Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces

Mann, Sander A.; Nookala, Nishant; Johnson, Samuel C.; Cotrufo, Michele; Mekawy, Ahmed; Klem, John F.; Brener, Igal; Raschke, Markus B.; Alù, Andrea; Belkin, Mikhail A.

doi:10.1364/OPTICA.415581

Ultrafast optical switching and power limiting in intersubband polaritonic metasurfaces

Journal Article · Thu Apr 29 00:00:00 EDT 2021 · Optica

DOI:https://doi.org/10.1364/OPTICA.415581· OSTI ID:1779953

; Nookala, Nishant; ; ; Mekawy, Ahmed; Klem, John F.; Brener, Igal; ; ;

Highly nonlinear optical materials with fast third-order nonlinear optical response are crucial for the operation of all-optical photonic devices, such as switches for signal processing and computation, power limiters, and saturable absorbers. The nonlinear response of traditional optical materials is weak, thus requiring large light intensities to induce significant changes in their properties. Here we show that optical control of the coupling rate in subwavelength patch antennas coupled to intersubband transitions in multi-quantum-well semiconductor heterostructures can provide a giant third-order nonlinear response, on the order of ${3.4 \times <#comment/> 10}^{- <#comment/> 13} m^{2} / V^{2}$ , with a response time $< <#comment/> 2 p s$ . We utilize this effect to realize intersubband polaritonic metasurfaces and demonstrate their operation as highly nonlinear saturable and reverse saturable absorbers, enabling optical power limiters and other elements for all-optical modulation and control. Our approach enables a plethora of compact, low-power, highly nonlinear devices with spectral, temporal, and structured wavefront responses tailored by design.

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Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: NA0003525

OSTI ID:: 1779953

Journal Information:: Optica, Journal Name: Optica Journal Issue: 5 Vol. 8; ISSN 2334-2536

Publisher:: Optical Society of AmericaCopyright Statement

Country of Publication:: United States

Language:: English

References (56)

Nanostructured Plasmonic Medium for Terahertz Bandwidth All-Optical Switching Ren, Mengxin; Jia, Baohua; Ou, Jun-Yu Advanced Materials, Vol. 23, Issue 46 https://doi.org/10.1002/adma.201103162	journal	October 2011
Emerging Low-Dimensional Materials for Nonlinear Optics and Ultrafast Photonics Liu, Xiaofeng; Guo, Qiangbing; Qiu, Jianrong Advanced Materials, Vol. 29, Issue 14 https://doi.org/10.1002/adma.201605886	journal	February 2017
Ultrathin Second‐Harmonic Metasurfaces with Record‐High Nonlinear Optical Response Lee, Jongwon; Nookala, Nishant; Gomez‐Diaz, J. Sebastian Advanced Optical Materials, Vol. 4, Issue 5 https://doi.org/10.1002/adom.201500723	journal	February 2016
Difference-Frequency Generation in Polaritonic Intersubband Nonlinear Metasurfaces Liu, Yingnan; Lee, Jongwon; March, Stephen Advanced Optical Materials, Vol. 6, Issue 20 https://doi.org/10.1002/adom.201800681	journal	August 2018
Non-linear population processes of Er3+ laser levels in chromium-doped garnet crystals Noginov, M. A.; Smirnov, V. A.; Shcherbakov, I. A. Optical and Quantum Electronics, Vol. 22, Issue S1 https://doi.org/10.1007/BF02089001	journal	July 1990
Nonlinear Fano-Resonant Dielectric Metasurfaces Yang, Yuanmu; Wang, Wenyi; Boulesbaa, Abdelaziz Nano Letters, Vol. 15, Issue 11, p. 7388-7393 https://doi.org/10.1021/acs.nanolett.5b02802	journal	October 2015
Ultrafast All-Optical Switching with Magnetic Resonances in Nonlinear Dielectric Nanostructures Shcherbakov, Maxim R.; Vabishchevich, Polina P.; Shorokhov, Alexander S. Nano Letters, Vol. 15, Issue 10 https://doi.org/10.1021/acs.nanolett.5b02989	journal	September 2015
Resonantly Enhanced Second-Harmonic Generation Using III–V Semiconductor All-Dielectric Metasurfaces Liu, Sheng; Sinclair, Michael B.; Saravi, Sina Nano Letters, Vol. 16, Issue 9, p. 5426-5432 https://doi.org/10.1021/acs.nanolett.6b01816	journal	August 2016
Resonant Nanophotonic Spectrum Splitting for Ultrathin Multijunction Solar Cells Mann, Sander A.; Garnett, Erik C. ACS Photonics, Vol. 2, Issue 7 https://doi.org/10.1021/acsphotonics.5b00260	journal	July 2015
Low-Power Absorption Saturation in Semiconductor Metasurfaces Zubyuk, Varvara V.; Vabishchevich, Polina P.; Shcherbakov, Maxim R. ACS Photonics, Vol. 6, Issue 11 https://doi.org/10.1021/acsphotonics.9b00842	journal	September 2019
Plexciton Dynamics: Exciton−Plasmon Coupling in a J-Aggregate−Au Nanoshell Complex Provides a Mechanism for Nonlinearity Fofang, Nche T.; Grady, Nathaniel K.; Fan, Zhiyuan Nano Letters, Vol. 11, Issue 4 https://doi.org/10.1021/nl104352j	journal	April 2011
Quantum Plexcitonics: Strongly Interacting Plasmons and Excitons Manjavacas, A.; García de Abajo, F. J.; Nordlander, P. Nano Letters, Vol. 11, Issue 6 https://doi.org/10.1021/nl200579f	journal	May 2011
Ultrafast Manipulation of Strong Coupling in Metal−Molecular Aggregate Hybrid Nanostructures Vasa, P.; Pomraenke, R.; Cirmi, G. ACS Nano, Vol. 4, Issue 12 https://doi.org/10.1021/nn101973p	journal	November 2010
Sub-cycle switch-on of ultrastrong light–matter interaction Günter, G.; Anappara, A. A.; Hees, J. Nature, Vol. 458, Issue 7235 https://doi.org/10.1038/nature07838	journal	March 2009
Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos Nature, Vol. 511, Issue 7507 https://doi.org/10.1038/nature13455	journal	July 2014
Strong coupling in the sub-wavelength limit using metamaterial nanocavities Benz, A.; Campione, S.; Liu, S. Nature Communications, Vol. 4, Article No. 2882 https://doi.org/10.1038/ncomms3882	journal	November 2013
Nonlinear plasmonics Kauranen, Martti; Zayats, Anatoly V. Nature Photonics, Vol. 6, Issue 11 https://doi.org/10.1038/nphoton.2012.244	journal	November 2012
Real-time observation of ultrafast Rabi oscillations between excitons and plasmons in metal nanostructures with J-aggregates Vasa, Parinda; Wang, Wei; Pomraenke, Robert Nature Photonics, Vol. 7, Issue 2 https://doi.org/10.1038/nphoton.2012.340	journal	January 2013
Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber Yang, Yuanmu; Kelley, Kyle; Sachet, Edward Nature Photonics, Vol. 11, Issue 6 https://doi.org/10.1038/nphoton.2017.64	journal	May 2017
Large optical nonlinearity of nanoantennas coupled to an epsilon-near-zero material Alam, M. Zahirul; Schulz, Sebastian A.; Upham, Jeremy Nature Photonics, Vol. 12, Issue 2 https://doi.org/10.1038/s41566-017-0089-9	journal	January 2018
High-harmonic generation from an epsilon-near-zero material Yang, Yuanmu; Lu, Jian; Manjavacas, Alejandro Nature Physics, Vol. 15, Issue 10 https://doi.org/10.1038/s41567-019-0584-7	journal	July 2019
Ultrastrong coupling between light and matter Frisk Kockum, Anton; Miranowicz, Adam; De Liberato, Simone Nature Reviews Physics, Vol. 1, Issue 1 https://doi.org/10.1038/s42254-018-0006-2	journal	January 2019
Tuning optical properties of metasurface via piezoelectric effect Mekawy, Ahmed; Khalifa, Mohammad; Ali, Tamer A. IET Optoelectronics, Vol. 13, Issue 3 https://doi.org/10.1049/iet-opt.2018.5045	journal	June 2019
Observation of large second order susceptibility via intersubband transitions at λ∼10 μm in asymmetric coupled AlInAs/GaInAs quantum wells Sirtori, Carlo; Capasso, Federico; Sivco, Deborah L. Applied Physics Letters, Vol. 59, Issue 18 https://doi.org/10.1063/1.106050	journal	October 1991
Transition from strong to ultrastrong coupling regime in mid-infrared metal-dielectric-metal cavities Jouy, P.; Vasanelli, A.; Todorov, Y. Applied Physics Letters, Vol. 98, Issue 23 https://doi.org/10.1063/1.3598432	journal	June 2011
Subwavelength optical absorber with an integrated photon sorter Le Perchec, J.; Desieres, Y.; Rochat, N. Applied Physics Letters, Vol. 100, Issue 11 https://doi.org/10.1063/1.3694749	journal	March 2012
Enhanced optical nonlinearities in the near-infrared using III-nitride heterostructures coupled to metamaterials Wolf, Omri; Allerman, Andrew A.; Ma, Xuedan Applied Physics Letters, Vol. 107, Issue 15, Article No. 151108 https://doi.org/10.1063/1.4933332	journal	October 2015
Third order optical nonlinearity of graphene Cheng, J. L.; Vermeulen, N.; Sipe, J. E. New Journal of Physics, Vol. 16, Issue 5 https://doi.org/10.1088/1367-2630/16/5/053014	journal	May 2014
Ultra-subwavelength resonators for high temperature high performance quantum detectors Palaferri, Daniele; Todorov, Yanko; Mottaghizadeh, Alireza New Journal of Physics, Vol. 18, Issue 11 https://doi.org/10.1088/1367-2630/18/11/113016	journal	November 2016
Nuclear Induction Bloch, F. Physical Review, Vol. 70, Issue 7-8 https://doi.org/10.1103/PhysRev.70.460	journal	October 1946
Theory of patch-antenna metamaterial perfect absorbers Bowen, Patrick T.; Baron, Alexandre; Smith, David R. Physical Review A, Vol. 93, Issue 6 https://doi.org/10.1103/PhysRevA.93.063849	journal	June 2016
Thin Perfect Absorbers for Electromagnetic Waves: Theory, Design, and Realizations Ra’di, Y.; Simovski, C. R.; Tretyakov, S. A. Physical Review Applied, Vol. 3, Issue 3 https://doi.org/10.1103/PhysRevApplied.3.037001	journal	March 2015
Second-order nonlinear effects in asymmetric quantum-well structures Khurgin, J. Physical Review B, Vol. 38, Issue 6 https://doi.org/10.1103/PhysRevB.38.4056	journal	August 1988
Transition from strong to weak coupling and the onset of lasing in semiconductor microcavities Butté, R.; Delalleau, G.; Tartakovskii, A. I. Physical Review B, Vol. 65, Issue 20 https://doi.org/10.1103/PhysRevB.65.205310	journal	April 2002
Wide-angle perfect absorber/thermal emitter in the terahertz regime Diem, Marcus; Koschny, Thomas; Soukoulis, C. M. Physical Review B, Vol. 79, Issue 3 https://doi.org/10.1103/PhysRevB.79.033101	journal	January 2009
Ultrafast optical bleaching of intersubband cavity polaritons Zanotto, Simone; Degl'Innocenti, Riccardo; Xu, Ji-Hua Physical Review B, Vol. 86, Issue 20 https://doi.org/10.1103/PhysRevB.86.201302	journal	November 2012
Ultrafast reversal of a Fano resonance in a plasmon-exciton system Shah, Raman A.; Scherer, Norbert F.; Pelton, Matthew Physical Review B, Vol. 88, Issue 7 https://doi.org/10.1103/PhysRevB.88.075411	journal	August 2013
Saturation and bistability of defect-mode intersubband polaritons Zanotto, Simone; Bianco, Federica; Sorba, Lucia Physical Review B, Vol. 91, Issue 8 https://doi.org/10.1103/PhysRevB.91.085308	journal	February 2015
Nonlinear processes in multi-quantum-well plasmonic metasurfaces: Electromagnetic response, saturation effects, limits, and potentials Gomez-Diaz, J. S.; Tymchenko, M.; Lee, J. Physical Review B, Vol. 92, Issue 12 https://doi.org/10.1103/PhysRevB.92.125429	journal	September 2015
Strong Light-Matter Coupling in Subwavelength Metal-Dielectric Microcavities at Terahertz Frequencies Todorov, Y.; Andrews, A. M.; Sagnes, I. Physical Review Letters, Vol. 102, Issue 18 https://doi.org/10.1103/PhysRevLett.102.186402	journal	May 2009
Ultrastrong Light-Matter Coupling Regime with Polariton Dots Todorov, Y.; Andrews, A. M.; Colombelli, R. Physical Review Letters, Vol. 105, Issue 19 https://doi.org/10.1103/PhysRevLett.105.196402	journal	November 2010
Ultrafast Nonlinear Optical Response of a Single Gold Nanorod near Its Surface Plasmon Resonance Baida, H.; Mongin, D.; Christofilos, D. Physical Review Letters, Vol. 107, Issue 5 https://doi.org/10.1103/PhysRevLett.107.057402	journal	July 2011
Thermalization and Cooling of Plasmon-Exciton Polaritons: Towards Quantum Condensation Rodriguez, S. R. K.; Feist, J.; Verschuuren, M. A. Physical Review Letters, Vol. 111, Issue 16 https://doi.org/10.1103/PhysRevLett.111.166802	journal	October 2013
Gradient Nonlinear Pancharatnam-Berry Metasurfaces Tymchenko, Mykhailo; Gomez-Diaz, J. Sebastian; Lee, Jongwon Physical Review Letters, Vol. 115, Issue 20 https://doi.org/10.1103/PhysRevLett.115.207403	journal	November 2015
Enhanced Nonlinear Refractive Index in ε -Near-Zero Materials Caspani, L.; Kaipurath, R. P. M.; Clerici, M. Physical Review Letters, Vol. 116, Issue 23 https://doi.org/10.1103/PhysRevLett.116.233901	journal	June 2016
Self-Induced Transparency by Pulsed Coherent Light McCall, S. L.; Hahn, E. L. Physical Review Letters, Vol. 18, Issue 21 https://doi.org/10.1103/PhysRevLett.18.908	journal	May 1967
Microcavity Polariton Splitting of Intersubband Transitions Dini, Dimitri; Köhler, Rüdeger; Tredicucci, Alessandro Physical Review Letters, Vol. 90, Issue 11 https://doi.org/10.1103/PhysRevLett.90.116401	journal	March 2003
Nonlinear optics of normal-mode-coupling semiconductor microcavities Khitrova, G.; Gibbs, H. M.; Jahnke, F. Reviews of Modern Physics, Vol. 71, Issue 5 https://doi.org/10.1103/RevModPhys.71.1591	journal	October 1999
Semiconductor saturable absorber mirrors (SESAM's) for femtosecond to nanosecond pulse generation in solid-state lasers Keller, U.; Weingarten, K. J.; Kartner, F. X. IEEE Journal of Selected Topics in Quantum Electronics, Vol. 2, Issue 3 https://doi.org/10.1109/2944.571743	journal	January 1996
Coupled quantum well semiconductors with giant electric field tunable nonlinear optical properties in the infrared Capasso, F.; Sirtori, C.; Cho, A. Y. IEEE Journal of Quantum Electronics, Vol. 30, Issue 5 https://doi.org/10.1109/3.303697	journal	May 1994
Theory of optical maser amplifiers Arecchi, F.; Bonifacio, R. IEEE Journal of Quantum Electronics, Vol. 1, Issue 4 https://doi.org/10.1109/JQE.1965.1072212	journal	July 1965
Light Propagation with Phase Discontinuities: Generalized Laws of Reflection and Refraction Yu, N.; Genevet, P.; Kats, M. A. Science, Vol. 334, Issue 6054 https://doi.org/10.1126/science.1210713	journal	September 2011
Quantum Engineering of Optical Nonlinearities Rosencher, E.; Fiore, A.; Vinter, B. Science, Vol. 271, Issue 5246 https://doi.org/10.1126/science.271.5246.168	journal	January 1996
Large optical nonlinearity of indium tin oxide in its epsilon-near-zero region Alam, M. Z.; De Leon, I.; Boyd, R. W. Science, Vol. 352, Issue 6287 https://doi.org/10.1126/science.aae0330	journal	April 2016
Nonlinear epsilon-near-zero materials explained: opinion Kinsey, N.; Khurgin, J. Optical Materials Express, Vol. 9, Issue 7 https://doi.org/10.1364/OME.9.002793	journal	January 2019
Ultrathin gradient nonlinear metasurface with a giant nonlinear response Nookala, Nishant; Lee, Jongwon; Tymchenko, Mykhailo Optica, Vol. 3, Issue 3 https://doi.org/10.1364/OPTICA.3.000283	journal	January 2016

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