Nanoarchitectonics of Metal–Organic Frameworks for Capacitive Deionization via Controlled Pyrolyzed Approaches

Wang, Hao; Chen, Biaohua; Liu, Di‐Jia; Xu, Xingtao; Osmieri, Luigi; Yamauchi, Yusuke

doi:10.1002/smll.202102477

Title: Nanoarchitectonics of Metal–Organic Frameworks for Capacitive Deionization via Controlled Pyrolyzed Approaches

Journal Article · Tue Sep 28 00:00:00 EDT 2021 · Small

DOI:https://doi.org/10.1002/smll.202102477· OSTI ID:1822952

Wang, Hao ^[1]; Chen, Biaohua ^[2]; Liu, Di‐Jia ^[3]; Xu, Xingtao ^[4]; Osmieri, Luigi ^[5];

^[6]

Faculty of Environment and Life Beijing University of Technology Beijing 100124 China, Chemical Sciences and Engineering Division Argonne National Laboratory Lemont IL 60439 USA
Faculty of Environment and Life Beijing University of Technology Beijing 100124 China
Chemical Sciences and Engineering Division Argonne National Laboratory Lemont IL 60439 USA, Pritzker School of Molecular Engineering The University of Chicago Chicago IL 60637 USA
JST‐ERATO Yamauchi Materials Space‐Tectonics Project and International Center for Materials Nanoarchitectonics (WPI‐MANA) National Institute for Materials Science Ibaraki 305‐0044 Japan
Department of Applied Science and Technology Politecnico di Torino Corso Duca degli Abruzzi 24 Torino 10129 Italy
Australian Institute for Bioengineering and Nanotechnology (AIBN) The University of Queensland Brisbane Queensland 4072 Australia

Abstract Next‐generation desalination technologies are needed to meet the increasing demand for clean water. Capacitive deionization (CDI) is a thermodynamically efficient technique to treat non‐potable water with relatively low salinity. The salt removal capacity and rate of CDI are highly dependent on the electrode materials, which are preferentially porous to store ions through electrosorption and/or redox reactions. Metal–organic frameworks (MOFs) with “infinite” combinations of transition metals and organic linkers simplify the production of carbonaceous materials often with redox‐active components after pyrolysis. MOFs‐derived materials show great tunability in both compositions and structures but require further refinement to improve CDI performance. This review article summarizes recent progress in derivatives of MOFs and MOF‐like materials used as CDI electrodes, focusing on the structural and compositional material considerations as well as the processing parameters and electrode architectures of the device. Furthermore, the challenges and opportunities associated with this research area are also discussed.

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Sponsoring Organization:: USDOE

OSTI ID:: 1822952

Journal Information:: Small, Journal Name: Small Vol. 18 Journal Issue: 2; ISSN 1613-6810

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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