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Yielding in dense suspensions: cage, bond, and rotational confinements

Journal Article · · Journal of Physics. Condensed Matter
 [1];  [2]
  1. Univ. of Illinois, Urbana, IL (United States); University of Illinois
  2. Univ. of Illinois, Urbana, IL (United States)

The effect of weak particle anisotropy on the onset of fluidity in dense suspensions of glasses of repulsive, weakly attractive and strongly attractive spherical and dumbbell shaped particles is explored. Yield stresses are found to scale with volume fraction showing a divergence at random close packing for all systems. However the onsets of yielding in suspensions of spherical and dumbbell shaped particles are shown to display qualitatively different behaviors. Suspensions of hard spheres exhibit a single yield stress (strain) while suspensions of spheres experiencing short range attractions in dense gels display two yielding events. Double yielding occurs when attractions between particles are only a few kT and the suspensions are sufficiently dense. For dumbbell suspensions, single yielding is observed for hard dumbbell glasses in a region where the glasses are expected to be plastic while double yielding is observed when the particles are expected to have localized centers of mass and localized orientations. Double yielding is also observed for dense dumbbell suspensions that experience attractions while only single yielding events are observed in strongly attractive gels for both dumbbells and spheres. Furthermore, these results are discussed in the light of recent theories and simulations of mechanisms of localization in suspensions of spherical and weakly anisotropic particles.

Research Organization:
Univ. of Illinois at Urbana-Champaign, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
Grant/Contract Number:
FG02-07ER46471; FG02-07ER46453
OSTI ID:
1876415
Alternate ID(s):
OSTI ID: 21528054
Journal Information:
Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 3 Vol. 23; ISSN 0953-8984
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

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Cited By (2)

Heterogeneous materials: metastable and non-ergodic internal structures
  • Alexandrov, Dmitri V.; Zubarev, Andrey Yu.
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2143 https://doi.org/10.1098/rsta.2018.0353
journal March 2019
Two-step yielding and directional strain-induced strengthening in dilute colloidal gels journal April 2012

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