Opportunities of Aqueous Manganese-Based Batteries with Deposition and Stripping Chemistry

Wang, Mingming; Zheng, Xinhua; Zhang, Xiang; Chao, Dongliang; Qiao, Shi‐Zhang; Alshareef, Husam N.; Cui, Yi; Chen, Wei

doi:10.1002/aenm.202002904

Opportunities of Aqueous Manganese-Based Batteries with Deposition and Stripping Chemistry

Journal Article · Mon Dec 21 04:00:00 EST 2020 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.202002904· OSTI ID:1768031

Wang, Mingming ^[1]; Zheng, Xinhua ^[1]; Zhang, Xiang ^[1]; Chao, Dongliang ^[2]; Qiao, Shi‐Zhang ^[2]; Alshareef, Husam N. ^[3]; Cui, Yi ^[4]; Chen, Wei ^[1]

Univ. of Science and Technology of China, Hefei (China)
Univ. of Adelaide, SA (Australia)
King Abdullah Univ. of Science and Technology (KAUST), Thuwal (Saudi Arabia)
Stanford Univ., CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)

Rechargeable aqueous manganese-based batteries have been attracting significant attention owing to their advantages of low cost, high safety, and ease of manufacturing, which are promising attributes for grid-scale energy storage applications. However, most traditional manganese-based batteries with solid-state conversion and intercalation reactions suffer from low capacity and poor long-term cycling stability. The recent novel storage mechanism based on cathode Mn²⁺/MnO₂ deposition/stripping chemistry has fundamentally tackled these issues, enabling a new generation of manganese-based batteries with superior electrochemical performance. Here, the recent advances in aqueous manganese-based batteries with the Mn²⁺/MnO₂ deposition/stripping chemistry are reviewed. Furthermore, a summary of the development of manganese-based batteries with different storage mechanisms is provided and new opportunities for the emerging Mn²⁺/MnO₂ chemistry in the latest generation are highlighted. Then, the current understanding of the Mn²⁺/MnO₂ charge storage mechanism and its potential in manganese-based batteries for large-scale energy storage applications is presented. Moreover, insights into opportunities and future directions for manganese-based batteries with the Mn²⁺/MnO₂ chemistry are proposed.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); University of Science and Technology of China (USTC); KAUST

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1768031

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 5 Vol. 11; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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