Strength, deformation, and equation of state of tungsten carbide to 66 GPa

Brugman, B. L.; Lin, F.; Lv, M.; Kenney-Benson, C.; Popov, D.; Miyagi, L.; Dorfman, S. M.

doi:10.1016/j.actamat.2021.117301

Title: Strength, deformation, and equation of state of tungsten carbide to 66 GPa

Journal Article · Thu Sep 09 00:00:00 EDT 2021 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2021.117301· OSTI ID:1830374

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^[3]; Kenney-Benson, C. ^[4]; Popov, D. ^[4]; Miyagi, L. ^[2];

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Michigan State Univ., East Lansing, MI (United States); Arizona State Univ., Tempe, AZ (United States)
Univ. of Utah, Salt Lake City, UT (United States)
Michigan State Univ., East Lansing, MI (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Here, strength, texture, and equation of state of hexagonal tungsten monocarbide (WC) have been determined under quasi-hydrostatic and non-hydrostatic compression to 66 GPa using angle-dispersive X-ray diffraction in the diamond anvil cell. Quasi-hydrostatic compression in a Ne pressure medium demonstrates that nanocrystalline WC is slightly less incompressible than bulk-scale WC, with respective bulk moduli of K₀ = 377 ± 7 and 397 ± 7 GPa and pressure derivatives K₀’ = 3.8 ± 0.3 and 3.7 ±0.3. This decrease in incompressibility with grain size is similar to behavior observed in other ceramics. Under nonhydrostatic compression, WC supports a mean differential stress of ~12-15 GPa at plastic yielding, which occurs at ~30 GPa. Strength in WC is anisotropic, with the (001) plane supporting 29-42% higher stress than stresses calculated from mean strain. Simulations using an Elasto-ViscoPlastic Self-Consistent model indicate that strength inferred from lattice strain theory may be overestimated due to effects of plastic deformation. Plastic deformation generates a texture maximum near $$\langle\bar{2}110\rangle$$ in the compression orientation, initially through prismatic slip on the {$$10\bar{1}0$$}$$\langle\bar{1}2\bar{1}0\rangle$$ and {$$10\bar{1}0$$}$$\langle0001\rangle$$ slip systems, followed by activation of pyramidal slip on {$$10\bar{1}1$$}$$\langle\bar{2}113\rangle$$ at ~40-50 GPa.

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Research Organization:: Univ. of Illinois, Chicago, IL (United States); Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP); National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division

Grant/Contract Number:: NA0003975; AC02-06CH11357; EAR 1663442; EAR 1654687

OSTI ID:: 1830374

Alternate ID(s):: OSTI ID: 1840908

Journal Information:: Acta Materialia, Vol. 220; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
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tungsten carbide

Title: Strength, deformation, and equation of state of tungsten carbide to 66 GPa

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