Dynamics of polymer segments, polymer chains, and nanoparticles in polymer nanocomposite melts: A review

Bailey, Eric J.; Winey, Karen I.

doi:10.1016/j.progpolymsci.2020.101242

Dynamics of polymer segments, polymer chains, and nanoparticles in polymer nanocomposite melts: A review

Journal Article · Tue Apr 14 00:00:00 EDT 2020 · Progress in Polymer Science

DOI:https://doi.org/10.1016/j.progpolymsci.2020.101242· OSTI ID:1797286

Bailey, Eric J. ^[1]; Winey, Karen I. ^[2]

Univ. of Pennsylvania, Philadelphia, PA (United States); University of Pennsylvania
Univ. of Pennsylvania, Philadelphia, PA (United States)

The addition of nanoparticles (NPs) to a polymer matrix, forming a polymer nanocomposite (PNC), is known to alter the microscopic dynamic processes of both species which leads to unique macroscopic material properties of the PNC. Because the NPs and polymers have overlapping characteristic length, time, and energy scales, the interactions within these materials are complex and the dynamics are interrelated. In this review, we present an overview of experimental, simulation, and theoretical results that probe multi-scale polymer and nanoparticle dynamics in polymer nanocomposites and navigate the dense parameter space presented by these multicomponent systems. Although a variety of PNC systems are mentioned, we focus this discussion on linear thermoplastics filled with hard spherical or cylindrical NPs in the melt state. We begin by introducing PNCs, the dynamic processes within them, and the importance of dynamics for properties and processing. At the smallest length and time scales, we discuss segmental dynamics in PNCs, including the role of polymer attributes, NP attributes, and NP-polymer interactions. Then, we present measurements of collective motions and intermediate (Rouse) dynamics in various PNC materials. At longer length and time scales, we discuss polymer center-of-mass diffusion in PNCs with either spherical or anisotropic NPs. We then explore the dynamics of the NPs in PNCs and polymer melts, including theoretical predictions, simulation results, and experimental observations. Lastly, we note some of the remaining challenges in probing dynamics in PNC materials and fundamentally studying PNCs more generally.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Pennsylvania, Philadelphia, PA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0016421

OSTI ID:: 1797286

Alternate ID(s):: OSTI ID: 1776318

Journal Information:: Progress in Polymer Science, Journal Name: Progress in Polymer Science Vol. 105; ISSN 0079-6700

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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