Nonresonant pump/probe electronic Raman scattering within nonequilibrium dynamical mean-field theory

Freericks, James K.; Matveev, Oleh P.; Shvaika, Andrij M.; Devereaux, Thomas P.

doi:10.1117/12.2305103

Nonresonant pump/probe electronic Raman scattering within nonequilibrium dynamical mean-field theory

Journal Article · Tue May 08 00:00:00 EDT 2018 · Proceedings of SPIE - The International Society for Optical Engineering

DOI:https://doi.org/10.1117/12.2305103· OSTI ID:1783723

Freericks, James K. ^[1]; Matveev, Oleh P. ^[2]; Shvaika, Andrij M. ^[2]; Devereaux, Thomas P. ^[3]

Georgetown Univ., Washington, DC (United States); Georgetown University
Inst. for Condensed Matter Physics of the National Academy of Sciences of Ukraine, Lviv (Ukraine)
Stanford Univ., CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

We develop the theory for nonresonant Raman scattering of strongly correlated electrons in time-resolved pump-probe experiments. The electrons are initially pumped with an intense pulse of light and then a probe pulse measures the Raman response function after an adjustable time delay. Here, we describe how the width of the probe pulse and the strength of the electron correlations affect the Raman cross section. The theory is developed for the case of B_1g symmetry, where incident and scattered light are polarized perpendicular to each other. We illustrate the exact solution with the Falicov-Kimball model, which is solved via nonequilibrium dynamical mean-field theory.

View Accepted Manuscript (DOE)

Research Organization:: Georgetown Univ., Washington, DC (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: FG02-08ER46542; AC02-76SF00515; AC02-05CH11231

OSTI ID:: 1783723

Alternate ID(s):: OSTI ID: 1544279

Journal Information:: Proceedings of SPIE - The International Society for Optical Engineering, Journal Name: Proceedings of SPIE - The International Society for Optical Engineering Vol. 10638; ISSN 0277-786X

Publisher:: SPIECopyright Statement

Country of Publication:: United States

Language:: English

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Cited By (1)

Stroboscopic Tests for Thermalization of Electrons in Pump-Probe Experiments Matveev, O. P.; Shvaika, A. M.; Devereaux, T. P. Physical Review Letters, Vol. 122, Issue 24 https://doi.org/10.1103/physrevlett.122.247402	journal	June 2019

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Related Subjects

75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY
Condensed matter physics
Electrons
Falicov-Kimball model
Light scattering
Nonequilibrium Raman scattering
Nonequilibrium dynamical mean-field theory
Photons
Physics
Polarization
Pump-probe spectroscopy
Raman scattering
Raman spectroscopy
Scattering
Solids
Strongly correlated electrons

Nonresonant pump/probe electronic Raman scattering within nonequilibrium dynamical mean-field theory

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References (16)

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