CO2 chirped-probe-pulse femtosecond CARS thermometry

Gu, Mingming; Satija, Aman; Lucht, Robert P.

doi:10.1016/j.proci.2020.06.134

Title: CO₂ chirped-probe-pulse femtosecond CARS thermometry

Journal Article · Sat Aug 15 00:00:00 EDT 2020 · Proceedings of the Combustion Institute

DOI:https://doi.org/10.1016/j.proci.2020.06.134· OSTI ID:1849427

^[1]; Satija, Aman ^[1];

^[1]

Purdue University, West Lafayette, IN (United States)

The application of CO₂ chirped-probe-pulse (CPP) fs coherent anti-Stokes Raman scattering (CARS) for flame thermometry is discussed. A phenomenological model for CO₂/O₂ CPP fs CARS was developed, and the simulations showed the potential for CO₂ temperature measurements free of interferences from O₂ and with no contribution from the nonresonant background by using a long-time delay for the chirped probe pulse. The accuracy and precision for CO₂ CPP fs CARS thermometry is compared with N₂ CPP fs CARS thermometry for temperatures between 295 K and 1420 K. The measurement accuracy for the CO₂ measurements is comparable with that for the N₂ measurements, while the precision for the CO₂ temperature measurements is significantly better at lower temperatures. In conclusion, we also demonstrate that accurate flame thermometry using a single set of laser parameters can be achieved using the delayed CPP approach.

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Research Organization:: Purdue Univ., West Lafayette, IN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-03ER15391

OSTI ID:: 1849427

Alternate ID(s):: OSTI ID: 1777024

Journal Information:: Proceedings of the Combustion Institute, Vol. 38, Issue 1; ISSN 1540-7489

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Thermodynamics
Energy & Fuels
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Title: CO2 chirped-probe-pulse femtosecond CARS thermometry

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Title: CO₂ chirped-probe-pulse femtosecond CARS thermometry