Stretchable batteries with self-similar serpentine interconnects and integrated wireless recharging systems

Xu, Sheng; Zhang, Yihui; Cho, Jiung; Lee, Juhwan; Huang, Xian; Jia, Lin; Fan, Jonathan A.; Su, Yewang; Su, Jessica; Zhang, Huigang; Cheng, Huanyu; Lu, Bingwei; Yu, Cunjiang; Chuang, Chi; Kim, Tae-il; Song, Taeseup; Shigeta, Kazuyo; Kang, Sen; Dagdeviren, Canan; Petrov, Ivan; Braun, Paul V.; Huang, Yonggang; Paik, Ungyu; Rogers, John A.

doi:10.1038/ncomms2553

Title: Stretchable batteries with self-similar serpentine interconnects and integrated wireless recharging systems

Journal Article · Tue Feb 26 00:00:00 EST 2013 · Nature Communications

DOI:https://doi.org/10.1038/ncomms2553· OSTI ID:1876393

Xu, Sheng ^[1]; Zhang, Yihui ^[2]; Cho, Jiung ^[1]; Lee, Juhwan ^[1]; Huang, Xian ^[1]; Jia, Lin ^[1]; Fan, Jonathan A. ^[1]; Su, Yewang ^[2]; Su, Jessica ^[1]; Zhang, Huigang ^[1]; Cheng, Huanyu ^[3]; Lu, Bingwei ^[4]; Yu, Cunjiang ^[1]; Chuang, Chi ^[1]; Kim, Tae-il ^[1]; Song, Taeseup ^[5]; Shigeta, Kazuyo ^[1]; Kang, Sen ^[1]; Dagdeviren, Canan ^[1]; Petrov, Ivan ^[1] more »

Univ. of Illinois at Urbana-Champaign, IL (United States)
Tsinghua Univ., Beijing (China); Northwestern Univ., Evanston, IL (United States)
Northwestern Univ., Evanston, IL (United States)
Univ. of Illinois at Urbana-Champaign, IL (United States); Tsinghua Univ., Beijing (China)
Hanyang Univ., Seoul (Korea, Republic of)

An important trend in electronics involves the development of materials, mechanical designs and manufacturing strategies that enable the use of unconventional substrates, such as polymer films, metal foils, paper sheets or rubber slabs. The last possibility is particularly challenging because the systems must accommodate not only bending but also stretching. Although several approaches are available for the electronics, a persistent difficulty is in power supplies that have similar mechanical properties, to allow their co-integration with the electronics. In this study we introduce a set of materials and design concepts for a rechargeable lithium ion battery technology that exploits thin, low modulus silicone elastomers as substrates, with a segmented design in the active materials, and unusual ‘self-similar’ interconnect structures between them. The result enables reversible levels of stretchability up to 300%, while maintaining capacity densities of ~1.1 mAh cm^⁻2. Stretchable wireless power transmission systems provide the means to charge these types of batteries, without direct physical contact.

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Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; National Science Foundation (NSF); National Research Foundation of Korea (NRF)

Grant/Contract Number:: FG02-07ER46471; FG02-91ER45439; FG02-07ER46453; ECCS-0824129; K2070400000307A050000310

OSTI ID:: 1876393

Journal Information:: Nature Communications, Vol. 4, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Mechanical Analyses and Structural Design Requirements for Flexible Energy Storage Devices Mao, Lijuan; Meng, Qinghai; Ahmad, Aziz Advanced Energy Materials, Vol. 7, Issue 23 https://doi.org/10.1002/aenm.201700535	journal	July 2017
Stretchable electronics: functional materials, fabrication strategies and applications Wu, Wei Science and Technology of Advanced Materials, Vol. 20, Issue 1 https://doi.org/10.1080/14686996.2018.1549460	journal	March 2019
Light Weight and Flexible High-Performance Diagnostic Platform Karnaushenko, Daniil; Ibarlucea, Bergoi; Lee, Sanghun Advanced Healthcare Materials, Vol. 4, Issue 10 https://doi.org/10.1002/adhm.201500128	journal	May 2015
In-Plane Deformation Mechanics for Highly Stretchable Electronics Su, Yewang; Ping, Xuecheng; Yu, Ki Jun Advanced Materials, Vol. 29, Issue 8 https://doi.org/10.1002/adma.201604989	journal	December 2016
High-performance flexible energy storage and harvesting system for wearable electronics Ostfeld, Aminy E.; Gaikwad, Abhinav M.; Khan, Yasser Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep26122	journal	May 2016
3D Porous Sponge-Inspired Electrode for Stretchable Lithium-Ion Batteries Liu, Wei; Chen, Zheng; Zhou, Guangmin Advanced Materials, Vol. 28, Issue 18 https://doi.org/10.1002/adma.201505299	journal	March 2016
Solution Deposition of Conformal Gold Coatings on Knitted Fabric for E‐Textiles and Electroluminescent Clothing Wu, Yunyun; Mechael, Sara S.; Chen, Yiting Advanced Materials Technologies, Vol. 3, Issue 3 https://doi.org/10.1002/admt.201700292	journal	January 2018
Graphene-based integrated electrodes for flexible lithium ion batteries Shi, Ying; Wen, Lei; Zhou, Guangmin 2D Materials, Vol. 2, Issue 2 https://doi.org/10.1088/2053-1583/2/2/024004	journal	April 2015
Highly Stretchable Piezoresistive Graphene-Nanocellulose Nanopaper for Strain Sensors Yan, Chaoyi; Wang, Jiangxin; Kang, Wenbin Advanced Materials, Vol. 26, Issue 13 https://doi.org/10.1002/adma.201304742	journal	December 2013
Kirigami Patterning of MXene/Bacterial Cellulose Composite Paper for All‐Solid‐State Stretchable Micro‐Supercapacitor Arrays Jiao, Shangqing; Zhou, Aiguo; Wu, Mingzai Advanced Science, Vol. 6, Issue 12 https://doi.org/10.1002/advs.201900529	journal	April 2019
Selective Area Epitaxial Growth of Stretchable Geometry AlGaN-GaN Heterostructures Mahaboob, Isra; Marini, Jonathan; Hogan, Kasey Journal of Electronic Materials, Vol. 47, Issue 11 https://doi.org/10.1007/s11664-018-6576-z	journal	August 2018
3D Multifunctional Composites Based on Large-Area Stretchable Circuit with Thermoforming Technology Yang, Yang; Vervust, Thomas; Dunphy, Sheila Advanced Electronic Materials, Vol. 4, Issue 8 https://doi.org/10.1002/aelm.201800071	journal	May 2018
A New Frontier of Printed Electronics: Flexible Hybrid Electronics Khan, Yasser; Thielens, Arno; Muin, Sifat Advanced Materials, Vol. 32, Issue 15 https://doi.org/10.1002/adma.201905279	journal	April 2020
Direct Transfer of Magnetic Sensor Devices to Elastomeric Supports for Stretchable Electronics Melzer, Michael; Karnaushenko, Daniil; Lin, Gungun Advanced Materials, Vol. 27, Issue 8 https://doi.org/10.1002/adma.201403998	journal	January 2015
Recent Progress in Electronic Skin Wang, Xiandi; Dong, Lin; Zhang, Hanlu Advanced Science, Vol. 2, Issue 10 https://doi.org/10.1002/advs.201500169	journal	July 2015
Engineering Smart Hybrid Tissues with Built-In Electronics Feiner, Ron; Dvir, Tal iScience, Vol. 23, Issue 2 https://doi.org/10.1016/j.isci.2020.100833	journal	February 2020
Flexible lithium–oxygen battery based on a recoverable cathode Liu, Qing-Chao; Xu, Ji-Jing; Xu, Dan Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms8892	journal	August 2015
Extremely stretchable and conductive water-repellent coatings for low-cost ultra-flexible electronics Mates, Joseph E.; Bayer, Ilker S.; Palumbo, John M. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9874	journal	November 2015
Extremely stretchable and self-healing conductor based on thermoplastic elastomer for all-three-dimensional printed triboelectric nanogenerator Parida, Kaushik; Thangavel, Gurunathan; Cai, Guofa Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10061-y	journal	May 2019
Decoupling of mechanical properties and ionic conductivity in supramolecular lithium ion conductors Mackanic, David G.; Yan, Xuzhou; Zhang, Qiuhong Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-13362-4	journal	November 2019
Thermally Triggered Mechanically Destructive Electronics Based On Electrospun Poly(ε-caprolactone) Nanofibrous Polymer Films Gao, Yang; Sim, Kyoseung; Yan, Xin Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-01026-6	journal	April 2017
Cross-buckled structures for stretchable and compressible thin film silicon solar cells Nam, Jiyoon; Seo, Bowook; Lee, Youngjoo Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-08012-y	journal	August 2017
Stretchable conductive elastomer for wireless wearable communication applications Chen, Zhibo; Xi, Jingtian; Huang, Wei Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-11392-w	journal	September 2017
Electrochemical Evaluations of Fractal Microelectrodes for Energy Efficient Neurostimulation Park, Hyunsu; Takmakov, Pavel; Lee, Hyowon Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-22545-w	journal	March 2018
High-performance transparent and stretchable all-solid supercapacitors based on highly aligned carbon nanotube sheets Chen, Tao; Peng, Huisheng; Durstock, Michael Scientific Reports, Vol. 4, Issue 1 https://doi.org/10.1038/srep03612	journal	January 2014
Versatile, kinetically controlled, high precision electrohydrodynamic writing of micro/nanofibers Huang, YongAn; Duan, Yongqing; Ding, Yajiang Scientific Reports, Vol. 4, Issue 1 https://doi.org/10.1038/srep05949	journal	August 2014
Columnar grown copper films on polyimides strained beyond 100% Sun, Jeong-Yun; Lee, Hae-Ryung; Hwan Oh, Kyu Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep13791	journal	September 2015
Wearable Fall Detector using Integrated Sensors and Energy Devices Jung, Sungmook; Hong, Seungki; Kim, Jaemin Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep17081	journal	November 2015
Mechanically Stretchable and Electrically Insulating Thermal Elastomer Composite by Liquid Alloy Droplet Embedment Jeong, Seung Hee; Chen, Si; Huo, Jinxing Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep18257	journal	December 2015
Wireless thin film transistor based on micro magnetic induction coupling antenna Jun, Byoung Ok; Lee, Gwang Jun; Kang, Jong Gu Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep18621	journal	December 2015
In Situ Study of Strain-Dependent Ion Conductivity of Stretchable Polyethylene Oxide Electrolyte Kelly, Taylor; Ghadi, Bahar Moradi; Berg, Sean Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep20128	journal	February 2016
Multilayer Patterning of High Resolution Intrinsically Stretchable Electronics Tybrandt, Klas; Stauffer, Flurin; Vörös, Janos Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep25641	journal	May 2016
Fully printable, strain-engineered electronic wrap for customizable soft electronics Byun, Junghwan; Lee, Byeongmoon; Oh, Eunho Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/srep45328	journal	March 2017
Instant tough bonding of hydrogels for soft machines and electronics Wirthl, Daniela; Pichler, Robert; Drack, Michael Science Advances, Vol. 3, Issue 6 https://doi.org/10.1126/sciadv.1700053	journal	June 2017
Fully rubbery integrated electronics from high effective mobility intrinsically stretchable semiconductors Sim, Kyoseung; Rao, Zhoulyu; Kim, Hae-Jin Science Advances, Vol. 5, Issue 2 https://doi.org/10.1126/sciadv.aav5749	journal	February 2019
Stretchable batteries with gradient multilayer conductors Gu, Minsu; Song, Woo-Jin; Hong, Jaehyung Science Advances, Vol. 5, Issue 7 https://doi.org/10.1126/sciadv.aaw1879	journal	July 2019
High-resolution, reconfigurable printing of liquid metals with three-dimensional structures Park, Young-Geun; An, Hyeon Seok; Kim, Ju-Young Science Advances, Vol. 5, Issue 6 https://doi.org/10.1126/sciadv.aaw2844	journal	June 2019
Integrated approach for smart implantable cardioverter defibrillator (ICD) device with real time ECG monitoring: use of flexible sensors for localized arrhythmia sensing and stimulation Puri, Munish; Chapalamadugu, Kalyan C.; Miranda, Aimon C. Frontiers in Physiology, Vol. 4 https://doi.org/10.3389/fphys.2013.00300	journal	January 2013
Stretchable Piezoelectric Power Generators Based on ZnO Thin Films on Elastic Substrates Voiculescu, Ioana; Li, Fang; Kowach, Glen Micromachines, Vol. 10, Issue 10 https://doi.org/10.3390/mi10100661	journal	September 2019
Requirements for Durability Improvement of Conductive Patterns Permeated in Textiles under Cyclic Tensile Deformation Micromachines, Vol. 10, Issue 11 https://doi.org/10.3390/mi10110721	journal	October 2019
Materials, Mechanics, and Patterning Techniques for Elastomer-Based Stretchable Conductors Yu, Xiaowei; Mahajan, Bikram; Shou, Wan Micromachines, Vol. 8, Issue 1 https://doi.org/10.3390/mi8010007	journal	December 2016
Stretchable Tattoo-Like Heater with On-Site Temperature Feedback Control Stier, Andrew; Halekote, Eshan; Mark, Andrew Micromachines, Vol. 9, Issue 4 https://doi.org/10.3390/mi9040170	journal	April 2018
Real Time Analysis of Bioanalytes in Healthcare, Food, Zoology and Botany Wang, Tianqi; Ramnarayanan, Ashwin; Cheng, Huanyu Sensors, Vol. 18, Issue 2 https://doi.org/10.3390/s18010005	journal	December 2017
Soft and Deformable Sensors Based on Liquid Metals Kim, Taeyeong; Kim, Dong-min; Lee, Bong Jae Sensors, Vol. 19, Issue 19 https://doi.org/10.3390/s19194250	journal	September 2019

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