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Theoretical description of pump/probe experiments in nesting induced charge density wave insulators

Journal Article · · Proceedings of SPIE - The International Society for Optical Engineering
DOI:https://doi.org/10.1117/12.2223335· OSTI ID:1783721
 [1];  [2];  [3];  [4]
  1. Georgetown Univ., Washington, DC (United States); Georgetown University
  2. Georgetown Univ., Washington, DC (United States); Inst. for Condensed Matter Physics of National Academy of Sciences of Ukraine, Lviv (Ukraine)
  3. Inst. for Condensed Matter Physics of National Academy of Sciences of Ukraine, Lviv (Ukraine)
  4. Geballe Lab. for Advanced Materials, Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)

We present a theoretical description of time-resolved photoemission in charge-density-wave insulators that derive their ordering from electron nesting effects. In these pump/probe experiments, a large amplitude (but short duration) pump pulse excites the system into nonequilibrium and then a higher frequency low amplitude probe pulse photoexcites electrons, which are measured at the detector. We describe effects of electron correlations on the photoelectron spectroscopy and provide details for the theoretical techniques used to solve these problems. Here, we also show how the gap fills in as the system is excited, even though the order parameter does not go to zero. The theory is developed for the Falicov-Kimball model, which can be solved exactly with nonequilibrium dynamical mean-field theory.

Research Organization:
Georgetown Univ., Washington, DC (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division
Grant/Contract Number:
FG02-08ER46542
OSTI ID:
1783721
Journal Information:
Proceedings of SPIE - The International Society for Optical Engineering, Journal Name: Proceedings of SPIE - The International Society for Optical Engineering Vol. 9835; ISSN 0277-786X
Publisher:
SPIECopyright Statement
Country of Publication:
United States
Language:
English

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Cited By (2)

Theoretical description of pump/probe experiments in electron-mediated charge-density-wave insulators journal February 2017
Time-domain pumping a quantum-critical charge density wave ordered material journal September 2016

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