crevice corrosion conditions on SS in a 0.6 M NaCl solution with and without 142 ppm dissolved silica species enriched in ²⁹Si. Corrosion on SS was observed with large pits located close to the crevice mouth at the end of 1 year in 0.6 M NaCl solution. The SS corrosion was also associated with the dissolution of nearby glass in a highly localized manner. When the leaching solution was saturated with silica species, the corrosion rate of SS was suppressed. However, the presence of SS enhances ISG dissolution in both conditions. The implications of the observed phenomena on the long-term storage of nuclear waste are discussed.

View Accepted Manuscript (DOE)

Research Organization:: The Ohio State Univ., Columbus, OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0016584

OSTI ID:: 1881006

Journal Information:: npj Materials Degradation, Journal Name: npj Materials Degradation Journal Issue: 1 Vol. 6; ISSN 2397-2106

Publisher:: SpringerCopyright Statement

Country of Publication:: United States

Language:: English

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