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Title: Evidence for a Magnetic-Field-Induced Ideal Type-II Weyl State in Antiferromagnetic Topological Insulator Mn ( Bi 1 x Sb x ) 2 Te 4

Journal Article · · Physical Review. X

The discovery of Weyl semimetals (WSMs) has fueled tremendous interest in condensed matter physics. The realization of WSMs requires the breaking of either inversion symmetry (IS) or time-reversal symmetry (TRS). WSMs can be categorized into type-I and type-II WSMs, which are characterized by untilted and strongly tilted Weyl cones, respectively. Type-I WSMs with breaking of either IS or TRS and type-II WSMs with solely broken IS have been realized experimentally, but a TRS-breaking type-II WSM still remains elusive. In this article, we report transport evidence for a TRS-breaking type-II WSM observed in the intrinsic antiferromagnetic topological insulator Mn(Bi1-xSbx)2Te4 under magnetic fields. This state is manifested by the electronic structure transition caused by the spin-flop transition. The transition results in an intrinsic anomalous Hall effect and negative c -axis longitudinal magnetoresistance attributable to the chiral anomaly in the ferromagnetic phases of lightly hole-doped samples. Our results establish a promising platform for exploring the underlying physics of the long-sought, ideal TRS-breaking type-II WSM.

Research Organization:
Pennsylvania State Univ., University Park, PA (United States); Univ. of Arkansas, Fayetteville, AR (United States); Univ. of California, Oakland, CA (United States)
Sponsoring Organization:
USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; National Science Foundation (NSF)
Grant/Contract Number:
SC0019467; SC0019064; AC02-05-CH11231; AC02-05CH11231; DMR-1539916; DM-1917579; DMR 1644779; DMR-2011839; DMR-1847811
OSTI ID:
1812765
Alternate ID(s):
OSTI ID: 1852798
Journal Information:
Physical Review. X, Journal Name: Physical Review. X Vol. 11 Journal Issue: 3; ISSN 2160-3308
Publisher:
American Physical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (62)

Generalized Gradient Approximation Made Simple journal October 1996
Large intrinsic anomalous Hall effect in half-metallic ferromagnet Co3Sn2S2 with magnetic Weyl fermions journal September 2018
Fermi-arc diversity on surface terminations of the magnetic Weyl semimetal Co 3 Sn 2 S 2 journal September 2019
Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal journal July 2018
Ideal Weyl points and helicoid surface states in artificial photonic crystal structures journal January 2018
Topological surface Fermi arcs in the magnetic Weyl semimetal Co 3 Sn 2 S 2 journal June 2018
Time-reversal symmetry breaking type-II Weyl state in YbMnBi2 journal July 2019
Site Mixing for Engineering Magnetic Topological Insulators journal May 2021
Signatures of a time-reversal symmetric Weyl semimetal with only four Weyl points journal October 2017
Topological Materials: Weyl Semimetals journal March 2017
Time-Reversal-Breaking Weyl Fermions in Magnetic Heusler Alloys journal November 2016
Giant anomalous Nernst effect and quantum-critical scaling in a ferromagnetic semimetal journal July 2018
Large anomalous Hall effect in a half-Heusler antiferromagnet journal July 2016
Discovery of a new type of topological Weyl fermion semimetal state in MoxW1−xTe2 journal December 2016
Experimental observation of topological Fermi arcs in type-II Weyl semimetal MoTe2 journal September 2016
Chern Semimetal and the Quantized Anomalous Hall Effect in HgCr 2 Se 4 journal October 2011
Spin scattering and noncollinear spin structure-induced intrinsic anomalous Hall effect in antiferromagnetic topological insulator MnB i 2 T e 4 journal August 2019
Electron-energy-loss spectra and the structural stability of nickel oxide: An LSDA+U study journal January 1998
Weyl Semimetal Phase in Noncentrosymmetric Transition-Metal Monophosphides journal March 2015
Topological Axion States in the Magnetic Insulator MnBi 2 Te 4 with the Quantized Magnetoelectric Effect journal May 2019
Tracking surface photovoltage dipole geometry in Bi 2 Se 3 with time-resolved photoemission journal October 2019
Transport of Topological Semimetals journal July 2019
Experimental Discovery of Weyl Semimetal TaAs journal July 2015
Quantum oscillations in the field-induced ferromagnetic state of Mn Bi 2 x Sb x Te 4 journal May 2021
Transport evidence for Fermi-arc-mediated chirality transfer in the Dirac semimetal Cd3As2 journal July 2016
Negative flat band magnetism in a spin–orbit-coupled correlated kagome magnet journal February 2019
Fully unconstrained noncollinear magnetism within the projector augmented-wave method journal November 2000
Intrinsic anomalous Hall effect in type-II Weyl semimetals journal June 2016
Quantum Hall effect based on Weyl orbits in Cd3As2 journal December 2018
Weyl semimetal phase in the non-centrosymmetric compound TaAs journal August 2015
Anomalous Hall Effect in Weyl Metals journal October 2014
TaIrTe 4 : A ternary type-II Weyl semimetal journal May 2016
Intrinsic magnetic topological insulators in van der Waals layered MnBi 2 Te 4 -family materials journal June 2019
A consistent and accurate ab initio parametrization of density functional dispersion correction (DFT-D) for the 94 elements H-Pu journal April 2010
Spin fluctuation induced Weyl semimetal state in the paramagnetic phase of EuCd 2 As 2 journal July 2019
Weyl and Dirac semimetals in three-dimensional solids journal January 2018
Recent Progress in the Study of Topological Semimetals journal April 2018
Magnetic Weyl semimetal phase in a Kagomé crystal journal September 2019
Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2 journal July 2016
Generalized Gradient Approximation Made Simple [Phys. Rev. Lett. 77, 3865 (1996)] journal February 1997
Type-II Weyl semimetals journal November 2015
High-Chern-number and high-temperature quantum Hall effect without Landau levels journal April 2020
Evolution of structural, magnetic, and transport properties in MnBi 2 x Sb x Te 4 journal September 2019
Discovery of Lorentz-violating type II Weyl fermions in LaAlGe journal June 2017
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal October 1996
Ideal Weyl semimetal induced by magnetic exchange journal November 2019
Crystal growth and magnetic structure of MnBi 2 Te 4 journal June 2019
Interplay between interaction and chiral anomaly: Anisotropy in the electrical resistivity of interacting Weyl metals journal May 2013
Discovery of a Weyl fermion semimetal and topological Fermi arcs journal July 2015
Intrinsic magnetic topological insulator phases in the Sb doped MnBi2Te4 bulks and thin flakes journal October 2019
Quantum anomalous Hall effect in intrinsic magnetic topological insulator MnBi 2 Te 4 journal January 2020
Robust axion insulator and Chern insulator phases in a two-dimensional antiferromagnetic topological insulator journal January 2020
Quantum oscillations from surface Fermi arcs in Weyl and Dirac semimetals journal October 2014
Realization of interlayer ferromagnetic interaction in MnS b 2 T e 4 toward the magnetic Weyl semimetal state journal November 2019
Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet journal September 2019
Chiral anomaly and classical negative magnetoresistance of Weyl metals journal September 2013
Prediction and observation of an antiferromagnetic topological insulator journal December 2019
Ferromagnetism in van der Waals compound MnS b 1.8 B i 0.2 T e 4 journal June 2020
The chiral anomaly and thermopower of Weyl fermions in the half-Heusler GdPtBi journal June 2016
Topological semimetal and Fermi-arc surface states in the electronic structure of pyrochlore iridates journal May 2011
Single pair of Weyl fermions in the half-metallic semimetal EuC d 2 A s 2 journal June 2019
A Weyl Fermion semimetal with surface Fermi arcs in the transition metal monopnictide TaAs class journal June 2015