Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Light-Induced Renormalization of the Dirac Quasiparticles in the Nodal-Line Semimetal ZrSiSe

Journal Article · · Physical Review Letters
 [1];  [1];  [1];  [2];  [2];  [2];  [1];  [1];  [1];  [1];  [1];  [3];  [3];  [4];  [5];  [6];  [6];  [7];  [1];  [1]
  1. Ecole Polytechnique Federale Lausanne (Switzerland)
  2. Max Planck Institute for the Structure and Dynamics of Matter. (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science
  3. National Research Council-Institute for Photonics and Nanotechnologies (CNR-IFN), Padova (Italy)
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS); Univ. of California, Berkeley, CA (United States)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS); Univ. of Wurzburg (Germany)
  6. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  7. Max Planck Institute for the Structure and Dynamics of Matter. (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science; Universidad del País Vasco, San Sebastian (Spain); Flatiron Institute, New York, NY (United States)
In nodal-line semimetals, linearly dispersing states form Dirac loops in the reciprocal space with a high degree of electron-hole symmetry and a reduced density of states near the Fermi level. The result is reduced electronic screening and enhanced correlations between Dirac quasiparticles. In this study we investigate the electronic structure of ZrSiSe, by combining time- and angle-resolved photoelectron spectroscopy with ab initio density functional theory (DFT) complemented by an extended Hubbard model ( DFT+U+V ) and by time-dependent DFT+U+V . We show that electronic correlations are reduced on an ultrashort timescale by optical excitation of high-energy electrons-hole pairs, which transiently screen the Coulomb interaction. Our findings demonstrate an all-optical method for engineering the band structure of a quantum material.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Swiss National Science Foundation (SNSF); European Research Council (ERC)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1775402
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 7 Vol. 125; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (59)

Evidence of Both Surface and Bulk Dirac Bands and Anisotropic Nonsaturating Magnetoresistance in ZrSiS journal August 2016
Semiempirical GGA-type density functional constructed with a long-range dispersion correction journal January 2006
Determining the electron-phonon mass enhancement parameter λ on metal surfaces journal February 2005
A First-Principles Time-Dependent Density Functional Theory Framework for Spin and Time-Resolved Angular-Resolved Photoelectron Spectroscopy in Periodic Systems journal December 2016
Dirac cone protected by non-symmorphic symmetry and three-dimensional Dirac line node in ZrSiS journal May 2016
Quantum criticality of topological phase transitions in three-dimensional interacting electronic systems journal August 2014
Unconventional mass enhancement around the Dirac nodal loop in ZrSiS journal November 2017
Strong-correlation induced high-mobility electrons in Dirac semimetal of perovskite oxide journal January 2019
Collapse of superconductivity in cuprates via ultrafast quenching of phase coherence journal April 2018
Electronic correlations in nodal-line semimetals journal April 2020
Real-space grids and the Octopus code as tools for the development of new simulation approaches for electronic systems journal January 2015
Hybrid functionals based on a screened Coulomb potential journal May 2003
Harmonium: A pulse preserving source of monochromatic extreme ultraviolet (30–110 eV) radiation for ultrafast photoelectron spectroscopy of liquids journal October 2015
Similar ultrafast dynamics of several dissimilar Dirac and Weyl semimetals journal December 2017
Large nonsaturating magnetoresistance and signature of nondegenerate Dirac nodes in ZrSiS journal February 2017
First-principles study of structural, mechanical, lattice dynamical and thermal properties of nodal-line semimetals ZrXY (X=Si,Ge; Y=S,Se) journal October 2016
Chiral anomaly and transport in Weyl metals journal February 2015
Topological nodal line semimetals journal November 2016
Electron thermalization in gold journal November 1992
Ab initiomolecular dynamics for liquid metals journal January 1993
Projector augmented-wave method journal December 1994
Marginal-Fermi-liquid behavior from two-dimensional Coulomb interaction journal January 1999
Topological semimetal and Fermi-arc surface states in the electronic structure of pyrochlore iridates journal May 2011
Topological nodal semimetals journal December 2011
Chiral anomaly, charge density waves, and axion strings from Weyl semimetals journal April 2013
Photoinduced changes in the cuprate electronic structure revealed by femtosecond time- and angle-resolved photoemission journal March 2014
Long-range Coulomb interaction in nodal-ring semimetals journal January 2016
Observation of topological nodal fermion semimetal phase in ZrSiS journal May 2016
Dirac line nodes and effect of spin-orbit coupling in the nonsymmorphic critical semimetals M SiS ( M = Hf , Zr ) journal March 2017
Tunability of the topological nodal-line semimetal phase in ZrSi X -type materials ( X = S ,   Se ,   Te ) journal April 2017
Interacting nodal-line semimetal: Proximity effect and spontaneous symmetry breaking journal July 2017
Nearly massless Dirac fermions and strong Zeeman splitting in the nodal-line semimetal ZrSiS probed by de Haas–van Alphen quantum oscillations journal July 2017
Lattice dynamics of Dirac node-line semimetal ZrSiS journal August 2017
Electron transport in nodal-line semimetals journal October 2017
Self-consistent DFT + U method for real-space time-dependent density functional theory calculations journal December 2017
Importance of nonlocal electron correlation in the BaNiS 2 semimetal from quantum oscillations studies journal February 2018
Excitonic instability and unconventional pairing in the nodal-line materials ZrSiS and ZrSiSe journal December 2018
Chemical pressure effect on the optical conductivity of the nodal-line semimetals ZrSi Y ( Y = S , Se , Te ) and ZrGe Y ( Y = S , Te ) journal March 2019
Evidence for bulk nodal loops and universality of Dirac-node arc surface states in ZrGe X c ( X c = S , Se, Te) journal June 2019
Charge Transport in Weyl Semimetals journal January 2012
Dirac Semimetal in Three Dimensions journal April 2012
Direct View of Hot Carrier Dynamics in Graphene journal July 2013
Dirac Line Nodes in Inversion-Symmetric Crystals journal July 2015
Evidence of Topological Nodal-Line Fermions in ZrSiSe and ZrSiTe journal June 2016
Flat Optical Conductivity in ZrSiS due to Two-Dimensional Dirac Bands journal November 2017
Excitonic Instability and Pseudogap Formation in Nodal Line Semimetal ZrSiS journal May 2018
Ultrafast Modification of Hubbard U in a Strongly Correlated Material: Ab initio High-Harmonic Generation in NiO journal August 2018
Evidence of a Coulomb-Interaction-Induced Lifshitz Transition and Robust Hybrid Weyl Semimetal in T d − MoTe 2 journal September 2018
Generalized Gradient Approximation Made Simple journal October 1996
Reformulation of DFT + U as a Pseudohybrid Hubbard Density Functional for Accelerated Materials Discovery journal January 2015
Surface Floating 2D Bands in Layered Nonsymmorphic Semimetals: ZrSiS and Related Compounds journal December 2017
Colloquium: Topological insulators journal November 2010
Weyl and Dirac semimetals in three-dimensional solids journal January 2018
Butterfly magnetoresistance, quasi-2D Dirac Fermi surface and topological phase transition in ZrSiS journal December 2016
Quantum Spin Hall Effect and Topological Phase Transition in HgTe Quantum Wells journal December 2006
Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission journal May 2012
Screening Effect and Impurity Scattering in Monolayer Graphene journal July 2006
Topological Semimetals in Square-Net Materials journal July 2019
Time-resolved ARPES at LACUS: Band Structure and Ultrafast Electron Dynamics of Solids journal May 2017

Cited By (3)


Similar Records

Electron transport in nodal-line semimetals
Journal Article · Wed Oct 11 00:00:00 EDT 2017 · Physical Review B · OSTI ID:1388198

Role of Lithium Codoping in Enhancing the Scintillation Yield of Aluminate Garnets
Journal Article · Thu Jun 25 00:00:00 EDT 2020 · Physical Review Applied · OSTI ID:1649422