Low-temperature high-frequency dynamic magnetic susceptibility of classical spin-ice Dy2Ti2O7

Teknowijoyo, S.; Cho, K.; Timmons, E. I.; Tanatar, M. A.; Krizan, J. W.; Cava, R. J.; Prozorov, R.

doi:10.1088/1361-648x/ac1cb0

Low-temperature high-frequency dynamic magnetic susceptibility of classical spin-ice Dy₂Ti₂O₇

Journal Article · Mon Aug 30 04:00:00 EDT 2021 · Journal of Physics. Condensed Matter

DOI:https://doi.org/10.1088/1361-648x/ac1cb0· OSTI ID:1820993

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Ames Lab., and Iowa State Univ., Ames, IA (United States)
Ames Lab., Ames, IA (United States)
Princeton Univ., NJ (United States)

In this study, radio-frequency (14.6 MHz) AC magnetic susceptibility, , of Dy₂Ti₂O₇ was measured using self-oscillating tunnel-diode resonator. Measurements were made with the excitation AC field parallel to the superimposed DC magnetic field up to 5 T in a wide temperature range from 50 mK to 100 K. At 14.6 MHz, a known broad peak of from kHz—range audio-frequency measurements around 15 K for both [111] and [110] directions shifts to 45 K, continuing the Arrhenius activated behavior with the same activation energy barrier of E_a ≈ 230 K. Magnetic field dependence of along [111] reproduces previously reported low-temperature two-in-two-out to three-in-one-out spin configuration transition at about 1 T, and an intermediate phase between 1 and 1.5 T. The boundaries of the intermediate phase show reasonable overlap with the literature data and connect at a critical endpoint of the first order transition line, suggesting that these features are frequency independent. An unusual upturn of the magnetic susceptibility at T → 0 was observed in magnetic fields between 1.5 T and 2 T for both magnetic field directions, before fully polarized configuration sets in above 2 T.

View Accepted Manuscript (DOE)

Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-07CH11358; SC0019331

OSTI ID:: 1820993

Report Number(s):: IS--J-10,591

Journal Information:: Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 45 Vol. 33; ISSN 0953-8984

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Low-temperature high-frequency dynamic magnetic susceptibility of classical spin-ice Dy2Ti2O7

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Low-temperature high-frequency dynamic magnetic susceptibility of classical spin-ice Dy₂Ti₂O₇