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Methane detection of chirped laser dispersion spectroscopy using DSB-SC modulation

Conference · · Terahertz, RF, Millimeter, and Submillimeter-Wave Technology and Applications XII
DOI:https://doi.org/10.1117/12.2506917· OSTI ID:1870136

This paper discusses the use of double-sideband suppressed-carrier (DSB-SC) modulation and radio frequency mixer as phase detector to extract phase information for methane detection in chirped laser dispersion spectroscopy (CLaDS). The 1.66 μm light from narrow-linewidth laser was modulated by electro-optic modulator (EOM) working on DSB-SC mode. These two sidebands passed through gas chamber and formed interference on photodetector. The phase change from gas absorption in beating signal can be extracted by using passive RF mixer with another input as reference signal which is achieved by doubling RF drive signal of EOM. In RF mixer, two inputs with identical frequency but various phase shift corresponds to DC bias voltage variation of output. The phase change is proportional to refractive index change and can be referred to gas concentration by using Kramers-Kronig relations. The advantage of phase sensitive CLaDS is wide dynamic range for gas detection. It compensates the deficiency of wavelength modulation spectroscopy (WMS) on high concentration circumstances. And the passive scheme pushes the system requirement to the lowest level.

Research Organization:
University of Pittsburgh
Sponsoring Organization:
USDOE Office of Fossil Energy (FE)
DOE Contract Number:
FE0029063
OSTI ID:
1870136
Report Number(s):
DE-PITT-FE0029063-8
Journal Information:
Terahertz, RF, Millimeter, and Submillimeter-Wave Technology and Applications XII, Journal Name: Terahertz, RF, Millimeter, and Submillimeter-Wave Technology and Applications XII
Country of Publication:
United States
Language:
English

References (10)

Heterodyne phase-sensitive detection for calibration-free molecular dispersion spectroscopy journal January 2014
Chirped lasers dispersion spectroscopy implemented with single- and dual-sideband electro-optical modulators journal January 2013
Scanned-wavelength-modulation spectroscopy near 2.5 μm for H2O and temperature in a hydrocarbon-fueled scramjet combustor journal January 2014
Calibration-free wavelength modulation spectroscopy: symmetry approach and residual amplitude modulation normalization journal January 2016
Chirped laser dispersion spectroscopy with differential frequency generation source journal January 2014
Dual-sideband heterodyne of dispersion spectroscopy based on phase-sensitive detection journal January 2016
Molecular dispersion spectroscopy for chemical sensing using chirped mid-infrared quantum cascade laser journal January 2010
Sensitivity limits of a tunable diode laser spectrometer, with application to the detection of NO_2 at the 100-ppt level journal January 1980
Calibration-free wavelength modulated TDLAS under high absorbance conditions journal January 2011
Signal-to-noise ratio in chirped laser dispersion spectroscopy journal December 2011

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