Recent Advances in Rechargeable Aluminum-Ion Batteries and Considerations for Their Future Progress

Zhang, Kaiqiang; Kirlikovali, Kent O.; Suh, Jun Min; Choi, Ji-Won; Jang, Ho Won; Varma, Rajender S.; Farha, Omar K.; Shokouhimehr, Mohammadreza

doi:10.1021/acsaem.0c00957

Recent Advances in Rechargeable Aluminum-Ion Batteries and Considerations for Their Future Progress

Journal Article · Mon Jun 01 00:00:00 EDT 2020 · ACS Applied Energy Materials

DOI:https://doi.org/10.1021/acsaem.0c00957· OSTI ID:1771015

Zhang, Kaiqiang ^[1]; ^[2]; Suh, Jun Min ^[3]; ^[4]; ^[3]; ^[5]; ^[2]; ^[3]

Seoul National Univ. (Korea); Korea Inst. of Science and Technology (KIST), Seoul (Korea); University of Minnesota
Northwestern Univ., Evanston, IL (United States)
Seoul National Univ. (Korea)
Korea Inst. of Science and Technology (KIST), Seoul (Korea)
Palacky Univ., Olomouc (Czech Republic)

Owing to their high theoretical capacity and reliable operational safety, nonaqueous rechargeable aluminum batteries (RABs) have emerged as a promising class of battery materials and been intensively studied in recent years; however, a lack of suitable, high-performing positive electrode materials, along with the need for air-sensitive and expensive ionic liquid electrolytes, has significantly hindered the practical use of RABs in large-scale applications. Therefore, we sought to carefully analyze positive electrode materials and the associated electrolytes that have been reported in these battery systems in order to stimulate the design of the next generation of high-performance and low-cost RABs. In this review, we have summarized the electrode materials that have been used in both nonaqueous and aqueous RAB systems and provided a rational classification based on the types of materials used and their respective structures. Additionally, we have reviewed electrolytes employed in RABs and have categorized them according to two main types of applications, either for fixed battery systems or for use in portable devices. Here, a systematic account of recent developments on RABs, with a focus on electrode materials, innovative perspectives, and impending research efforts on future RABs, has been included. Finally, a proposed liquid RAB system is discussed with the aim of solving issues regarding fast-charging and long operational lifetimes, followed by insights into solid RABs for use in both portable and multistructural RAB systems.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: USDOE; Army Research Office; Korea Institute of Science and Technology Future Resource Program

Grant/Contract Number:: SC0008688

OSTI ID:: 1771015

Journal Information:: ACS Applied Energy Materials, Journal Name: ACS Applied Energy Materials Journal Issue: 7 Vol. 3; ISSN 2574-0962

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cascading Boost Effect on the Capacity of Nitrogen-Doped Graphene Sheets for Li- and Na-Ion Batteries Tian, Lei-Lei; Li, Si-Bai; Zhang, Ming-Jian ACS Applied Materials & Interfaces, Vol. 8, Issue 40 https://doi.org/10.1021/acsami.6b07390	journal	September 2016
Highly Oriented Graphene Sponge Electrode for Ultra High Energy Density Lithium Ion Hybrid Capacitors Ahn, Wook; Lee, Dong Un; Li, Ge ACS Applied Materials & Interfaces, Vol. 8, Issue 38 https://doi.org/10.1021/acsami.6b08298	journal	September 2016
High-Voltage and Noncorrosive Ionic Liquid Electrolyte Used in Rechargeable Aluminum Battery Wang, Huali; Gu, Sichen; Bai, Ying ACS Applied Materials & Interfaces, Vol. 8, Issue 41 https://doi.org/10.1021/acsami.6b10579	journal	October 2016
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Rechargeable Aluminum-Ion Battery Based on MoS ₂ Microsphere Cathode Li, Zhanyu; Niu, Bangbang; Liu, Jian ACS Applied Materials & Interfaces, Vol. 10, Issue 11 https://doi.org/10.1021/acsami.8b00100	journal	February 2018
One-Dimensional Cu _{2– x} Se Nanorods as the Cathode Material for High-Performance Aluminum-Ion Battery Jiang, Jiali; Li, He; Fu, Tao ACS Applied Materials & Interfaces, Vol. 10, Issue 21 https://doi.org/10.1021/acsami.8b03259	journal	May 2018
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Atomic Substitution Enabled Synthesis of Vacancy-Rich Two-Dimensional Black TiO _{2– x} Nanoflakes for High-Performance Rechargeable Magnesium Batteries Wang, Yanrong; Xue, Xiaolan; Liu, Pingying ACS Nano, Vol. 12, Issue 12 https://doi.org/10.1021/acsnano.8b06917	journal	November 2018
Rechargeable Nickel Telluride/Aluminum Batteries with High Capacity and Enhanced Cycling Performance Yu, Zhijing; Jiao, Shuqiang; Tu, Jiguo ACS Nano, Vol. 14, Issue 3 https://doi.org/10.1021/acsnano.9b09550	journal	March 2020
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An operando X-ray diffraction study of chloroaluminate anion-graphite intercalation in aluminum batteries Pan, Chun-Jern; Yuan, Chunze; Zhu, Guanzhou Proceedings of the National Academy of Sciences, Vol. 115, Issue 22 https://doi.org/10.1073/pnas.1803576115	journal	May 2018
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Aluminum Bis(trifluoromethanesulfonyl)imide as a Chloride-Free Electrolyte for Rechargeable Aluminum Batteries Chiku, Masanobu; Matsumura, Shota; Takeda, Hiroki Journal of The Electrochemical Society, Vol. 164, Issue 9 https://doi.org/10.1149/2.0701709jes	journal	January 2017
Ternary AlCl ₃ -Urea-[EMIm]Cl Ionic Liquid Electrolyte for Rechargeable Aluminum-Ion Batteries Li, Junfeng; Tu, Jiguo; Jiao, Handong Journal of The Electrochemical Society, Vol. 164, Issue 13 https://doi.org/10.1149/2.0811713jes	journal	January 2017
Graphene-Coated Activated Carbon Fiber Cloth Positive Electrodes for Aluminum Rechargeable Batteries with a Chloroaluminate Room-Temperature Ionic Liquid Tsuda, Tetsuya; Uemura, Yuya; Chen, Chih-Yao Journal of The Electrochemical Society, Vol. 164, Issue 12 https://doi.org/10.1149/2.0981712jes	journal	January 2017
The Aluminum-Ion Battery: A Sustainable and Seminal Concept? Leisegang, Tilmann; Meutzner, Falk; Zschornak, Matthias Frontiers in Chemistry, Vol. 7 https://doi.org/10.3389/fchem.2019.00268	journal	May 2019
Electrochemically Treated TiO2 for Enhanced Performance in Aqueous Al-Ion Batteries Holland, Alexander; McKerracher, Rachel; Cruden, Andrew Materials, Vol. 11, Issue 11 https://doi.org/10.3390/ma11112090	journal	October 2018
Graphene Nanoplatelet-Polysulfone Composite Cathodes for High-Power Aluminum Rechargeable Batteries Tsuda, Tetsuya; Uemura, Yuya; Chen, Chih-Yao Electrochemistry, Vol. 86, Issue 2 https://doi.org/10.5796/electrochemistry.17-00088	journal	January 2018

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aluminum-ion battery
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