High-pressure inelastic neutron scattering study of the anisotropic S=1 spin chain [Ni(HF2)(3-Clpyradine)4]BF4

Pajerowski, Daniel M.; Podlesnyak, Andrey P.; Herbrych, Jacek; Manson, Jamie

doi:10.1103/physrevb.105.134420

High-pressure inelastic neutron scattering study of the anisotropic S=1 spin chain [ Ni ( HF2 ) ( 3-Clpyradine ) 4 ] B F4

Journal Article · Mon Apr 18 00:00:00 EDT 2022 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.105.134420· OSTI ID:1864419

^[1]; ^[1]; Herbrych, Jacek ^[2]; Manson, Jamie ^[3]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Wrocław Univ. of Science and Technology (Poland)
Eastern Washington Univ., Cheney, WA (United States)

[Ni(HF₂)(3-Clpyradine)₄]BF₄ (NBCT) is a one-dimensional, S=1 spin-chain material that shows no long-range magnetic order down to thermometer temperatures of 0.1 K. Previous ambient pressure inelastic neutron scattering experiments identified NBCT to be in the large-D quantum paramagnetic phase of the D/J phase diagram, where D is the axial single-ion anisotropy and J is the intrachain superexchange. In this work, we extend the previous experiments to a hydrostatic pressure of 0.9 GPa. By comparing to density matrix renormalization group calculations, we find D/J increases from 1.5 to 3.2 as pressure increases from 0 GPa to 0.9 GPa, which pushes the system further into the large-D phase.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: Polish National Agency for Academic Exchange (NAWA); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1864419

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 13 Vol. 105; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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High-pressure inelastic neutron scattering study of the anisotropic S=1 spin chain [ Ni ( HF2 ) ( 3-Clpyradine ) 4 ] B F4

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