Controlling electron-ion rescattering in two-color circularly polarized femtosecond laser fields

Mancuso, Christopher A.; Hickstein, Daniel D.; Dorney, Kevin M.; Ellis, Jennifer L.; Hasović, Elvedin; Knut, Ronny; Grychtol, Patrik; Gentry, Christian; Gopalakrishnan, Maithreyi; Zusin, Dmitriy; Dollar, Franklin J.; Tong, Xiao-Min; Milošević, Dejan B.; Becker, Wilhelm; Kapteyn, Henry C.; Murnane, Margaret M.

doi:10.1103/physreva.93.053406

Controlling electron-ion rescattering in two-color circularly polarized femtosecond laser fields

Journal Article · Mon May 09 00:00:00 EDT 2016 · Physical Review A

DOI:https://doi.org/10.1103/physreva.93.053406· OSTI ID:1690340

Mancuso, Christopher A. ^[1]; Hickstein, Daniel D. ^[2]; Dorney, Kevin M. ^[2]; Ellis, Jennifer L. ^[2]; Hasović, Elvedin ^[3]; Knut, Ronny ^[2]; Grychtol, Patrik ^[2]; Gentry, Christian ^[2]; Gopalakrishnan, Maithreyi ^[2]; Zusin, Dmitriy ^[2]; Dollar, Franklin J. ^[2]; Tong, Xiao-Min ^[4]; Milošević, Dejan B. ^[5]; Becker, Wilhelm ^[6]; Kapteyn, Henry C. ^[2]; Murnane, Margaret M. ^[2]

Univ. of Colorado and NIST, Boulder, CO (United States); JILA, University of Colorado Boulder
Univ. of Colorado and NIST, Boulder, CO (United States)
Univ. of Sarajevo (Bosnia and Herzegovina)
Univ. of Tsukuba (Japan)
Univ. of Sarajevo (Bosnia and Herzegovina); Academy of Sciences and Arts of Bosnia and Herzegovina, Sarajevo (Bosnia and Herzegovina); Max-Born-Inst., Berlin (Germany)
Max-Born-Inst., Berlin (Germany)

High-harmonic generation driven by two-color counter-rotating circularly polarized laser fields was recently demonstrated experimentally as a breakthrough source of bright, coherent, circularly polarized beams in the extreme ultraviolet and soft-x-ray regions. However, the conditions for optimizing the single-atom yield are significantly more complex than for linearly polarized driving lasers and are not fully understood. In this study we present a comprehensive study of strong-field ionization—the complementary process to high-harmonic generation—driven by two-color circularly polarized fields. We uncover the conditions that lead to enhanced electron-ion rescattering, which should correspond to the highest single-atom harmonic flux. Using a velocity map imaging photoelectron spectrometer and tomographic reconstruction techniques, we record three-dimensional photoelectron distributions resulting from the strong-field ionization of argon atoms across a broad range of driving laser intensity ratios. In combination with analytical predictions and advanced numerical simulations, we show that “hard” electron-ion rescattering is optimized when the second-harmonic field has an intensity approximately four times higher than that of the fundamental driving field. We also investigate electron-ion rescattering with co-rotating fields, and find that rescattering is significantly suppressed when compared with counter-rotating fields.

View Accepted Manuscript (DOE)

Research Organization:: National Inst. of Standards and Technology (NIST), Boulder, CO (United States); Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: Japan Society for the Promotion of Science (JSPS); National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division

Grant/Contract Number:: FG02-99ER14982

OSTI ID:: 1690340

Alternate ID(s):: OSTI ID: 1252126
OSTI ID: 1690342

Journal Information:: Physical Review A, Journal Name: Physical Review A Journal Issue: 5 Vol. 93; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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