Yielding in dense suspensions: cage, bond, and rotational confinements
- Univ. of Illinois, Urbana, IL (United States); University of Illinois
- Univ. of Illinois, Urbana, IL (United States)
The effect of weak particle anisotropy on the onset of fluidity in dense suspensions of glasses of repulsive, weakly attractive and strongly attractive spherical and dumbbell shaped particles is explored. Yield stresses are found to scale with volume fraction showing a divergence at random close packing for all systems. However the onsets of yielding in suspensions of spherical and dumbbell shaped particles are shown to display qualitatively different behaviors. Suspensions of hard spheres exhibit a single yield stress (strain) while suspensions of spheres experiencing short range attractions in dense gels display two yielding events. Double yielding occurs when attractions between particles are only a few kT and the suspensions are sufficiently dense. For dumbbell suspensions, single yielding is observed for hard dumbbell glasses in a region where the glasses are expected to be plastic while double yielding is observed when the particles are expected to have localized centers of mass and localized orientations. Double yielding is also observed for dense dumbbell suspensions that experience attractions while only single yielding events are observed in strongly attractive gels for both dumbbells and spheres. Furthermore, these results are discussed in the light of recent theories and simulations of mechanisms of localization in suspensions of spherical and weakly anisotropic particles.
- Research Organization:
- Univ. of Illinois at Urbana-Champaign, IL (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
- Grant/Contract Number:
- FG02-07ER46471; FG02-07ER46453
- OSTI ID:
- 1876415
- Alternate ID(s):
- OSTI ID: 21528054
- Journal Information:
- Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 3 Vol. 23; ISSN 0953-8984
- Publisher:
- IOP PublishingCopyright Statement
- Country of Publication:
- United States
- Language:
- English
Heterogeneous materials: metastable and non-ergodic internal structures
|
journal | March 2019 |
Two-step yielding and directional strain-induced strengthening in dilute colloidal gels
|
journal | April 2012 |
Similar Records
Exploration of the volume fraction above which suspensions of spherical and weakly anisotropic colloid particles cannot flow
Nonlinear rheology and yielding in dense suspensions of hard anisotropic colloids